Yong-Hee Lee’s research while affiliated with Daejeon Institute of Science and Technology and other places

We demonstrate the quantitative pressure measurement of gas molecules in the mid-infrared using chip-based supercontinuum and cepstrum analysis without additional measurements for baseline normalization. A supercontinuum generated in an on-chip waveguide made of chalcogenide glass having high nonlinearity passes through CO gas and provides a transmission spectrum. The gas absorption information is deconvoluted from the original supercontinuum spectral information containing temporal fluctuation by cepstrum analysis and extracted simply by applying a bandpass filter in the temporal domain. The gas pressure estimated from the extracted absorption information is consistent with the value measured by a pressure gauge within a difference of 1.25%, despite spectral fluctuations in the supercontinuum baseline comparable to the spectral depth of the gas absorption lines.

We experimentally demonstrate a transverse magnetic (TM) mode laser in a photonic crystal (PhC) slab structure at room temperature. This study proposes a PhC nanobeam (NB) cavity to support a high-quality-factor (Q-factor) TM mode. For a large and complete photonic band gap, the PhC NB structures consist of large air holes in a thick dielectric slab. The PhC NB cavity is optimized numerically for a high-Q-factor TM mode of over 1 000 000 by reducing the radii of the air holes quadratically from the center to the edge of the PhC NB. A single-TM-mode lasing action is observed in an In-Ga-As-P quantum well (QW)-embedded optimized PhC NB cavity structure at room temperature via optical pulse pumping, where the QW layer is lightly etched. We believe that the TM mode lasers in PhC NB cavities with a lightly etched QW can be good candidates for a surface plasmon excitation source or a highly sensitive optical sensor.

We first experimentally demonstrated a transverse magnetic (TM) mode laser in a Photonic crystal (PhC) slab structure at room temperature. This study proposes a PhC nanobeam (NB) cavity to support a high-quality-factor (Q-factor) TM mode. For a large and complete photonic bandgap, the PhC NB structures consist of large air holes in a thick dielectric slab. The PhC NB cavity was optimized numerically for a high-Q-factor TM mode of over 1,000,000 by reducing the radii of the air holes quadratically from the center to the edge of the PhC NB. A single TM mode lasing action was observed in an InGaAsP quantum-well (QW)-embedded optimized PhC NB cavity structure at room temperature via optical pulse pumping, where the QW layer was lightly etched. We believe that the TM mode lasers in PhC NB cavities with a lightly etched QW can be good candidates for a surface plasmon excitation source or a highly sensitive optical sensor.

We report a supercontinuum generation (SCG) in a waveguide that spontaneously forms without an etching process during the deposition of a core material on a preformed ${\rm{Si}}{{\rm{O}}_2}$ substructure. The mechanism of dispersion control for this new, to the best of our knowledge, type of waveguide is analyzed by numerical simulation, which results in a design rule to achieve a target dispersion profile by adjusting the substructure geometry. SCG is experimentally demonstrated with a waveguide made of ${\rm{A}}{{\rm{s}}_2}{{\rm{S}}_3}$ , chalcogenide glass, which has low material absorption over the mid-IR range. A dispersion-controlled waveguide with a length of 10 mm pumped with 77 pJ pulses at a telecommunication wavelength of 1560 nm resulted in a supercontinuum that extends by more than 1.5 octaves.

We demonstrated lasing from TM modes in photonic nanobeam cavities. By varying the radius of air holes, Q-factor reaches around 1,000,000. The single-mode lasing action was performed at room temperature, and confirmed by numerical results.

By providing an effective way to leverage nonlinear phenomena in integrated devices, high-Q optical resonators have led to recent advances in on-chip photonics. However, developing fabrication processes to shape any new material into a resonator with extremely smooth surfaces on a chip has been an exceptionally challenging task. Here, we describe a universal method to implement ultra-high-Q resonators with any new material having desirable properties that can be deposited by physical vapor deposition. Using this method light-guiding cores with surface roughness on the molecular-scale are created automatically on pre-patterned substrates. Its efficacy has been verified using As2S3, a chalcogenide glass that has high-nonlinearity. The Q-factor of the As2S3 resonator so-developed approached the propagation loss record achieved in chalcogenide fibers which were limited by material losses. Owing to the boosted Q-factor, lasing by stimulated Brillouin scattering has been demonstrated with 100 times lower threshold power than the previous record.

Thermally induced particle hopping in the nanoscale double-well potential is fundamental in material design and device operation. After the proposal of the basic hopping theory, several experimental studies, including some using the optical trapping method, have validated the theoretical approach over various friction ranges of the surrounding medium. However, only external parameters, such as viscosity, temperature, and pressures, have been varied in practical circumstances, and other tools capable of adjusting the potential profile itself to modulate the hopping rate are needed. By using metallic nanoantenna with various gap sizes and different optical pump power, we engineered a double-well potential landscape and directly observed the hopping of a single nanoparticle with a diameter of 4 nm. The distance between the two potential wells was 0.6-5 nm, and the maximum well depth and maximum height of the central potential barrier were approximately 69 and 4 k B T, respectively. The hopping rate was governed by the Arrhenius law and showed a vertex when the barrier height was approximately 2 k B T, which was in good agreement with the computational expectations.

Thermally induced particle hopping in the nanoscale double-well potential is fundamental in material design and device operation. After the proposal of the basic hopping theory, several experimental studies, including some using the optical trapping method, have validated the theoretical approach over various friction ranges of the surrounding medium. However, only external parameters, such as viscosity, temperature, and pressures, have been varied in practical circumstances, and other tools capable of adjusting the potential profile itself to modulate the hopping rate are needed. By using metallic nanoantenna with various gap sizes and different optical pump power, we engineered a double-well potential landscape and directly observed the hopping of a single nanoparticle with a diameter of 4 nm. The distance between the two potential wells was 0.6–5 nm, and the maximum well depth and maximum height of the central potential barrier were approximately 69 and 4 kBT, respectively. The hopping rate was governed by the Arrhenius law and showed a vertex when the barrier height was approximately 2 kBT, which was in good agreement with the computational expectations.

Recent development in nanofabrication technology has enabled the fabrication of plasmonic nanoapertures that can provide strong field concentrations beyond the diffraction limit. Further utilization of plasmonic nanoaperture requires the broadband tuning of the operating wavelength and precise control of aperture geometry. Here, we present a novel plasmonic coaxial aperture that can support resonant extraordinary optical transmission (EOT) with a peak transmittance of ~10% and a wide tuning range over a few hundred nanometers. Because of the shadow deposition process, we could precisely control the gap size of the coaxial aperture down to the sub–10-nm scale. The plasmonic resonance of the SiN x /Au disk at the center of the coaxial aperture efficiently funnels the incident light into the sub–10-nm gap and allows strong electric field confinement for efficient second harmonic generation (SHG), as well as EOT. In addition to the experiment, we theoretically investigated the modal properties of the plasmonic coaxial aperture depending on the structural parameters and correlation between EOT and SHG through finite-difference time-domain simulations. We believe that our plasmonic coaxial apertures, which are readily fabricated by the nanoimprinting process, can be a versatile, practical platform for enhanced light–matter interaction and its nonlinear optical applications.