Song Luo’s research while affiliated with Xiamen University and other places

ZnO nanowire (NW) lasing driven by mid-infrared (MIR) laser pulses has attracted significant attention owing to its remarkable wavelength-independent lasing threshold and potential applications in diverse situations. However, the properties of MIR laser-driven ZnO microwire (MW) lasing are rarely studied when the wire diameter is increased from nanoscale to microscale, comparable to the wavelength of the driving laser. Here we experimentally measured the ZnO MW lasing driven by MIR laser with different polarizations. The measurements show that the laser polarized along the c axis was more efficient for the lasing in MW with diameter smaller than the driving laser wavelength, while the polarization dependence was ambiguous when the MW diameter was greater than the driving laser wavelength. Through the modeling of the lasing process in ZnO MW, the observed polarization dependence is reproduced and can be attributed to the combined effect of the optical interference of the driving laser in the MW and the varying absorption properties of different MWs. The former is related to the MW diameter and the latter is sensitive to the sample growth condition. Our findings shed light on the feasibility of manipulation of the ZnO MW lasing.

We propose an all-optical scheme of topological lasing and switching based on the Aubry-André-Harper (AAH) model of an exciton-polariton chain. We theoretically show that the phase parameter of the optical potential, with a tunable effective quasimomentum, allows the system to exhibit nontrivial topological properties which are attributed to higher dimensions. The topological modes emerging within the bulk band gaps are spatially localized at the edges of the polariton lattice, and their topological properties are characterized by the nonzero Chern numbers of the bulk bands. Polariton lasing in topological edge modes exhibits a higher efficiency and better robustness than in bulk modes, and can be switched between two opposite edges of the lattice by nonresonant excitation, which paves a way for topologically protected optical circuits.

Pursuing nanometer-scale nonlinear converters based on second harmonic generation (SHG) is a stimulating strategy for bio-sensing, on-chip optical circuits, and quantum information processing, but the light-conversion efficiency is still poor in such ultra-small dimensional nanostructures. Herein, we demonstrate a highly enhanced broadband frequency converter through a hybrid plasmonic–dielectric coupler, a ZnTe/ZnO single core–shell nanowire (NW) integrated with silver (Ag) nanoparticles (NPs). The NW dimension has been optimized to allow the engineering of dielectric resonances at both fundamental wave and second harmonic frequencies. Meanwhile, the localized surface plasmon resonances are excited in the regime between the Ag NPs and ZnTe/ZnO dielectric NW, as evidenced by plasmon-enhanced Raman scattering and resonant absorption. These two contributors remarkably enhance local fields and consequently support the strong broadband SHG outputs in this hybrid nanostructure by releasing stringent phase-matching conditions. The proposed nanoscale nonlinear optical converter enables the manipulation of nonlinear light–matter interactions toward the development of on-chip nanophotonic systems.

Absorption spectroscopy has long been hailed as an absolute necessity for detecting the properties of complex chemical and biological samples. While conventional spectroscopy using classical light is severely limited by shot noise and lacks robustness against experimental imperfections, quantum light offers an avenue to perform absorption spectroscopy with provable advantages in the technical operations and the measurement precision. Here, we present an experimental approach to implement entanglement-based absorption spectroscopy with the assistance of Hong-Ou-Mandel interference. Since the temporal interference fringe is determined by the spectrum pattern, a maximum-likelihood decision is sufficient for revealing the relevant quantum information about the absorptive properties of the test samples. These experimental results may significantly facilitate the use of quantum interferometric spectroscopy to practical applications, which may be particularly relevant for photon-sensitive biological and chemical samples.

Whispering gallery modes in a microwire are characterized by a nearly equidistant energy spectrum. In the strong exciton-photon coupling regime, this system represents a bosonic cascade: a ladder of discrete energy levels that sustains stimulated transitions between neighboring steps. In this work, by using femtosecond angle-resolved spectroscopic imaging technique, the ultrafast dynamics of polaritons in a bosonic cascade based on a one-dimensional ZnO whispering gallery microcavity is explicitly visualized. Clear ladder-form build-up process from higher to lower energy branches of the polariton condensates are observed, which are well reproduced by modeling using rate equations. Moreover, the polariton parametric scattering dynamics are distinguished on a timescale of hundreds of femtoseconds. Our understanding of the femtosecond condensation and scattering dynamics paves the way towards ultrafast coherent control of polaritons at room temperature, which will make it promising for high-speed all-optical integrated applications.