Siwei Mao’s research while affiliated with Chinese Academy of Sciences and other places

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Publications (7)


Fig. 1 (a) The schematic diagram of Co 2 MnSi/GaAs/PZT heterostructures controlled by piezo-voltages. When the piezo-voltages were applied, the direction of the strain is parallel to the z-axis. The [1À10] and [110] directions are parallel to the z-axis in samples I and II, respectively. The inset figures are the schematic of an axially acting multilayer piezo-stack and the structure of the magnetic film. (b) The magnetic hysteresis loops of the Co 2 MnSi thin film in the initial state along the in-plane [110], [1À10], and [100] directions. The inset shows the saturated magnetization in the [100] direction with 420 Oe magnetic field.
Fig. 2 The magnetic hysteresis loops under different piezo-voltages (from À60 V to 50 V; step is 10 V) along the in-plane [1À10] and [110] directions. (a) The magnetic hysteresis loops in the [1À10] direction are square curves with U PZT > À10 V. (b) Contrary to (a), the square curve changed to two-step curves with U PZT < À30 V and the saturated field increased with the increase of U PZT absolute value. (c) The magnetic hysteresis loops in the [110] direction are changed to two-step curves from square curves with U PZT > 0 V. (d) The magnetic hysteresis loops keep the square curve with U PZT < À30 V (compressed states).
Fig. 3 The magnetic properties of the Co 2 MnSi film under different piezo-voltages. (a) Compared with the Co 2 MnSi film under different piezovoltages, the magnetic hysteresis loops of [1À10] and [110] directions keep square and two-step curves with U PZT ¼ 40 V (stretched states), respectively. (b) The two-step axis and the square axis are exchanged with U PZT ¼ À40 V (compressed states). (c) The piezo-voltage dependence of the saturation field in the [1À10] and [110] directions; the voltage step is 5 V. (d) The magnetic hysteresis loops maintain the hard axis in the [100] direction under different piezo voltages.
Fig. 4 The magnetic hysteresis loops under different piezo-voltages (from À40 V to 90 V, step is 10 V) along the in-plane [110] and [1À10] directions of the sample II. (a) The magnetic hysteresis loops in the [110] direction change to square curves from two-step curves with U PZT > 20 V (stretched states). (b) The magnetic hysteresis loops in the [110] direction keep the two-step curves with U PZT < À20 V and the saturation field increase with the negative piezo-voltage increase. (c) The magnetic hysteresis loops in the [1À10] direction are changed to two-step curves from square curves with U PZT > 40 V. (d) The magnetic hysteresis loops keep the square curve with U PZT < À20 V in the [1À10] direction.
Fig. 5 The magnetic properties of the Co 2 MnSi film under different piezo-voltages. (a) The piezo-voltage dependence of the saturation field in the [1À10] and [110] directions; the voltage step is 10 V. (b) The magnetic hysteresis loops maintain the hard axis in the [100] direction under different piezo-voltages. The inset is the definition of the q and a. q(a) is the angle between the magnetization (magnetic field) and [1À10] direction.

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Dual-axis control of magnetic anisotropy in single crystal Co 2 MnSi thin film through piezo-voltage-induced strain
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May 2022

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79 Reads

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siwei Mao

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Chunlong Li

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Voltage controlled magnetic anisotropy (VCMA) has been considered as an effective method in traditional magnetic devices with lower power consumption. In this article, we have investigated the dual-axis control of magnetic anisotropy in Co2MnSi/GaAs/PZT hybrid heterostructures through piezo-voltage-induced strain using longitudinal magneto-optical Kerr effect (LMOKE) microscopy. The major modification of in-plane magnetic anisotropy of the Co2MnSi thin film is controlled obviously by the piezo-voltages of the lead zirconate titanate (PZT) piezotransducer, accompanied by the coercivity field and magnetocrystalline anisotropy significantly manipulated. Because in-plane cubic magnetic anisotropy and uniaxial magnetic anisotropy coexist in the Co2MnSi thin film, the initial double easy axes of cubic split to an easiest axis (square loop) and an easier axis (two-step loop). While the stress direction is parallel to the [1-10] easiest axis (sample I), the square loop of the [1-10] direction could transform to a two-step loop under the negative piezo-voltages (compressed state). At the same time, the initial two-step loop of the [110] axis simultaneously changes to a square loop (the easiest axis). Otherwise, we designed and fabricated the sample II in which the PZT stress is parallel to the [110] two-step axis. The phenomenon of VCMA was also obtained along the [110] and [1-10] directions. However, the manipulated results of sample II were in contrast to those of the sample I under the piezo-voltages. Thus, an effective dual-axis regulation of the in-plane magnetization rotation was demonstrated in this work. Such a finding proposes a more optimized method for the magnetic logic gates and memories based on voltage-controlled magnetic anisotropy in the future.

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Antiferromagnet-mediated spin–orbit torque induced magnetization switching in perpendicularly magnetized L 1 0 -MnGa

March 2021

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12 Reads

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7 Citations

Current-induced magnetization switching plays an essential role in spintronic devices exhibiting nonvolatility, high-speed processing, and low-power consumption. Here, we report on the spin–orbit torque-induced magnetization switching in perpendicularly magnetized L10-MnGa/FeMn/Pt trilayers grown by molecular-beam epitaxy. An antiferromagnetic FeMn layer is inserted between the spin current generating Pt layer and spin absorbing MnGa layer. Due to the exchange bias effect, the trilayers show field-free spin–orbit torque switching. Overall, the spin transmission efficiency decreases monotonically as the FeMn thickness increases. It is found that the spin current can be transmitted through an 8 nm-thick FeMn layer as evidenced by partial switching of the L10-MnGa. The damping-like spin–orbit torque efficiency shows a peak value at tFeMn = 1.5 nm due to the enhanced interfacial spin transparency and crystalline quality of the FeMn. These results help demonstrate the efficacy of emerging spintronic devices containing antiferromagnetic elements.


(a) Schematic diagram of idealized L10-MnAl crystal structure. (b) XRD (θ–2θ) pattern of the Co2MnSi(1 nm)/L10-MnAl(65 nm) thin film, peaks marked with * are from the substrate. (c) AFM image. (d) In-plane and out-of-plane hysteresis loops of Co2MnSi(1 nm)/L10-MnAl(65 nm) prepared at 350 °C.
(a) HRTEM image of the Co2MnSi(1 nm)/L10-MnAl(15 nm)/MgO(2.5 nm)/Co2MnSi(0.8 nm)/MnAl(5 nm)/ Pt(2.5 nm) MTJ structure. (b) HRTEM image of the region around MgO barrier. (c) HAADF (Z-contrast) STEM image. (d)–(g) EDS mapping data of Mn, Al, Mg and Co elements.
(a) Schematic diagram of the band structure of Co2MnSi and MnAl. (b) TMR behavior for MnAl/MgO/Co2MnSi/MnAl structure measured at 5 K. (c) Schematic diagrams of the magnetization states in figure (b).
(a) Temperature dependence of TMR ratio. (b) Temperature dependence of junction resistance in parallel and anti-parallel magnetization configuration. (c) Bias voltage dependence of (dI/dV)/(dI/dV)V=0. (d) Bias voltage dependence of normalized TMR measured at 5 K.
I–V curve measured by current source (mode 6221, KEITHLEY Inst. Inc.) and nanovoltmeter (mode 2182, KEITHLEY Inst. Inc.) at 5 K. The result fitted by Brinkman’s model is shown by the red line. The inset shows wide range I–V relationship, a nonlinear I–V behavior reflects the character of tunneling conductance.
Observation of tunneling magnetoresistance effect in L10-MnAl/MgO/Co2MnSi/MnAl perpendicular magnetic tunnel junctions

July 2019

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134 Reads

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12 Citations

We report on the tunneling magnetoresistance (TMR) effect in fully perpendicular magnetic tunnel junctions (p-MTJs) with the core structure of L10-MnAl/MgO/Co2MnSi/MnAl. The multilayer is epitaxially grown on GaAs (0 0 1) substrate by molecular-beam epitaxy (MBE), and both the top and bottom MnAl layers show well perpendicular magnetic anisotropy (PMA). Meanwhile, an inverse TMR effect with the MR ratio of 10% is observed at 5 K, which is attributed to the intrinsic negative spin polarization of MnAl in contrast to the positive one in Co2MnSi. This work proposes a MnAl-based fully p-MTJ for future STT-MRAM applications.


Design and Synthesis of an Artificial Perpendicular Hard Ferrimagnet with High Thermal and Magnetic Field Stabilities

December 2017

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191 Reads

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8 Citations

It is of great fundamental and practical interest to develop effective means of modulating the magnetic hystereses of magnetic materials and their heterostructures. A notable example is the exchange bias (EB) effect between an antiferromagnet or ferrimagnet and a ferromagnet, which has been widely employed to manipulate magnetic anisotropy in spintronic devices and artificial magnets. Here, we report the design, synthesis and characterization of a synthetic perpendicularly-magnetized ferrimagnet based on [Mn2.9Ga/Co2MnSi]n superlattices, which attains thermal stability above 400 K and a coercive field up to 45 kOe through a mechanism of magnetic compensation. The structure is incorporated into a prototype Heusler alloy and MgO barrier based magnetic tunnel junction, which demonstrates high dynamic range linear field responses and an unusual in-plane EB effect. With increasing temperature, the coercive field reaches beyond 70 kOe at 400 K in this device due to the increasing degree of magnetic moment compensation in the superlattice. The results demonstrate that the compensation mechanism can be utilized to achieve simultaneous thermal robustness and high coercivity in realistic spintronic devices.



Figure 2. (a) HRTEM image of the whole MTJ structure. (b) HRTEM image of the region around MgO barrier. (c) Z-contrast STEM image. (d–f) Plane-scan EDS data of Mg, Co and Mn element distributions.  
Figure 3. Hysteresis loop of the MTJ sample measured at 280 K with magnetic field perpendicular to the sample surface.
Figure 4. (a) Room-temperature TMR behavior for MnGa/Co 2 MnSi/MgO/Co 2 MnSi/MnGa structure. The inset shows the temperature dependence of the junction resistance. (b) Schematic diagram of the magnetization state.
Figure 5. Temperature dependence of TMR ratio for MnGa-based MTJ. (Minor loop within ± 20 kOe).
Figure 6. Bias voltage dependence of (dI/dV)/(dI/dV) V=0 in the parallel magnetization configuration (black line) and bias voltage dependence of TMR ratio (red line) measured at 10 K.
MnGa-based fully perpendicular magnetic tunnel junctions with ultrathin Co2MnSi interlayers

February 2017

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454 Reads

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40 Citations

Because tetragonal structured MnGa alloy has intrinsic (not interface induced) giant perpendicular magnetic anisotropy (PMA), ultra-low damping constant and high spin polarization, it is predicted to be a kind of suitable magnetic electrode candidate in the perpendicular magnetic tunnel junction (p-MTJ) for high density spin transfer torque magnetic random access memory (STT-MRAM) applications. However, p-MTJs with both bottom and top MnGa electrodes have not been achieved yet, since high quality perpendicular magnetic MnGa films can hardly be obtained on the MgO barrier due to large lattice mismatch and surface energy difference between them. Here, a MnGa-based fully p-MTJ with the structure of MnGa/Co2MnSi/MgO/Co2MnSi/MnGa is investigated. As a result, the multilayer is with high crystalline quality, and both the top and bottom MnGa electrodes show well PMA. Meanwhile, a distinct tunneling magnetoresistance (TMR) ratio of 65% at 10 K is achieved. Ultrathin Co2MnSi films are used to optimize the interface quality between MnGa and MgO barrier. A strong antiferromagnetic coupling in MnGa/Co2MnSi bilayer is confirmed with the interfacial exchange coupling constant of −5erg/cm2. This work proposes a novel p-MTJ structure for the future STT-MRAM progress.


Citations (4)


... Magnon torque current, which can transfer angular momentum from an insulating antiferromagnetic (AFM)/ferromagnetic insulator to the magnetic moment of an adjacent ferromagnetic layer, can be of importance parallel to the electronic spin current in many different spintronic applications. [1][2][3][4][5][6] While the magnon torque has demonstrated several crucial advantages over spin-polarized electrical currents, including low Joule heating, the potential for long-distance information transmission, and immunity to disruptive magnetic fields, 1,4,[7][8][9][10][11][12] its relationship with the magnetic order has yet to be fully elucidated. Particularly noteworthy is the recent finding that the antiferromagnetic layer can serve as an efficient spin current amplifier and carrier, especially in ultra-thin film configurations. ...

Reference:

Temperature-dependent magnon torque in SrIrO3/NiO/ferromagnetic multilayers
Antiferromagnet-mediated spin–orbit torque induced magnetization switching in perpendicularly magnetized L 1 0 -MnGa
  • Citing Article
  • March 2021

... [7][8][9][10][11][12] Therefore, there have been many studies focusing on those thin films for such STT-device applications. [13][14][15][16][17][18][19][20][21][22][23][24][25][26][27] One issue of p-MTJs using Mn-based ordered magnetic alloys has been their low tunnel magnetoresistance (TMR) effect. The TMR effect is used for memory reading in STT-MRAM, for examples, therefore the TMR ratio should be large, at least, more than 100% for practical use. ...

Observation of tunneling magnetoresistance effect in L10-MnAl/MgO/Co2MnSi/MnAl perpendicular magnetic tunnel junctions

... [7][8][9][10][11][12] Therefore, there have been many studies focusing on those thin films for such STT-device applications. [13][14][15][16][17][18][19][20][21][22][23][24][25][26][27] One issue of p-MTJs using Mn-based ordered magnetic alloys has been their low tunnel magnetoresistance (TMR) effect. The TMR effect is used for memory reading in STT-MRAM, for examples, therefore the TMR ratio should be large, at least, more than 100% for practical use. ...

MnGa-based fully perpendicular magnetic tunnel junctions with ultrathin Co2MnSi interlayers