Roshan Achal's research while affiliated with University of Alberta and other places

Publications (20)

Article
Many diverse material systems are being explored to enable smaller, more capable and energy efficient devices. These bottom up approaches for atomic and molecular electronics, quantum computation, and data storage all rely on a well-developed understanding of materials at the atomic scale. Here, we report a versatile scanning tunneling microscope (...
Article
With nanoelectronics reaching the limit of atom-sized devices, it has become critical to examine how irregularities in the local environment can affect device functionality. Here, we characterize the influence of charged atomic species on the electrostatic potential of a semiconductor surface at the sub-nanometer scale. Using noncontact atomic forc...
Preprint
Many new material systems are being explored to enable smaller, more energy efficient and capable electronic devices. In the extreme size limits, approaches for atomic and molecular electronics, quantum computation, and data storage all rely on a well-developed understanding of the behaviour of materials at the atomic scale. Here, we report a scann...
Preprint
With nanoelectronics reaching the limit of atom-sized devices, it has become critical to examine how irregularities in the local environment can affect device functionality. Here, we characterize the influence of charged atomic species on the electrostatic potential of a semiconductor surface at the sub-nanometer scale. Using non-contact atomic for...
Article
Full-text available
It has been proposed that miniature circuitry will ultimately be crafted from single atoms. Despite many advances in the study of atoms and molecules on surfaces using scanning probe microscopes, challenges with patterning and limited thermal structural stability have remained. Here we demonstrate rudimentary circuit elements through the patterning...
Article
Full-text available
At the atomic scale, there has always been a trade-off between the ease of fabrication of structures and their thermal stability. Complex structures that are created effortlessly often disorder above cryogenic conditions. Conversely, systems with high thermal stability do not generally permit the same degree of complex manipulations. Here, we repor...
Article
Full-text available
We report on tuning the carrier capture events at a single dangling bond (DB) midgap state by varying the substrate temperature, doping type, and doping concentration. All-electronic time-resolved scanning tunneling microscopy (TR-STM) is employed to directly measure the carrier capture rates on the nanosecond time scale. A characteristic negative...
Article
Full-text available
The miniaturization of semiconductor devices to the scales where small numbers of dopants can control device properties requires the development of new techniques capable of characterizing their dynamics. Investigating single dopants requires sub-nanometer spatial resolution which motivates the use of scanning tunneling microscopy (STM), however, c...
Article
Full-text available
Nanoelectronics has long striven for the ultimate limit of fabrication: reliable use of single atoms as building blocks for computational components. This has required years of development in tools not only to manipulate single atoms with sub-angstrom precision, but also tools that can read the sensitive outputs and dynamics. Here, we report the fi...
Article
We report the mechanically induced formation of a silicon-hydrogen covalent bond and its application in engineering nanoelectronic devices. We show that using the tip of a non-contact atomic force microscope, a single H atom could be vertically manipulated. When applying a localized electronic excitation, a single hydrogen atom is desorbed from the...
Article
Full-text available
As the ultimate miniaturization of semiconductor devices approaches, it is imperative that the effects of single dopants be clarified. Beyond providing insight into functions and limitations of conventional devices, such information enables identification of new device concepts. Investigating single dopants requires sub-nanometre spatial resolution...
Data
Supplementary Figures 1-6, Supplementary Notes 1-2 and Supplementary References
Article
Full-text available
Here we report the direct observation of single electron charging of a single atomic dangling bond (DB) on the H-Si(100)-2×1 surface. The tip of a scanning tunneling microscope is placed adjacent to the DB to serve as a single-electron sensitive charge detector. Three distinct charge states of the dangling bond-positive, neutral, and negative-are d...
Article
Full-text available
Here we report the observation and control of single electron charging of atomic Dangling Bonds. The tip of a scanning tunneling microscope is placed adjacent to the dangling bond to serve as a single electron sensitive charge-sensor. Three distinct charge states of the dangling bond, positive, neutral and negative are discerned. Charge state popul...

Citations

... The controlled change of the DB charge state allows to study interesting and complex physical phenomena, making the DBs attractive from the fundamental point of view [7][8][9][10]. From the practical point of view, DBs are promising for many applications in atomic scale silicon-based electronic devices due to the well-developed process of their precise creation on Si(100)-2 × 1-H [11][12][13][14]. ...
... This is because electric charges are shielding the electrostatic field. More precisely, the electrostatic potential Vi,j at position i generated by an SiDB in state nj ∈ {−1, 0, 1} at position j is given by [8], [29] ...
... Recent years have seen an increase in scientific interest in the Silicon Dangling Bond (SiDB) logic platform-an emerging computational beyond-CMOS nanotechnology [1]- [7]. Of particular significance are its sub-nanometer elementary devices that allow for an integration density improvement of several orders of magnitude over current CMOS fabrication nodes [3], [4], [6]- [11]; and its properties to compute Boolean logic without the flow of electrostatic current but, instead, via the Coulombic repulsion of charges [4], [8]. By this, SiDB logic promises ultra-low energy dissipation and establishes itself as a highly-anticipated green competitor in the beyond-CMOS domain [3], [8], [11]- [15]. ...
... Recently, atom manipulation has been extended to platforms including superconductors 9,10 , 2D materials [11][12][13] , semiconductors 14,15 , and topological insulators 16 to create topological and many-body effects not found in naturally occurring materials. In addition, atom manipulation is used to build and operate computational devices scaled to the limit of individual atoms, including quantum and classical logic gates [17][18][19][20] , memory 21,22 , and Boltzmann machines 23 . ...
... Trap states are normally hard to be controlled in conventional semiconductors. However, with the help of STM, the trap states can be introduced more precisely, [134,135] which may find applications in negative differential resistance devices. [136,137] For instance, PbS/(p-type etched) InP with interfacial trapping states are employed in neuromorphic computing through a STM circuit based on single-electron tunneling, acting as both synapses (weighted connections) and spiking elements. ...
... Recent years have seen an increase in scientific interest in the Silicon Dangling Bond (SiDB) logic platform-an emerging computational beyond-CMOS nanotechnology [1]- [7]. Of particular significance are its sub-nanometer elementary devices that allow for an integration density improvement of several orders of magnitude over current CMOS fabrication nodes [3], [4], [6]- [11]; and its properties to compute Boolean logic without the flow of electrostatic current but, instead, via the Coulombic repulsion of charges [4], [8]. By this, SiDB logic promises ultra-low energy dissipation and establishes itself as a highly-anticipated green competitor in the beyond-CMOS domain [3], [8], [11]- [15]. ...
... The bandwidth of the electronics used in STM is typically in the kHz range, Journal of Applied Physics corresponding to a time resolution of milliseconds. 30,31 However, this limitation can be overcome with the use of ultrashort pulsed lasers. 32 Instead of measuring the time evolution of the tunneling current directly, researchers shined ultrashort optical double pulses onto an STM tip and observed tunneling current variations as a function of the time interval between the pulses. ...
... First, we list features that involve only one side of a dimer. These We start with a discussion of silicon DBs, which are wellstudied unterminated silicon atoms [52][53][54]. In STM, the centre of a DB is imaged as a bright protrusion due to its conductive orbital which extends into vacuum. ...
... The locations can be atomically accurate due to the regular surface lattice structure as illustrated in Fig. 1. They were found to behave like quantum dots as their energetic charge transition levels fall within the bulk band gap, allowing them to take on vacant, singly-occupied, or doubly-occupied states corresponding to positive, neutral, and negative charge states [17], [18]. In [5], Huff et al. experimentally demonstrated logic cells, wires, and an OR gate that represented logic states via the location of charges shared between pairs of SiDBs as illustrated in Fig. 1. ...