Michael P. Short’s research while affiliated with Massachusetts Institute of Technology and other places

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Publications (33)


Beam heating explains critical current suppression measured during ion irradiation of REBCO tapes
  • Article

November 2024

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17 Reads

Superconductor Science and Technology

Alexis Rustam Devitre

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David X Fischer

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Zachary Seth Hartwig

Reports of critical current (Ic\rm I_c) suppression during cryogenic ion irradiation of REBCO tapes have raised concerns for the operational margins of fusion power plant (FPP) magnets. However, the data remain inconclusive regarding beam heating due to the difficulty of measuring local temperatures with contact probes. This leaves a critical knowledge gap concerning the mechanism behind Ic\rm I_c suppression, and whether the so-called \textit{beam on effect} is to be expected under neutron irradiation during FPP operation. In this paper, we show that Ic\rm I_c suppression is independent of atomic displacement rate in the REBCO layer, the latter of which increases twelve-fold as we reduce the beam energy from 2400 to 800~keV. At fixed power, we observe statistically identical suppression with 150~keV protons, which do not have enough energy to reach the REBCO layer, refuting hypotheses about beam on effects being caused by nuclear displacements or direct ion-Cooper pair interactions. These results show that REBCO temperature rise alone can explain Ic\rm I_c suppression, leaving little to no margin for alternative mechanisms. With this insight, we developed a method to measure beam spot temperature that does not depend on the specific installation of our temperature sensor. With this new method, we measured the temperature gradient across the tape during irradiation and found that thermal resistance at the tape/target interface is the controlling variable in Ic\rm I_c suppression. As such, accelerator-based facilities aiming to reproduce the operation of REBCO magnets in a nuclear fusion environment should find strategies to minimize interface thermal resistance. Most importantly, we find that the dose rates expected in a FPP will not change Ic\rm I_c due to ballistic radiation damage or ion-Cooper pair interactions, allowing us to safely ignore these effects when designing FPP magnets.





Decomposition of the TGS signal from pure tungsten for reference. Shows frequency, thermal decay, and acoustic damping as they relate to the signal. Frequency is used to yield the elastic properties of material from SAW frequency. Thermal decay informs thermal diffusivity. The amplitude decay of oscillations is contributed to by acoustic damping and the SAW packet exiting the probe. The DC level in this case is near zero and corresponds to the average intensity of the light detected by the sensor when the beam is present.
(a) Schematic of major TGS components, including the detector (APD), phase adjusters 1 and 2 (PA1, PA2), phase mask, and the linear stage with sample and vacuum port, as well as other optical devices used for beam manipulation and fine tuning. (b) Picture of the complete TGS setup.
Exploded view of wafer holder assembly.
Sample TGS measurement from a pure tungsten calibration sample. Fitting is performed on the trace a short time after its peak. In red is the functional fit for an ideal TGS waveform lain overtop the recorded trace. Start time refers to the start of the signal spike, and only data after the time index are used for fitting. Upper right depicts the Fourier transform, the peak of which corresponds to a SAW frequency of 4.36 × 10⁸ Hz, which is concurrent with expected values.
Diagram of the mapping control scheme. Thick black, green, and red arrows represent moving to the next stage in the control scheme, represented by rectangles. Thin grey arrows represent the output of remembered data, which are shown in ovals. Each scanning point follows a flow where it is compared against the minimum and previous signal amplitude and determined whether to probe for a better signal or move to the next point until mapping is finished.

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Automated transient grating spectroscopy mapping and signal control for large samples
  • Article
  • Full-text available

July 2024

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7 Reads

We present developments for the mapping of large areas using transient grating spectroscopy (TGS) that allow for smoother, larger, autonomous measurements of material samples. The addition of a precise linear stage in the direction parallel to laser sampling coupled with signal optimizing control allows for hands free, self-correcting measurements. In addition, the simplification of the sample holding design to a form that is small enough to mount directly to the linear stage exhibits a straightforward, low-cost solution for automated TGS applications. This capability is demonstrated by taking large uninterrupted maps of gradient wafers, and the results are validated on calibrated tungsten samples and control TGS samples from gradient wafers.

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A facility for cryogenic ion irradiation and in situ characterization of rare-earth barium copper oxide superconducting tapes

June 2024

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34 Reads

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3 Citations

Superconducting magnets based on Rare Earth Barium Copper Oxides (REBCO) offer transformative capabilities in the fields of fusion energy, high energy physics, and space exploration. A challenge shared by these applications is the limited lifetime of REBCO due to radiation damage sustained during operation. Here we present a new ion-beam facility that enables simultaneous cryogenic irradiation and in situ characterization of commercial REBCO tapes. The ion source provides spatially uniform fluxes up to 10¹⁸ protons/m²s with kinetic energies up to 3.4 MeV, in addition to helium and higher-Z species. Using this facility, we can induce uniform damage profiles in the first 10–20 µm of REBCO tapes with less than 0.25 appm of hydrogen implanted in REBCO after a dose of 10²⁰ protons/m². The tape can be held between 20 and 300 K with an accuracy of ±0.1 K and is connected to a four-point probe measuring the critical current, Ic, and critical temperature, Tc, before, during, and after irradiation with transport current ranging from 100 nA to 100 A, and a typical voltage noise less than 0.1 μV. These capabilities are presently used to study the effect of irradiation temperature on REBCO performance change during and after proton bombardment, to assess the possibility of Ic and Tc recovery after irradiation through thermal annealing, and to explore the instantaneous and recoverable suppression of Ic and Tc observed during irradiation.




Open volume defect accumulation with irradiation in GaN, GaP, InAs, InP, Si, ZnO, and MgO

December 2023

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48 Reads

Vacancies are generated in semiconductor devices while operating in the space radiation environment, impacting semiconductor carrier concentrations and dynamics. Positron annihilation lifetime spectroscopy (PALS) is used to probe these defect concentrations in bulk grown GaN, GaP, InAs, InP, Si, MgO, and ZnO both as-grown and as a function of 2–4 MeV proton irradiation. All samples were irradiated to yield a common initial damage production and characterized identically. In as-grown samples, PALS reveals vacancy concentrations above the saturation limit in the oxides, disabling further analysis. As a function of dose, of the materials in which defect accumulation could be probed, it is observed that GaN is the most resistant to the accumulation of defects (attributed to the Ga vacancies) and Si is the least. GaP (attributed to the Ga vacancy) and InAs exhibit slightly higher rates of vacancy accumulation than GaN. InP exhibits high defect accumulation rates approaching that of Si. This information is key to understanding the operation of a diverse set of semiconductors in the space radiation environment.



Citations (17)


... Bridged samples were irradiated with 1.2 MeV protons (P) at room temperature with a General Ionix 1.7 MV tandem accelerator at the Plasma Science and Fusion Center of MIT.[27] 1.2 MeV protons introduce mainly small defects. High levels of disorder can be obtained with short irradiation times and avoiding problems with the generation of radioisotopes; thus, the radiation tolerance of a superconductor can be tested with a comparably low effort.IV. ...

Reference:

Universal degradation of high-temperature superconductors due to impurity scattering: predicting the performance loss in fusion magnets
A facility for cryogenic ion irradiation and in situ characterization of rare-earth barium copper oxide superconducting tapes

... For example, Landau et al. investigated the accumulation of helium bubbles during He ion irradiation in LPBF AlSi10Mg alloy and suggested that increased internal stresses could help retard radiation damage [24]. In another study, Ungarish et al. used silicon ions to simultaneously emulate aluminum neutron transmutation and the radiation damage associated with Frenkel pair formation in an as-built and heat-treated AlSi10Mg alloy [25]. They found that large silicon precipitates contained fewer sinks, allowing more defects to be introduced by irradiation. ...

The Effect of Thermal History on the Additively Manufactured AlSi10Mg Alloy Response to Ion Irradiation
  • Citing Article
  • October 2023

Journal of Nuclear Materials

... The maximum operating temperature of the outer surface of the LMFR shell tube is 550 • C under nominal conditions [25]. At temperatures above 550 • C, the iron-based oxide layer transforms into unprotective Wüstite, increasing Cr dissolution and LBE intrusion [26]. Additionally, 1000 h is a critical time point for steel corrosion in LBE at 500 • C; corrosion occurring with this timeframe is considered the early stage, characterized predominantly by dissolution corrosion [27]. ...

Characterisation of corrosion damage in T91/F91 steel exposed to static liquid lead-bismuth eutectic at 700-715°C
  • Citing Article
  • August 2023

Journal of Nuclear Materials

... Lastly, θ ijk in Eq. (6) is the angle formed between atoms i, j,and k when atom i is in the center, a j and a k is a constant associated with atom i. In this context, the use of MEAM in MD simulations has shown promise in accurately representing interatomic interactions (Sheng et al. 2011;Paul et al. 2023). ...

A Modified Embedded-Atom Method Potential for a Quaternary Fe-Cr-Si-Mo Solid Solution Alloy

Materials

... Besides salts, other materials and coolants such as water and liquid metals can be investigated. The synergistic effects of combined irradiation and corrosion damage [5] can be investigated using the DICE. To our knowledge, the DICE is the second experiment of this kind [6] and the only one in Europe. ...

Effects of Simultaneous Proton Irradiation on the Corrosion of Commercial Alloys in Molten Fluoride Salt
  • Citing Article
  • March 2023

Corrosion Science

... This alumina fills all space within a 0.83-mm radius. Lastly, the whole probe is covered in a Nickel-200 sheath, achieving the probes final diameter of 2.7 mm, to combat corrosion from the molten salts [47]. ...

One dimensional wormhole corrosion in metals

... The above factors may lead to imperceptible damage, such as delamination and debonding in composites [8], or corrosion and impact in metals [9]. Therefore, the development of a robust NDT method is imperative to detect damage during the manufacturing stage, as well as to perform routine maintenance during the operational stage [10]. ...

Detecting Thermally-Induced Spinodal Decomposition with Picosecond Ultrasonics in Cast Austenitic Stainless Steels
  • Citing Article
  • November 2022

Acta Materialia

... Epoxy coatings show widespread utilization in industrial anticorrosion applications due to their impressive adhesion, corrosion resistance, physicomechanical properties, etc., making them highly favored by the market [5,6]. However, the hydrophilic groups or surfactants remaining after the curing of waterborne epoxy coatings probably form polar channels, accelerating the corrosion rate of steel structures, and water absorption and seepage make the coating material deteriorate and cause corrosion, thereby losing the corrosion resistance [7,8]. Therefore, waterborne epoxy coatings have some shortcomings such as flash rust and poor adhesion, which limits their application for metal corrosion protection [8]. ...

Coupled effect of water absorption and ion transport in hydrated latex anti-corrosion coatings

Journal of Coatings Technology and Research

... The core theme of this study is that these nanoscale defects or stress concentrations are more vulnerable to incoming radiation compared to the defect free regions. This is because they already store large strain energy, which reduces the threshold energy for radiation damage [18,19]. ...

Revealing hidden defects through stored energy measurements of radiation damage

Science Advances

... This variation may relate to sample quality or preparation. Measurements using the flash heating method on bulk samples resulted in values between 6.5 and 7.4 × 10 −5 m 2 /s, 29,31-37 and those using TGS resulted in values from 6.6 to 7.8 × 10 −5 m 2 /s, 7,9,10,30 as detailed in Table II. The scatter in values may be partially attributed to the manufacturing process, for instance, as Hust et al. 32 showed that α increases as the residual-resistance ratio (RRR) increases (i.e., lower intrinsic defects). ...

Thermal diffusivity in ion-irradiated single-crystal iron, chromium, vanadium, and tungsten measured using transient grating spectroscopy
  • Citing Article
  • July 2022