M. Zahirul Alam’s research while affiliated with University of Ottawa and other places

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Publications (59)


Metasurfaces for wavefront control. (a) Generalized laws of refraction for beam steering through phase gradients (reproduced with permission from Yu et al., Science 334, 333 (2011). Copyright 2011 AAAS;⁵ (b) metasurface holograms with high efficiency (from Ref. 20); (c) multi-wavelength, polarization-insensitive metalenses (from Ref. 21). All images are reprinted (adapted) with permission from the respective Journal and copyright remains with the original publisher.
(a) Metasurface for complex wavefront shaping to impart orbital angular momenta to the impinging light (reproduced with permission from Ren et al., Nat. Commun. 10, 2986 (2019). Copyright 2019 Springer Nature Publishing Group;³² (b) nonlocal metasurface for eyetracking applications (from Ref. 33); (c) concept of metasurfaces to facilitate chemical processes (from Ref. 34); (d) metasurface for augmented reality applications (from Ref. 35). All images are reprinted (adapted) with permission from the respective Journal and copyright remains with the original publisher.
(a) Edge detection metasurfaces for image processing and biomedical applications (from Ref. 42); (b) analog optical computing based on nonlocal metasurfaces (from Refs. 44 and 46); (c) nonlocal metasurface to manipulate thermal emission (from Ref. 47); (d) metasurfaces integrating 2D materials (from Ref. 49); (e) spatiotemporally modulated metasurface to extend the degree of control over wavefront manipulation to space-time diffraction (from Ref. 50). All images are reprinted (adapted) with permission from the respective Journal and copyright remains with the original publisher.
of the key aspects of light-emitting metasurfaces discussed in this chapter including material platforms, physical mechanisms, desired functionality, performance requirements, as well as future goals.
(a) Schematic illustration of a silicon metasurface supporting high-Q quasi-BIC resonances; (b) SEM images of the fabricated metasurface; (c) illustration of the carbon G-centers on the side walls of the etch holes; (d) emission from the carbon G-centers resonantly enhanced by the quasi-BIC [(a)–(d) from Ref. 81]; (e) illustration of chiral emission due to circularly polarized states (CPS) originating from BIC in a metasurface with broken symmetry; (f) distribution of polarization vectors in the momentum space, with a pair of CPS shown as red and blue dots (topological charges ±1/2); (g) SEM images of the fabricated metasurface; (h) enhanced circularly polarized emission from polycarbonate (PC) film doped with 2-methyl-6–(4-dimethylaminostyryl)-4H-pyran (DCM) deposited on the metasurface [(e)–(h) from Ref. 87]; (i) schematic of a single layer TMD integrated with an achiral dielectric metasurfaces for controlling valleytronic emission; (j) detected valley resolved photoluminescence of excitons and trions upon left-handed and right-handed circularly polarized laser excitation for structure shown in (i); (k) measured trion and exciton degree of polarization, for structure shown in (i) [(i)–(k) from Ref. 69)]; (l) schematic of a polymer layer containing Eu³⁺ compound integrated with a broken symmetry TiO2 metasurface for tailoring directionality and fluorescence enhancement of MD transitions; (m) measured fluorescence spectra for the metasurface scheme shown in (l) (red curve) normalized to the spectra of the substrate (blue curve); (n) measured back focal plane images of (n) MD and (o) ED transitions coupled to the metasurface shown in (l) [(l)–(o) from Ref. 72]. All images are reprinted (adapted) with permission from the respective Journal and copyright remains with the original publisher.

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Roadmap on photonic metasurfaces
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June 2024

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829 Reads

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16 Citations

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Mitchell Kenney

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Here we present a roadmap on Photonic metasurfaces. This document consists of a number of perspective articles on different applications, challenge areas or technologies underlying photonic metasurfaces. Each perspective will introduce the topic, present a state of the art as well as give an insight into the future direction of the subfield.

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Feature issue introduction: temporal and spatiotemporal metamaterials

May 2023

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37 Reads

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2 Citations

Temporal modulation of material parameters provides a new degree of freedom for metamaterials, metasurfaces and wave-matter interactions as a whole. In time-varying media the electromagnetic energy may not be conserved, and the time reversal symmetry may be broken, which may lead to novel physical effects with potential applications. Currently, theoretical and experimental aspects of this field are rapidly advancing, expanding our understanding of wave propagation in such complex spatiotemporal platforms. This field promises novel possibilities and directions in research, innovation and exploration.


The design procedure of the plasmonic metasurface. (a) The phase of the reflected field from a metasurface of homogeneous gold antennas of a constant thickness (50 nm) and width (90 nm). The four selected lengths (L1 to L4) are indicated with black dots. (b) 3D schematic of the final design of the device; the dimensions in the figure are L1 = 420 nm, L2 = 330 nm, L3 = 270 nm, and L4 = 100 nm. The period along the gradient is Λ = 1375 nm, and the separation between rows is P = 600 nm. (c) Schematic demonstrating the similarity of a periodic gradient metasurface and a blazed grating. (d) FDTD simulation of the angular distribution of the +1, 0, and −1 DOs of reflection at different wavelengths.
Fabrication and characterization of the sample. (a) The SEM image of the fabricated device. (b) A simple schematic of the pump-probe set-up with a camera to image the diffracted beams at different time delays between the pump and the probe. (c) and (d) The angular distribution of DO = +1 and DO = −1 of the probe, respectively, at different time delays between the pump and the probe. The power of each row (each delay) is normalized to the brightest pixel in that row.
The spectral distribution of the (a) DO = +1 and (b) DO = −1 for different time delays between the pump and the probe. Here power is normalized to the brightest value in the whole graph.
The maximum steering angle at different incident wavelengths and powers. (a) and (b) Show the maximum steering angle of DO = +1 and DO = −1, respectively, at different pump intensities for an incident central wavelength of 1300 nm. (c) and (d) Show the maximum steering angle of DO = +1 and DO = −1, respectively, for different wavelengths of the incident beams while the intensity of the pump is kept constant at 14 GW/cm².
Time-varying gradient metasurface with applications in all-optical beam steering

March 2023

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189 Reads

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14 Citations

Integrating the large, subpicosecond nonlinear optical response of epsilon-near-zero (ENZ) materials with the broad design freedoms of plasmonic metasurfaces shows potential for creating rapidly modulated optical devices with possible applications in telecommunications, sensing, and reactive beam steering. In this work, we experimentally investigate a metasurface consisting of a plasmonic gradient array on a thin layer of indium tin oxide (ITO), characterize how incident probe pulses diffract from a system as it is being dynamically modulated by a pump pulse at wavelengths near the ENZ region. Angular shifts in the diffraction orders are observed and can be principally attributed to the adiabatic wavelength conversion of the probe as it witnesses the temporal change of index induced by the pump. Of note, the asymmetric gradient metasurface, considered to be a blazed diffraction grating, shows significantly different dynamic responses for different diffraction orders. The free-space wavelength shift to +1 and −1 diffraction orders is 6 and 12 nm, resulting in steering angle changes of 0.65 and 1.5°, respectively.



Proposed optically induced bianisotropy. A high-intensity pump illuminates an ITO sphere. Owing to ITO’s strong nonlinear response close to its ENZ wavelength (1240 nm), a spatially inhomogeneous permittivity is obtained, causing a bianisotropic response to a low-intensity probe. Then, the probe’s scattering cross section depends on its illumination direction.
(a) Pump intensity dependent real and imaginary parts of ITO’s permittivity at the ENZ wavelength (1240 nm). (b) Pump intensity dependent scattering, absorption, and extinction cross sections of the ITO sphere at the pump wavelength. The inset figure shows a visual illustration of the setup.
(a)–(c) Real and (d)–(f) imaginary part of the permittivity in different planes for a sphere, pumped with an intensity of 200 GW/ $\mathrm {cm^{2}}$ c m 2 at the probe wavelength (1180 nm). The incident pump is an $x$ x -polarized plane wave at a wavelength of 1300 nm that propagates in the $z$ z -direction.
(a) Setup for an optical pump–probe beam impinging on an ITO sphere. (b), (c) Absolute values of the T-matrix elements with an expansion order of 5 for optical pump intensities of 0.01 GW/ $\mathrm {cm^{2}}$ c m 2 and 200 GW/ $\mathrm {cm^{2}}$ c m 2 , corresponding to linear and highly nonlinear regime, respectively. (d), (e) Scattering cross section at the probe wavelength (1180 nm) in the linear and highly nonlinear regime depending on the spherical angles ( $\theta$ θ and $\phi$ ϕ ). (f), (g) Absorption cross section in the linear and highly nonlinear regimes, respectively.
Optically tunable bianisotropy in a sphere made from an epsilon-near-zero material

January 2023

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1 Citation

Bianisotropic media can be used to engineer absorbance, scattering, polarization, and dispersion of electromagnetic waves. However, the demonstration of a tunable light-induced bianisotropy at optical frequencies is still lacking. Here, we propose an experimentally feasible concept for a light-induced tunable bianisotropic response in a homogeneous sphere made of an epsilon-near-zero (ENZ) material. By exploiting the large linear absorption and the large possible intensity-dependent changes in the permittivity of ENZ materials, the direction-dependent scattering and absorption cross sections could be obtained. Our findings pave the way for further studies and applications in the optical regime requiring full dynamic control of the bianisotropic behavior.


Figure 2. Simulated (top) and measured (bottom) reflectance maps of the three bifilm samples in the k x /k 0 −ν space. The TM-polarized reflectance spectra R TM are normalized to the TE-polarized spectra R TE at each incident wavevector to exclude measurement artifacts. The range of wavevectors is limited by the critical angle for the prism−substrate interface, and the maximum rotation of the prism−sample assembly is possible without clipping the incoming field.
Figure 3. (a) Simulated reflectance map of bifilm A in k x −ν space. (b) Dispersion lines of the SPP mode (green, dot-dashed), the ENZ mode (purple, dot-dashed), the hybrid polaritons in bifilm A (blue, solid), and their Hopfield model fits (red, dashed). (c) The SPP (solid) and ENZ (dot-dashed) mode fractions for the upper (red and maroon) and lower (cyan and blue) polaritons. The upper (lower) polariton is formed by a symmetric (antisymmetric) superposition of the constituent modes. (d) g R for bifilms with various values of d ITO estimated from the simulated (green circles) and measured (purple squares) reflectance maps of bifilms A, B, and C and the simulated reflectance maps of bifilms with ϵ ITO assumed to be the same as in bifilm A (blue circles). The error bars for estimated g R from simulations for d ITO < 80 nm and from measurements for bifilm A are given by the difference in g R from fitting the upper and the lower polariton dispersion lines. The 95% confidence intervals for g R estimated from fitting only the upper polariton dispersion line form the error bars for estimated g R from simulations for d ITO ≥ 80 nm and from measurements for bifilms B and C. The red line is the parabolic fit to g R outside the gray region in which the Hopfield model yields large fitting errors.
Strongly Coupled Plasmon Polaritons in Gold and Epsilon-Near-Zero Bifilms

January 2023

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185 Reads

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11 Citations

ACS Photonics

Epsilon-near-zero (ENZ) polaritons in a thin transparent conducting-oxide film exhibit a significant electric field enhancement and localization within the film at frequencies close to their plasma frequency, but do not propagate. Meanwhile, plasmon polariton modes in thin metallic films can propagate for several microns, but are more loosely confined in the metal. Here, we propose a strongly coupled bilayered structure of a thin gold film on a thin indium tin oxide (ITO) film that supports hybrid polariton modes. We experimentally characterize the dispersion of these modes and show that they have propagation lengths of 4-8 μm while retaining mode confinement greater than that of the polariton in gold films by nearly an order of magnitude. We study the tunability of this coupling strength by varying the thickness of the ITO film and show that ultrastrong coupling is possible at certain thicknesses. The unusual linear and nonlinear optical properties of ITO at ENZ frequencies make these bifilms useful for the active tuning of strong coupling, ultrafast switching, and enhanced nonlinear interactions at near-infrared frequencies.


Citations (30)


... Here, the silicon metasurface is designed with an array of nanoresonator meta-atoms which are formed by symmetric elliptic cylinders. Electrical and magnetic multipolar resonances can be customized by the nanostructure parameters, and achieve significant enhancement of optical nonlinearity [18,21,22]. By coupling the narrow magnetic quadrupole and the broad electric dipole, a typical asymmetric resonance profile can be formed in the transmittance spectrum, which produces the enhancement of THG [18]. ...

Reference:

Second harmonic generation and third harmonic enhancement in silicon by a composite metasurface and intense terahertz
Roadmap on photonic metasurfaces

... 18 In addition to plasmonic nanostructures, dielectric nanostructures, with low optical loss and high radiation efficiency, appear promising as alternative candidates to provide multiple optical resonances even with simple geometries. [21][22][23][24][25][26][27][28][29] Recently, Karami et. al investigated that the Mie resonances of the dielectric nanoantenna coupled with the ENZ mode of a thin ITO substrate, and measured a roughly 100-fold enhancement of the probe transmittance modulation. ...

Interactions of Fundamental Mie Modes with Thin Epsilon-near-Zero Substrates
  • Citing Article
  • December 2023

Nano Letters

... Diverse phenomena associated with light propaga on in materials with temporary modulated op cal proper es have moved into the focus of a en on of the photonic community in recent years [1][2][3][4][5]. One can argue that exploring the fourth, temporal dimension is a natural extension of the developments in the research on three and two dimensional spa ally modulated metamaterials and photonic crystals. ...

Feature issue introduction: temporal and spatiotemporal metamaterials

... Time-varying metamaterials have both enabled novel wave phenomena and provided new perspectives on classic physical problems 1,2 . Time-varying photonics, where the linear susceptibility χ 1 ð Þ of the medium is modulated at optical frequencies, enables ultrafast switching of transmittivity or reflectivity (on the fs time scale) [3][4][5] , frequency shifting and spectral modulation [6][7][8] , beam-steering [9][10][11] and nonreciprocal devices 12 . Furthermore, concepts such as time-crystals 13 , coherent wave control 14 , and lasing 15 have been predicted and hold promise for experimental implementations. ...

Time-varying gradient metasurface with applications in all-optical beam steering

... These unique properties make ENZ materials, such as indium tin oxide (ITO), useful for a variety of applications (2). For example, ITO's nonlinear properties can be used to tune its refractive index in useful ways (3). Furthermore, ENZ modes and surface plasmon polariton modes supported by these ENZ materials demonstrate substantial field enhancement within the material (4, 5). ...

Strongly Coupled Plasmon Polaritons in Gold and Epsilon-Near-Zero Bifilms

ACS Photonics

... [16][17][18][19][20] Extraordinarily fine measuring techniques, such as the quantum weak measurement, 6 are generally used, which require considerable efforts to enhance the PSHE by either increasing the interaction length of the spin-orbit or using specially designed metasurfaces, including techniques using inhomogeneous anisotropic media, 21 intensely focused light, 22 nanometer-size metasurfaces 7,8 with either spatially varying birefringence or metallic plasmonics, [12][13][14][15]23 or cylindrical glass. 24 Recently, techniques based on exceptional points, 25 non-Hermitian Skin effect, 26 and epsilon-near-zero material 27 have been proposed and demonstrated to significantly enhance the PSHE. Drawbacks, such as the high insertion loss, the high cost required by the utilized bulk components, and the extreme difficulty and complexity in combining the metal or the metamaterial with the optical system, are not avoidable, which considerably restrains these methods from practical applications. ...

Enhanced spin–orbit coupling in an epsilon-near-zero material

... Additionally, plasmonic nanoantennas, which enhance fields for both fundamental and signal waves and provide greater spatial mode overlap, have been employed to boost conversion efficiency [20]. Furthermore, zeroindex media have been proposed as a solution for phase matching, where photons interact nonlinearly and phase matching occurs automatically, thus easing the constraints traditionally associated with phase matching [21,22]. ...

Relaxed Phase-Matching Constraints in Zero-Index Waveguides
  • Citing Article
  • May 2022

Physical Review Letters

... The main challenge in experimenting with such media is their slow modulation speed for manipulating waves with short wavelength. Identifying efficient materials, such as epsilon-near-zero (ENZ) medium, and high-index dielectrics [30][31][32][33], remains a challenge. For instance, a recent study showed that an ENZ-based timevarying mirror extend the reflected wave frequency up to 31 THz [34]. ...

Adiabatic Frequency Conversion Using a Time-Varying Epsilon-Near-Zero Metasurface
  • Citing Article
  • July 2021

Nano Letters

... Time-varying optical media [1][2][3], characterized by a timedependent refractive index, opens up opportunities to manipulate the fundamental properties of electromagnetic waves for applications such as optical frequency conversion [4][5][6], Fresnel light drag [7] all-optical non-reciprocal photonics [8,9], and tuning and control of Doppler shifts [10,11]. In contrast to the reflection and refraction of light at a spatial interface arising due to a variation in the refractive index, a time boundary describes an abrupt change in the refractive index of a uniform medium at a specific time and necessitates revising these fundamental principles of optics. ...

Tunable Doppler shift using a time-varying epsilon-near-zero thin film near 1550 nm

... In recent years, the epsilon-near-zero (ENZ) material with a vanishing real part of permittivity has emerged as a promising platform for active manipulation of optical responses of nanophotonic devices [13,14]. Near the ENZ wavelength, extreme electromagnetic field enhancement and localization are exhibited in a ENZ film with a subwavelength thickness, supporting the so-called ENZ mode [15]. ...

Dependence of the coupling properties between a plasmonic antenna array and a sub-wavelength epsilon-near-zero film on structural and material parameters
  • Citing Article
  • June 2021