J. Pepijn Veefkind's research while affiliated with Delft University of Technology and other places

Publications (68)

Article
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The purpose of this study is to investigate the ability of the Sentinel-5P TROPOspheric Monitoring Instrument (TROPOMI) to derive accurate geometrical features of lofted aerosol layers, selecting the Mediterranean Basin as the study area. Comparisons with ground-based correlative measurements constitute a key component in the validation of passive...
Article
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The aim of this paper is to highlight how TROPOspheric Monitoring Instrument (TROPOMI) trace gas data can best be used and interpreted to understand event-based impacts on air quality from regional to city scales around the globe. For this study, we present the observed changes in the atmospheric column amounts of five trace gases (NO2, SO2, CO, HC...
Article
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Nitrogen dioxide (NO2) is one of the main data products measured by the Tropospheric Monitoring Instrument (TROPOMI) on the Sentinel-5 Precursor (S5P) satellite, which combines a high signal-to-noise ratio with daily global coverage and high spatial resolution. TROPOMI provides a valuable source of information to monitor emissions from local source...
Preprint
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DISAMAR is a computer model developed to simulate retrievals of properties of atmospheric trace gases, aerosols, clouds, and the ground surface from passive remote sensing observations in wavelength range from 270 to 2400 nm. It is being used for the TROPOMI/Sentinel-5P and Sentinel-4/5 missions to derive Level-1b product specifications. DISAMAR us...
Article
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Ozone in the troposphere affects humans and ecosystems as a pollutant and as a greenhouse gas. Observing, understanding and modelling this dual role, as well as monitoring effects of international regulations on air quality and climate change, however, challenge measurement systems to operate at opposite ends of the spatio-temporal scale ladder. Ab...
Preprint
Full-text available
Nitrogen dioxide (NO2) is one of the main data products measured by the Tropospheric Monitoring Instrument (TROPOMI) on the Sentinel-5 Precursor (S5P) satellite, which combines a high signal-to-noise ratio with daily global coverage and high spatial resolution. TROPOMI provides a valuable source of information to monitor emissions from local source...
Article
Full-text available
Southeast Australia experienced intensive and geographically extensive wildfires during the 2019–2020 summer season1,2. The fires released substantial amounts of carbon dioxide into the atmosphere3. However, existing emission estimates based on fire inventories are uncertain4, and vary by up to a factor of four for this event. Here we constrain emi...
Preprint
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The aim of this paper is two-fold: to provide guidance on how to best interpret TROPOMI trace gas retrievals and to highlight how TROPOMI trace gas data can be used to understand event-based impacts on air quality from regional to city-scales around the globe. For this study, we present the observed changes in the atmospheric column amounts of five...
Article
Full-text available
This paper reports on consolidated ground-based validation results of the atmospheric NO2 data produced operationally since April 2018 by the TROPOspheric Monitoring Instrument (TROPOMI) on board of the ESA/EU Copernicus Sentinel-5 Precursor (S5P) satellite. Tropospheric, stratospheric, and total NO2 column data from S5P are compared to correlative...
Article
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The global fire emission inventories depend on ground and airborne measurements of species-specific emission factors (EFs), which translate dry matter losses due to fires to actual trace gas and aerosol emissions. The EFs of nitrogen oxides (NOx) and carbon monoxide (CO) can function as a proxy for combustion efficiency to distinguish flaming from...
Article
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The ultraviolet (UV) Absorbing Aerosol Index (AAI) is widely used as an indicator for the presence of absorbing aerosols in the atmosphere. Here we consider the TROPOMI AAI based on the 340 nm/380 nm wavelength pair. We investigate the effects of clouds on the AAI observed at small and large scales. The large-scale effects are studied using an aggr...
Article
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Airborne and ground-based Pandora spectrometer NO2 column measurements were collected during the 2018 Long Island Sound Tropospheric Ozone Study (LISTOS) in the New York City/Long Island Sound region, which coincided with early observations from the Sentinel-5P TROPOspheric Monitoring Instrument (TROPOMI) instrument. Both airborne- and ground-based...
Preprint
Full-text available
Ozone in the troposphere affects humans and ecosystems as a pollutant and as a greenhouse gas. Observing, understanding and modelling this dual role, as well as monitoring effects of international regulations on air quality and climate change, however, challenge measurement systems to operate at opposite ends of the spatio-temporal scale ladder. On...
Article
Full-text available
The TROPOspheric Monitoring Instrument (TROPOMI) level-2 aerosol layer height (ALH) product has now been released to the general public. This product is retrieved using TROPOMI's measurements of the oxygen A-band, radiative transfer model (RTM) calculations augmented by neural networks and an iterative optimal estimation technique. The TROPOMI ALH...
Preprint
Full-text available
Abstract. This paper reports on consolidated ground-based validation results of the atmospheric NO<sub>2</sub> data produced operationally since April 2018 by the TROPOMI instrument on board of the ESA/EU Copernicus Sentinel-5 Precursor (S5p) satellite. Tropospheric, stratospheric, and total NO<sub>2</sub> column data from S5p are compared to corre...
Preprint
Full-text available
Abstract. Abundant NO<sub>2</sub> column measurements from airborne and ground-based Pandora spectrometers were collected as part of the 2018 Long Island Sound Tropospheric Ozone Study (LISTOS) in the New York City/Long Island Sound region and coincided with early measurements from the Sentinel-5P TROPOMI instrument. Both airborne- and ground-based...
Preprint
Full-text available
Abstract. The ultraviolet (UV) Absorbing Aerosol Index (AAI) is widely used as an indicator for the presence of absorbing aerosols in the atmosphere. Here we consider the TROPOMI AAI based on the 340/380 nm wavelength pair. We investigate the effects of clouds on the AAI observed at small and large scales. The large scale effects are studied using...
Preprint
Full-text available
Abstract. The global fire emission inventories depend on ground and airborne measurements of species-specific emission factors (EFs), which translate dry matter losses due to fires to actual trace gas and aerosol emissions. The EFs of nitrogen oxides (NO<sub>x</sub>) and carbon monoxide (CO) can function as a proxy for combustion efficiency to dist...
Article
Full-text available
The Tropospheric Monitoring Instrument (TROPOMI), aboard the Sentinel-5 Precursor (S5P) satellite, launched on 13 October 2017, provides measurements of atmospheric trace gases and of cloud and aerosol properties at an unprecedented spatial resolution of approximately 7×3.5 km2 (approx. 5.5×3.5 km2 as of 6 August 2019), achieving near-global covera...
Preprint
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Abstract. Aerosol vertical distributions are important for aerosol radiative forcing assessments and atmospheric remote sensing research. From our perspective, the aerosol layer height (ALH) is one of the major concerns in quantifying aerosol absorption from the ultra-violet aerosol index (UVAI). The UVAI has a global daily record since 1978, where...
Article
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Production of oil and natural gas in North America is at an all-time high due to the development and use of horizontal drilling and hydraulic fracturing. Methane emissions associated with this industrial activity are a concern because of the contribution to climate radiative forcing. We present new measurements from the space-based TROPOspheric Mon...
Preprint
Full-text available
Abstract. The Tropospheric Monitoring Instrument (TROPOMI), aboard the Sentinel-5 Precursor (S5P) satellite, launched on 13 Oct. 2017, provides measurements of atmospheric trace gases and of cloud and aerosol properties on an unprecedented spatial resolution of approximately 7 × 3.5 km<sup>2</sup> (approx. 5.5 × 3.5 km<sup>2</sup> as of 6 Aug. 2019...
Article
Full-text available
To retrieve aerosol properties from satellite measurements of the oxygen A-band in the near-infrared, a line-by-line radiative transfer model implementation requires a large number of calculations. These calculations severely restrict a retrieval algorithm's operational capability as it can take several minutes to retrieve the aerosol layer height...
Preprint
Full-text available
The Tropospheric Monitoring Instrument's (TROPOMI) level-2 aerosol layer height (ALH) product has now been released to the general public. This product is retrieved using TROPOMI's measurements of the oxygen A-band, radiative transfer model (RTM) calculations augmented by neural networks and an iterative optimal estimation technique. The TROPOMI AL...
Article
Full-text available
To retrieve aerosol properties from satellite measurements of the oxygen A-band in the near infrared, a line-by-line radiative transfer model implementation requires a large number of calculations. These calculations severely restrict a retrieval algorithm's operational capability as it can take several minutes to retrieve aerosol layer height for...
Article
New state‐of‐the‐art satellite measurements of tropospheric column NO2 from the TROPOMI instrument on‐board Sentinel‐5 Precursor (S5P), launched in October 2017, allow for an unprecedented high resolution (sub‐10km) assessment of UK air quality (AQ) from space. We present the first results from TROPOMI and compare them with its predecessor, the Ozo...
Article
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Global mapping of satellite tropospheric NO2 vertical column density (VCD), a key gas in air quality monitoring, requires accurate retrievals over complex urban and industrialized areas and under any atmospheric conditions. The high abundance of aerosol particles in regions dominated by anthropogenic fossil fuel combustion, e.g. megacities, and/or...
Article
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The absorbing aerosol index (AAI) is a qualitative parameter directly calculated from satellite-measured reflectance. Its sensitivity to absorbing aerosols in combination with a long-term data record since 1978 makes it an important parameter for climate research. In this study, we attempt to quantify aerosol absorption by retrieving the single-sca...
Article
Full-text available
Global mapping of satellite tropospheric NO2 vertical column density (VCD), a key gas in air quality monitoring, requires accurate retrievals over complex urban and industrialized areas. The high abundance of aerosol particles in regions dominated by anthropogenic fossil fuel combustion, mega-cities and biomass burning affects the space-borne spect...
Article
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This paper presents a weighted least squares approach to retrieve aerosol layer height from top-of-atmosphere reflectance measurements in the oxygen A band (758–770 nm) over bright surfaces. A property of the measurement error covariance matrix is discussed, due to which photons travelling from the surface are given a higher preference over photons...
Article
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This overview paper highlights the successes of the Ozone Monitoring Instrument (OMI) on board the Aura satellite spanning a period of nearly 14 years. Data from OMI has been used in a wide range of applications and research resulting in many new findings. Due to its unprecedented spatial resolution, in combination with daily global coverage, OMI p...
Article
This overview paper highlights the successes of the Ozone Monitoring Instrument (OMI) on board the Aura satellite spanning a period of nearly 14 years. Data from OMI has been used in a wide range of applications and research resulting in many new findings. Due to its unprecedented spatial resolution, in combination with daily global coverage, OMI p...
Article
Full-text available
A global picture of atmospheric aerosol vertical distribution with a high temporal resolution is of key importance not only for climate, cloud formation, and air quality research studies but also for correcting scattered radiation induced by aerosols in absorbing trace gas retrievals from passive satellite sensors. Aerosol layer height (ALH) was re...
Article
Full-text available
This paper presents a weighted least squares approach to retrieve aerosol layer height from top-of-atmosphere reflectance measurements in the oxygen A band (758 nm - 770 nm) over bright surfaces. A property of the measurement error covariance matrix is discussed, due to which photons traveling from the surface are given a higher preference over pho...
Article
Full-text available
The absorbing aerosol index (AAI) based on the near Ultra-Violet (near-UV) remote sensing techniques is a qualitative parameter that allows to retrieve aerosol optical properties with confidence. In the first part of this study, a series of AAI sensitivity analysis is presented exclusively on biomass burning aerosols. Later on, this study applies a...
Article
Full-text available
Retrieving aerosol optical thickness and aerosol layer height over a bright surface from measured top-of-atmosphere reflectance spectrum in the oxygen A band is known to be challenging, often resulting in large errors. In certain atmospheric conditions and viewing geometries, a loss of sensitivity to aerosol optical thickness has been reported in t...
Article
Full-text available
A global picture of atmospheric aerosol vertical distribution with a high temporal resolution is of key importance not only for climate, cloud formation and air quality research studies, but also for correcting aerosol radiation effect in absorbing trace gas retrievals from passive satellite sensors. Aerosol layer height (ALH) was retrieved from th...
Article
Full-text available
Retrieving aerosol optical thickness and aerosol layer height over a bright surface from measured top of atmosphere reflectance spectrum in the oxygen A-band is known to be challenging, often resulting in large errors. In certain atmospheric conditions and viewing geometries, a loss of sensitivity to aerosol optical thickness has been reported in l...
Article
Full-text available
This paper presents the retrieval method that was developed to derive tropospheric NO2 columns from UV/VIS spectral measurements obtained with the Spectrolite Breadboard Instrument during the AROMAPEX campaign in Berlin (April 2016). A typical DOAS retrieval approach is followed. For the calculation of air mass factors this study specifically focus...
Article
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The Dutch–Finnish Ozone Monitoring Instrument (OMI) is an imaging spectrograph flying on NASA's EOS Aura satellite since 15 July 2004. OMI is primarily used to map trace-gas concentrations in the Earth's atmosphere, obtaining mid-resolution (0.4–0.6 nm) ultraviolet–visible (UV–VIS; 264–504 nm) spectra at multiple (30–60) simultaneous fields of view...
Article
Full-text available
The Dutch-Finnish Ozone Monitoring Instrument (OMI) is an imaging spectrograph flying on NASA's EOS Aura satellite since July 15, 2004. OMI is primarily used to map trace gas concentrations in the Earth’s atmosphere, obtaining mid-resolution (0.4–0.6 nm) UV-VIS (264–504 nm) spectra at multiple (30–60) simultaneous fields of view. Assessed via vario...
Article
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The OMI (Ozone Monitoring Instrument on board NASA's Earth Observing System (EOS) Aura satellite) OMCLDO2 cloud product supports trace gas retrievals of for example ozone and nitrogen dioxide. The OMCLDO2 algorithm derives the effective cloud fraction and effective cloud pressure using a DOAS (differential optical absorption spectroscopy) fit of th...
Article
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The Ozone Monitoring Instrument (OMI) onboard NASA's Aura satellite has been providing global observations of the ozone layer and key atmospheric pollutant gases, such as nitrogen dioxide (NO2) and sulfur dioxide (SO2), since October 2004. The data products from the same instrument provide consistent spatial and temporal coverage and permit the stu...
Article
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The OMI (Ozone Monitoring Instrument) OMCLDO2 cloud product supports trace gas retrievals of for example ozone and nitrogen dioxide. The OMCLDO2 algorithm derives the effective cloud fraction and effective cloud pressure using a DOAS fit of the O2-O2 absorption feature around 477 nm. A new version of the OMI OMCLDO2 cloud product is presented that...
Article
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Satellite instruments are nowadays successfully utilised for measuring atmospheric aerosol in many applications as well as in research. Therefore, there is a growing need for rigorous error characterisation of the measurements. Here, we introduce a methodology for quantifying the uncertainty in the retrieval of aerosol optical thickness (AOT). In p...
Article
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We study uncertainty quantification in remote sensing of aerosols in the atmosphere with top of the atmosphere reflectance measurements from the nadir-viewing Ozone Monitoring Instrument (OMI). Focus is on the uncertainty in aerosol model selection of pre-calculated aerosol models and on the statistical modelling of the model inadequacies. The aim...
Article
a b s t r a c t The impact of Hurricanes Katrina and Rita in 2005 on pollution emissions in the Gulf of Mexico region was investigated using tropospheric column amounts of nitrogen dioxide (NO 2) from the Ozone Moni-toring Instrument (OMI) on the NASA Aura satellite. Around New Orleans and coastal Mississippi, we estimate that Katrina caused a 35%...
Article
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We present a validation of tropospheric NO2 columns from the Ozone Monitoring Instrument (OMI) using measurements from the Dutch Aerosol and Nitrogen Dioxide Experiments for vaLIdation of OMI and SCIAMACHY (DANDELIONS) and Intercontinental Transport Experiment (INTEX-B) campaigns held in 2006. These unique campaigns covered a wide range of pollutio...
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1] Aggressive measures were instituted by the Beijing municipal authorities to restrict vehicular traffic in the Chinese capital during the recent Sino-African Summit. We show that reductions in associated emissions of NO x were detected by the Dutch-Finnish Ozone Monitoring Instrument (OMI) aboard the Aura satellite. Interpretation of these data u...
Article
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The Ozone Monitoring Instrument (OMI) flies on NASA's Earth Observing System AURA satellite, launched in July 2004. OMI is an ultraviolet/visible (UV/VIS) nadir solar backscatter spectrometer, which provides nearly global coverage in one day, with a spatial resolution of 13 km×24 km. Trace gases measured include O<sub>3</sub>, NO<sub>2</sub>, SO<su...
Article
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We describe the operational algorithm for the retrieval of stratospheric, tropospheric, and total column densities of nitrogen dioxide (NO<sub>2</sub>) from earthshine radiances measured by the Ozone Monitoring Instrument (OMI), aboard the EOS-Aura satellite. The algorithm uses the DOAS method for the retrieval of slant column NO<sub>2</sub> densit...
Article
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This paper describes the algorithm for deriving the total column ozone from spectral radiances and irradiances measured by the Ozone Monitoring Instrument (OMI) on the Earth Observing System Aura satellite. The algorithm is based on the differential optical absorption spectroscopy technique. The main characteristics of the algorithm as well as an e...
Article
The Ozone Monitoring Instrument (OMI) was launched successfully in July 2004, as one of four instruments on the EOS Aura satellite. OMI makes hyperspectral measurements that are used to retrieve column densities of critical trace gases, including formaldehyde, BrO, SO2 and NO2 . We present the first results from the OM1 operational NO2 algorithm an...
Article
Two aerosol optical depth retrieval algorithms, using different instruments and different methods, are compared. The first method uses both the directional and the spectral information of the Along Track Scanning Radiometer 2 (ATSR-2) to compute the aerosol optical depth in the visible and near-infrared ranges. The second algorithm uses data in the...
Article
Full-text available
We examine aerosol extinction and optical thickness from the Lidar Atmospheric Sensing Experiment (LASE), the in situ nephelometer and absorption photometer on the University of Washington C-131A aircraft, and the NASA Ames Airborne Tracking Sun Photometer (AATS-6) on the C-131A measured during the Tropospheric Aerosol Radiative Forcing Observation...