Henk Eskes's research while affiliated with Koninklijk Nederlands Meteorologisch Instituut and other places

Publications (131)

Article
Full-text available
Airborne imaging differential optical absorption spectroscopy (DOAS), ground-based stationary DOAS, and car DOAS measurements were conducted during the S5P-VAL-DE-Ruhr campaign in September 2020. The campaign area is located in the Rhine-Ruhr region of North Rhine-Westphalia, western Germany, which is a pollution hotspot in Europe comprising urban...
Article
The Arctic region is experiencing notable warming as well as more lightning. Lightning is the dominant source of upper tropospheric nitrogen oxides (NOx), which are precursors for ozone and hydroxyl radicals. In this study, we combine the nitrogen dioxide (NO2) observations from the TROPOspheric Monitoring Instrument (TROPOMI) with Vaisala Global L...
Article
Full-text available
The Sentinel-5P TROPOspheric Monitoring Instrument (TROPOMI) instrument, launched in October 2017, provides unique observations of atmospheric trace gases at a high resolution of about 5 km, with near-daily global coverage, resolving individual sources like thermal powerplants, industrial complexes, fires, medium-scale towns, roads, and shipping ro...
Article
Full-text available
Quantification and control of NO x and CO 2 emissions are essential across the world to limit adverse climate change and improve air quality. We present a new top-down method, an improved superposition column model to estimate day-today NO x and CO 2 emissions from the large city of Wuhan, China, located in a polluted background. The latest release...
Preprint
Full-text available
Top-down CO2 emission estimates based on satellite observations are potentially of great importance for independently verifying the accuracy of reported emissions and emission inventories. Difficulties in verifying these satellite-derived emissions arise from the fact that emission inventories often provide annual mean emissions while estimates fro...
Preprint
Full-text available
Nitrogen dioxide (NOx) is an important primary air pollutant, dominantly produced by anthropogenic, mostly combustion based, activities from sectors such as industry, traffic and transport. NOx is directly linked to negative health and environmental impacts. Currently, the construction of emission inventories to keep track of NOx emissions is based...
Article
Full-text available
Clouds have a strong impact on satellite measurements of tropospheric trace gases in the ultraviolet, visible, and near-infrared spectral ranges from space. Therefore, trace gas retrievals rely on information on cloud fraction, cloud albedo, and cloud height from cloud products. In this study, the cloud parameters from different cloud retrieval alg...
Preprint
Full-text available
Airborne imaging differential optical absorption spectroscopy (DOAS), ground-based stationary and car DOAS measurements were conducted during the S5P-VAL-DE-Ruhr campaign in September 2020. The campaign area is located in the Rhine-Ruhr region of North Rhine-Westphalia, Western Germany, which is a pollution hotspot in Europe comprising urban and la...
Article
Full-text available
Citation: Pseftogkas, A.; Koukouli, M.-E.; Segers, A.; Manders, A.; Geffen, J.v.; Balis, D.; Meleti, C.; Stavrakou, T.; Eskes, H. Comparison of S5P/TROPOMI Inferred NO 2 Surface Concentrations with In Situ Measurements over Central Europe.
Preprint
Full-text available
Quantification and control of NOx and CO2 emissions are important across the world to limit adverse climate change. We present a new top-down method, an improved superposition column model to estimate day-to-day NOx and CO2 emissions from the large city of Wuhan, China, located in a polluted background. The lasted released version 2.3.1 TROPOMI NO2...
Preprint
Full-text available
The aim of this paper is to evaluate the surface concentration of nitrogen dioxide (NO2) inferred from the Sentinel-5 Precursor TROPOspheric Monitoring Instrument (S5P/TROPOMI) NO2 tropospheric column densities over Central Europe for two time periods, the summer of 2019 and the winter of 2019-2020. Simulations of the NO2 tropospheric vertical colu...
Preprint
Full-text available
The Copernicus Atmosphere Monitoring Service has recently produced a greenhouse gases reanalysis (version egg4) that covers almost two decades from 2003 to 2020 and will be extended in the future. This reanalysis dataset includes carbon dioxide (CO2) and methane (CH4). The reanalysis procedure combines model data with satellite data into a globally...
Preprint
Full-text available
Clouds have a strong impact on satellite measurements of tropospheric trace gases in the ultraviolet, visible, and near-infrared spectral ranges from space. Therefore, trace gas retrievals rely on information on cloud fraction, cloud albedo, and cloud height from cloud products. In this study, the cloud parameters from different cloud retrieval alg...
Preprint
Full-text available
The Sentinel-5P TROPOMI instrument, launched in October 2017, provides unique observations of atmospheric trace gases at a high resolution of about 5 km with near-daily global coverage, resolving individual sources like thermal power plants, industrial complexes, fires, medium-scale towns, roads and shipping routes. Even though Sentinel-5P (S5P) is...
Article
Full-text available
Lightning, one of the major sources of nitrogen oxides (NOx) in the atmosphere, contributes to the tropospheric concentration of ozone and to the oxidizing capacity of the atmosphere. Lightning produces between 2 and 8 Tg N yr−1 globally and on average about 250 ± 150 mol NOx per flash. In this work, we estimate the moles of NOx produced per flash...
Article
Full-text available
This study delves into the photochemical atmospheric changes reported globally during the pandemic by analyzing the change in emissions from mobile sources and the contribution of local meteorology to ozone (O3) and particle formation in Bogotá (Colombia), Santiago (Chile), and Sao Paulo (Brazil). The impact of mobility reductions (50%–80%) produce...
Article
Full-text available
Thunderstorms can significantly influence the air composition via strong updraft and lightning nitrogen oxides (LNOx). In this study, the ozonesondes and TROPOMI (TROPOspheric Monitoring Instrument) nitrogen dioxide (NO2) observations for two cases are combined with a model to investigate the effects of typical strong convection on vertical redistr...
Article
Full-text available
Nitrogen dioxide (NO2) is one of the main data products measured by the Tropospheric Monitoring Instrument (TROPOMI) on the Sentinel-5 Precursor (S5P) satellite, which combines a high signal-to-noise ratio with daily global coverage and high spatial resolution. TROPOMI provides a valuable source of information to monitor emissions from local source...
Article
Full-text available
The fast industrialization and urbanization in India lead to serious air quality problems. Using the long record of the satellite observations of NO2 from the Ozone Monitoring Instrument, we have derived monthly NOx emissions over India from 2007 to 2018 by applying an inversion algorithm to the QA4ECV NO2 retrieval product. Our results show that N...
Article
Full-text available
The COVID-19 lockdown had a large impact on anthropogenic emissions of air pollutants and particularly on nitrogen dioxide (NO2). While the overall NO2 decline over some large cities is well-established, understanding the details remains a challenge since multiple source categories contribute. In this study, a new method of isolation of three compo...
Article
Full-text available
We present tropospheric nitrogen dioxide (NO2) changes observed by the Canadian Pandora measurement program in the Greater Toronto Area (GTA), Canada, and compare the results with surface NO2 concentrations measured via in situ instruments to assess the local emission changes during the first two years of the COVID-19 pandemic. In the City of Toron...
Article
Full-text available
This study gives a systematic comparison of the Tropospheric Monitoring Instrument (TROPOMI) version 1.2 and Ozone Monitoring Instrument (OMI) QA4ECV tropospheric NO2 column through global chemical data assimilation (DA) integration for the period April–May 2018. DA performance is controlled by measurement sensitivities, retrieval errors, and cover...
Article
Full-text available
TROPOMI (TROPOspheric Monitoring Instrument) measurements of tropospheric NO2 columns provide powerful information on emissions of air pollution by ships on open sea. This information is potentially useful for authorities to help determine the (non-)compliance of ships with increasingly stringent NOx emission regulations. We find that the informati...
Article
Full-text available
Global trends in tropospheric nitrogen dioxide (NO2) have changed dramatically in the past decade. Here, we investigate tropospheric NO2 variabilities over United States, Europe, and E. China in 2005–2018 to explore the mechanisms governing the variation of this critical pollutant. We found large uncertainties in the trends of anthropogenic nitroge...
Article
Full-text available
. Lightning, one of the major sources of nitro�gen oxides (NOx ) in the atmosphere, contributes to the tropospheric concentration of ozone and to the oxidiz�ing capacity of the atmosphere. Lightning produces be�tween 2 and 8 Tg N yr−1 globally and on average about 250 ± 150 mol NOx per flash. In this work, we estimate the moles of NOx produced per...
Preprint
Full-text available
This study gives a systematic comparison of the Tropospheric Monitoring Instrument (TROPOMI) version 1.2 and Ozone Monitoring Instrument (OMI) QA4ECV tropospheric NO2 column through global chemical data assimilation (DA) integration for the period April−May 2018. DA performance is controlled by measurement sensitivities, retrieval errors, and cover...
Preprint
Full-text available
Nitrogen dioxide (NO2) is one of the main data products measured by the Tropospheric Monitoring Instrument (TROPOMI) on the Sentinel-5 Precursor (S5P) satellite, which combines a high signal-to-noise ratio with daily global coverage and high spatial resolution. TROPOMI provides a valuable source of information to monitor emissions from local source...
Preprint
Full-text available
Thunderstorms can significantly influence the air composition via strong updraft and lightning nitrogen oxides (LNOx). In this study, the ozonesondes and TROPOMI nitrogen dioxide (NO2) observations for two cases are combined with model to investigate the effects of typical strong convection on vertical redistribution of air pollutants in Nanjing, s...
Article
Full-text available
The aim of this paper is to apply a new lane separation methodology for the maritime sector emissions attributed to the different vessel types and marine traffic loads in the Mediterranean and the Black Sea defined via the European Marine and Observation Data network (EMODnet), developed in 2016. This methodology is implemented for the first time o...
Preprint
Full-text available
Lightning is one of the major sources of nitrogen oxides (NOx) in the atmosphere, contributing to the tropospheric concentration of ozone and to the oxidising capacity of the atmosphere. Lightning produces between 2–8 Tg N per year globally and on average about 250 ± 150 mol NOx per flash. In this work, we estimate the moles of NOx produced per fla...
Preprint
Full-text available
TROPOMI measurements of tropospheric NO2 columns provide powerful information on emissions of air pollution by ships on open sea. This information is potentially useful for authorities to help determine the (non-)compliance of ships with increasingly stringent NOx emission regulations. We find that the information quality is improved further by rec...
Preprint
Full-text available
The aim of this paper is to apply a new lane separation methodology for the maritime sector emissions attributed to the different vessel types and marine traffic loads in the Mediterranean and the Black Sea defined via the European Marine and Observation Data network (EMODnet), developed in 2016. This methodology is implemented for the first time o...
Article
Full-text available
We present a new divergence method to estimated methane (CH4) emissions from satellite observed mean mixing ratio of methane (XCH4) by deriving the regional enhancement of XCH4 in the Planetary Boundary Layer (PBL). The applicability is proven by comparing the estimated emissions with its known emission inventory from a 3‐month GEOS‐Chem simulation...
Article
Full-text available
Plain Language Summary Burning of fossil fuels at high temperatures constitutes a major anthropogenic source of nitrogen oxides (NOx) and carbon dioxide (CO2). While CO2 stays in the atmosphere for hundreds of years, thereby being a well‐mixed gas, NO2 has a much shorter lifetime of only a few hours. This substantial difference in lifetime between...
Preprint
Full-text available
The aim of this paper is two-fold: to provide guidance on how to best interpret TROPOMI trace gas retrievals and to highlight how TROPOMI trace gas data can be used to understand event-based impacts on air quality from regional to city-scales around the globe. For this study, we present the observed changes in the atmospheric column amounts of five...
Article
Full-text available
In this work, we investigate the ability of a data assimilation technique and space-borne observations to quantify and monitor changes in nitrogen oxides (NOx) emissions over Northwestern Greece for the summers of 2018 and 2019. In this region, four lignite-burning power plants are located. The data assimilation technique, based on the Ensemble Kal...
Preprint
Full-text available
The COVID-19 lockdown had a large impact on anthropogenic emissions of air pollutants and particularly on nitrogen dioxide (NO2). While the overall NO2 decline over some large cities is well-established, its quantification remains a challenge because of a variety of sources of NO2. In this study, a new method of isolation of three components: backg...
Article
Full-text available
We present version 1.0 of a global catalog of NOx emissions from point sources, derived from TROPOspheric Monitoring Instrument (TROPOMI) measurements of tropospheric NO2 for 2018–2019. The identification of sources and quantification of emissions are based on the divergence (spatial derivative) of the mean horizontal flux, which is highly sensitiv...
Preprint
Full-text available
In this work, we investigate the ability of a data assimilation technique and space-borne observations to quantify and monitor changes in nitrogen oxides (NOx) emissions over North-Western Greece for the summers of 2018 and 2019. In this region, four lignite-burning power plants are located. The data assimilation technique, based on the Ensemble Ka...
Article
Full-text available
We present the results from a global 0.56°‐resolution chemical data assimilation that integrates satellite observations of ozone, NO2, CO, HNO3, and SO2 from OMI, GOME‐2, SCIAMACHY, TES, MOPITT, and MLS. The assimilation is based on an ensemble Kalman filter technique and simultaneously optimizes ozone precursor emissions and concentrations of vari...
Article
Full-text available
Efforts to stem the transmission of coronavirus disease 2019 (COVID-19) led to rapid, global ancillary reductions in air pollutant emissions. Here, we quantify the impact on tropospheric ozone using a multiconstituent chemical data assimilation system. Anthropogenic NO x emissions dropped by at least 15% globally and 18 to 25% regionally in April...
Article
Full-text available
Nitrogen oxides produced by lightning (LNOx) play an important role in determining mid- and upper-tropospheric concentrations of the hydroxyl radical (OH), methane (CH4), and ozone (O3). The moles of NOx produced per flash was examined using nitrogen dioxide (NO2) columns and cloud properties from the Tropospheric Monitoring Instrument (TROPOMI) an...
Article
Full-text available
The Copernicus Atmosphere Monitoring Service (CAMS) is operationally providing forecast and reanalysis products of air quality and atmospheric composition. In this article, we present an extended evaluation of the CAMS global reanalysis data set of four reactive gases, namely, ozone (O3), carbon monoxide (CO), nitrogen dioxide (NO2), and formaldehy...
Article
Full-text available
Nitrogen oxides (NOx ≡ NO + NO2) in the NOx-limited upper troposphere (UT) are long-lived and so have a large influence on the oxidizing capacity of the troposphere and formation of the greenhouse gas ozone. Models misrepresent NOx in the UT and observations to address deficiencies in models are sparse. Here we obtain a year of near-global seasonal...
Article
Full-text available
The evaluation of chemical transport models, CTMs, is essential for the assessment of their performance regarding the physical and chemical parameterizations used. While regional CTMs have been widely used and evaluated over Europe, their validation over Greece is limited. In this study, we investigate the performance of the Long Term Ozone Simulat...
Article
Full-text available
The coronavirus-19 (COVID-19) pandemic led to government interventions to limit the spread of the disease which are unprecedented in recent history; for example, stay at home orders led to sudden decreases in atmospheric emissions from the transportation sector. In this review article, the current understanding of the influence of emission reductio...
Article
Full-text available
Nitrogen oxides (NOx≡NO+NO2) in the NOx-limited upper troposphere (UT) are long-lived and so have a large influence on the oxidizing capacity of the troposphere and formation of the greenhouse gas ozone. Models misrepresent NOx in the UT, and observations to address deficiencies in models are sparse. Here we obtain a year of near-global seasonal me...
Preprint
Full-text available
We present version 1.0 of a global catalog of NO x emissions from point sources, derived from TROPOMI measurements of tropospheric NO 2 for 2018-2019. The identification of sources and quantification of emissions are based on the divergence (spatial derivative) of the mean horizontal flux, which is highly sensitive for point sources like power plan...
Article
Full-text available
The unprecedented order, in modern peaceful times, for a near-total lockdown of the Greek population as a means of protection against severe acute respiratory syndrome coronavirus 2, commonly known as COVID-19, has generated unintentional positive side-effects with respect to the country's air quality levels. Sentinel-5 Precursor/Tropospheric Monit...
Article
Full-text available
Satellite measurements of tropospheric NO2 columns are valuable for monitoring long-term changes in air quality. However, direct linkage of satellite-derived NO2 trends with changes in underlying NOx emissions and NOx surface concentrations is complicated by the contribution of background NO2 to the column, by changes in the chemical regime wherein...
Article
Full-text available
Sentinel-5 Precursor (S-5P), launched in October 2017, carrying the TROPOspheric Monitoring Instrument (TROPOMI) nadir-viewing spectrometer, is the first mission of the Copernicus Programme dedicated to the monitoring of air quality, climate, and ozone. In the presented study, the TROPOMI tropospheric nitrogen dioxide (NO2) level-2 (L2) product (OF...
Article
Full-text available
A lockdown was implemented in Canada mid-March 2020 to limit the spread of COVID-19. In the wake of this lockdown, declines in nitrogen dioxide (NO2) were observed from the TROPOspheric Monitoring Instrument (TROPOMI). A method is presented to quantify how much of this decrease is due to the lockdown itself as opposed to variability in meteorology...
Conference Paper
Policies to regulate severe surface ozone pollution in cities in India are challenging to develop, due to the complex dependence on precursor emissions of volatile organic compounds (VOCs) and nitrogen oxides (NOx), non-linear chemistry leading to ozone formation, and very limited spatial and temporal surface air quality monitoring. Ratios of space...
Preprint
Efforts to slow the transmission of COVID-19 led to rapid, global ancillary reductions in air pollutant emissions. Here, we quantify the resulting decreases in global NOx emissions and their consequent impact on the production of global tropospheric ozone using a multi-constituent data assimilation system. Total anthropogenic NOx emissions were red...