Faquan Li’s research while affiliated with Chinese Academy of Sciences and other places

Understanding the thermodynamic horizontal structure of the mesopause is essential for studying atmospheric wave dynamics and energy transport. However, conventional models like MSISE-00 exhibit some discrepancies from lidar observations in the mesopause. To obtain a more reliable horizontal temperature structure, this study integrates coordinated lidar observations from Urumqi, Yuzhong, and Yangbajing with models using a three-dimensional variational (3DVAR) data assimilation method to construct a high-resolution temperature field over northwestern China. The assimilated temperature profiles closely match lidar observations, with the RMSE (root mean square error) of residual reductions of 67.35% at Urumqi, 60.69% at Yuzhong, and 34.80% at Yangbajing. Independent validation at Korla showed a RMSE of residual reductions of 40.14%, confirming the model's effectiveness. The thermodynamical horizontal structures of the mesopause obtained from this model were also analyzed. The lidar-based model for the mesopause extends the observation results from disparate lidar stations to the area between lidar stations and will contribute to a deeper understanding of upper atmospheric dynamics.

Atmospheric temperature information in the near space is of great academic significance and engineering value to support the development and utilization of the near space. Based on the theory of O2 molecular dayglow spectroscopy and the mechanism of atmospheric radiative transfer, a method is proposed for the joint retrieval of temperature profiles in the near space using O2(a¹Δg) and O2(b¹∑⁺g) bands dayglow spectroscopy signal with the self-absorption effect. First, the temperature dependence of O2(a¹Δg) and O2(b¹∑⁺g) bands dayglow is investigated, and the influence of the self-absorption effect on the radiative transfer characteristics is analyzed in the limb-view mode. Then, with the use of the onion peeling algorithm, the dayglow emission spectra signals of the O2(a¹Δg) and O2(b¹∑⁺g) bands measured by the SCanning Imaging Absorption spectroMeter for Atmospheric CHartographY (SCIAMACHY) in the limb-viewing mode were processed, and combined with optimization algorithms, the temperature profiles from 35 km to 120 km is successfully retrieved. Finally, the accuracy and reliability of the self-absorption effect correction as well as the joint temperature retrieval were verified by comparing with temperature product data from remote sensing satellites such as Sounding of the Atmosphere using Broadband Emission Radiometry (SABER), Atmospheric Chemistry Experiment Fourier-Transform Spectrometer (ACE-FTS), and Michelson Interferometer for Passive Atmospheric Sounding (MIPAS). The error analysis shows that the temperature retrieval error after correction for the self-absorption effect is about 3 K minimum and 20 K maximum.

The shot-to-shot measurement uncertainty restricts the application of laser-induced breakdown spectroscopy (LIBS) technically, to a certain extent. In order to further deepen the understanding of spectral stability, in this paper, the effects of the laser’s focus depth, the delay of the spectrometer, and the position of the spectrum collection on the spectral stability were carefully researched. Moreover, the dynamic characteristics of plasma were studied at different laser focusing depths. Research has found that the morphological changes of plasma are relatively stable, without significant changes, despite varying depths of laser focus on the sample surface. In addition, it was found that stable elemental emission spectra can always be obtained in the early plasma aggregation region.

The transmission spectrum of a narrow-band interference filter is crucial and highly influenced by factors such as the temperature and angle, thus requiring precise and online measurements. The traditional method of measuring the transmission spectrum of an interference filter involves the use of a spectrometer, but the accuracy of this method is limited. Moreover, placing a narrow-band interference filter inside a spectrometer hinders real-time online measurements. To address this issue, there is demand for high-precision online spectral testing methods. In response to this demand, we propose and experimentally validate a fine spectral characterization method for narrow-band interference filters. This method uses a narrow-linewidth tunable laser, achieving a spectral resolution in the MHz range for online testing. Two types of narrow-band interference filters were tested using the constructed laser spectroscopy experimental system, obtaining a transmission spectrum with a spectral resolution of 318 MHz. In comparison to spectrometer-based methods, our proposed method demonstrates higher spectral accuracy, enables online measurements, and provides more accurate measurements for special spectral interference filters. This approach has significant application value and promising development prospects.

Through long-term Rayleigh lidar observations during 2010-2022, atmospheric gravity wave (AGW) activities in the middle atmosphere (30–65 km) are statistically investigated at Haikou (110.3°E, 19.9°N) in China. In total, 827 quasi-monochromatic AGW events are identified from the lidar dataset, and the vertical wavelength, observed wave period, and vertical propagation direction of dominant waves are extracted for each AGW event by analyzing the power spectra of wave-induced temperature perturbations. It is revealed that 81.7% of all AGW events were associated with upward-propagating waves, and the proportion of upward-propagating AGWs reached a maximum in autumn and a minimum in winter. The most common vertical wavelengths and wave periods were 6–11 km and 4–10 hours, respectively. In particular, 68 AGW events associated with simultaneous upward and downward propagating waves were observed by lidar, corresponding to 8.2% of the events. The occurrence of such special AGW phenomena is qualitatively discussed, and multiple formation mechanisms may exist. Comparisons are made with previously reported lidar observation results, and the statistical features of AGW activity in the low-latitude middle atmosphere may vary over a relatively wide range depending on the location and altitude. However, a majority of AGWs propagate upward in the middle atmosphere.

This study introduces an innovative method to improve the quality and accuracy of LiDAR observation data by utilizing YOLOv9 image recognition technology. By correlating daytime cloud image grayscale values and nighttime sky star counts with LiDAR data, this method provides a robust solution for all-weather observations. Experimental results show that this technique can accurately predict LiDAR data quality under various environmental conditions, offering a valuable tool for atmospheric science research and meteorological monitoring.

Based on the resonance fluorescence scattering mechanism, a narrowband sodium (Na) lidar can measure temperature and wind in the mesosphere and lower thermosphere (MLT) region. By using a narrowband spectral filter, background light noise during the day can be suppressed, allowing for continuous observations. To obtain full-diurnal-cycle temperature and wind measurement results, a complex and precise retrieval process is required, along with necessary corrections to minimize measurement errors. This paper introduces the design of a data acquisition unit for three frequencies in three directions of the Na lidar system in the Chinese Meridian Project (Phase II) and investigates the calibration and retrieval methods for obtaining diurnal temperature and horizontal wind in the MLT region, using a Na Doppler lidar with Faraday anomalous dispersion optical filter (FADOF). Furthermore, these methods are applied to observations conducted by a Na lidar in Beijing, China. The wind and temperature results over full diurnal cycles obtained from the all-solid-state Na Doppler lidar are reported for the first time and compared with temperature measurements from satellite, as well as wind observations from a meteor radar. The comparison demonstrates a reasonable agreement between the results, indicating the rationality of the lidar-retrieved results and the feasibility and effectiveness of the data correction and retrieval method.

The thermospheric layers reported are located in the E and F regions of the ionosphere, which can be used as unique tracers for studies of interaction processes between neutral and ionized components in 105~200 km. In order to enhance our understanding of the origin and formation mechanisms of thermospheric layers, this study analyzes the observed sodium (Na) data by a high-sensitivity resonance fluorescence lidar at Yanqing Station, Beijing (40.42°N, 116.02°E). According to their morphological characteristics, occurrence frequency, and referring to the previous reports, the thermospheric Na atomic layers observed from the station are mainly classified into the following four types: lower thermosphere sporadic Na layers, dawn thermosphere-ionosphere Na layers, midnight thermosphere-ionosphere Na layers and mid-latitude thermosphere-ionosphere Na layers (Mid-TINa). Then we analyze the last thermospheric Na layer in detail. Based on totaling 415 nights and approximately 3914 hours of observation from 2018 to 2020, there were only about 17 Mid-TINa events found (with an occurrence rate of only 4.1%, mostly in winter). Among the 14 complete events analyzed, only about 35.7% (5/14) of the events' occurrence time is similar but earlier than the Sporadic E (Es) layers observed at the adjacent ground-based station. The remaining 9 events occurred between 2.5 to 8.6 hours after the latest Es layers. This weak correlation suggests that Mid-TINa layers may be triggered by other possible formation mechanisms.

The mesopause–lower thermosphere (MLT) region is an important spatial region in the Earth’s atmosphere, making it a valuable area to investigate the temperature variations. Kirchhoff’s law fails with the altitude increase due to the non-local thermal equilibrium effect, resulting in an increase in the error of the method to retrieve the atmospheric temperature in the MLT region using the A-band spectral line intensity. In the non-LTE state, the temperature retrieval method based on the Einstein coefficients is proposed to retrieve atmospheric temperature in the 92–140 km height range using the airglow radiation intensity images obtained from the Michelson Interferometer for global high-resolution thermospheric imaging (MIGHTI) measurements. Results show that the temperature deviation of the two-channel combinations does not exceed 15 K in the altitude range of 92–120 km. This deviation increases up to 45 K when the altitude is in the range of 120–140 km due to the influence of the N2 airglow spectrum. The two-channel combinations self-consistency is increased by 85 K compared with the temperature obtained using the spectral line intensity retrieval. Additionally, the comparison of the retrieval results with the spectral line intensity method and the comparison with the atmospheric chemistry experiment Fourier transform spectrometer (ACE-FTS) temperature measurement data shows that the Einstein coefficient method is significantly more rational and accurate than the spectral line intensity method.

The detection ability of SO2 cameras has been improved effectively, while the calibration is still the main factor that limits their measurement accuracy. This paper presents a nonlinear calibration theory by considering the effect of light dilution due to the path radiance as well as the dependence of plume aerosol on scattering wavelength. This new spectral calibration method is used to retrieve the SO2 column density and emission rate of the Etna volcano. Results show that, compared with the DOAS calibration approach, the inversion error can be reduced by 13% if the new spectral calibration is adopted. The superiority of the proposed method will become more obvious for long-distance detection of optically thick plumes.