F. S. Stephens’s research while affiliated with Lawrence Berkeley National Laboratory and other places

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Publications (467)


HEAVY ION COULOMB EXCITATION OF DEFORMED NUCLEI
  • Chapter

November 2023

R. M. Diamond

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F. S. Stephens

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B. Elbek

Experimental View of Backbending and BCS

March 2013

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14 Reads

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1 Citation

In rotating nuclei, backbending appears to be a large increase in the moment of inertia of a band, accompanied by a decrease in the rotational frequency. This has been shown to be a band crossing where one band (e.g. the ground or vacuum band) is crossed by a band in which the Coriolis force has unpaired two high-j nucleons and aligned their angular momentum with the rotation axis of the nucleus. With increasing spin this force gradually quenches the nuclear pairing correlations, with one or two of these band crossings in the process. © 2013 by World Scientific Publishing Co. Pte. Ltd. All rights reserved.


Band structure of 235U

December 2012

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25 Reads

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8 Citations

Physical Review C

D. Ward

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A. O. Macchiavelli

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R. M. Clark

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[...]

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C. Y. Wu

Over a period of several years we have performed three separate experiments at Lawrence Berkeley National Laboratory's 88-Inch Cyclotron in which 235U (thick target) was Coulomb-excited. The program involved stand-alone experiments with Gammmasphere and with the 8pi Spectrometer using 136Xe beams at 720 MeV, and a CHICO-Gammasphere experiment with a 40Ca beam at 184 MeV. In addition to extending the known negative-parity bands to high spin, we have assigned levels in some seven positive-parity bands which are in some cases (e.g., [631]1/2, [624]7/2, and [622]5/2) strongly populated by E3 excitation. The CHICO data have been analyzed to extract E2 and E3 matrix elements from the observed yields. Additionally, many M1 matrix elements could be extracted from the γ-ray branching ratios. A number of new features have emerged, including the unexpected attenuation of magnetic transitions between states of the same Nilsson multiplet, the breakdown of Coriolis staggering at high spin, and the effect of E3 collectivity on Coriolis interactions.


Table 1: Experimental conditions. 
Figure 1: Proposed level scheme for 254 No. Transition energies are given in keV. Suggested spins and parities of the states are indicated.  
Figure 2: Energy spectrum of gamma rays in coincidence with electron bursts from 257 Rf for all r-e events that did not have a spontaneous fission event following the electron. Asterisks indicate known Rf X-rays. The red circles represent gamma-ray lines that match the transition energies calculated with the rotational model. The results discussed below on 257 Rf were first reported by our group in the paper by Berryman et al. [19]. A total of 1904 r-α( 257 Rf) events were recorded. The half life for all r-α( 257 Rf) events was deduced to be 4.8 ± 0.2 s, which agrees with the value of 4.7 ± 0.3 s given in a recent paper by Qian et al. [20]. There were a total of 1083 r-e events, indicating the presence of an isomer. Conversion electrons coming from the decay of 257 Rf were distinguished from those coming from the decay of 256 Rf by observing an α decay following the conversion electron in the same pixel of the DSSD. There were 371 such events, labeled r-e-α( 257 Rf). The time difference between recoil implants and the subsequent electron burst for all r-e-α( 257 Rf) events was fit using a maximum likelihood method with an exponential decay, yielding a half life of 134.9 ± 7.7 µs for the isomeric state. Qian et al. [20] collected 22 r-e-α( 257 Rf) events, and they measured a half life of 160 +42 −31 µs, which is in agreement with our value. The γ-ray spectrum obtained in prompt coincidence with the electron bursts for all r-e events that did not have a spontaneous fission event following the electron is shown in Fig. 2. K-shell X-rays at energies expected for Rf [21] are seen (marked with an asterisk), along with a few prominent γ lines which are attributed to 257 Rf. While the γ-ray statistics are low, the presence of two high-energy γ lines at 446 keV and 585 keV may be attributed to the decay of the isomer. This work represents the first observation of any significant γ rays originating from the isomeric decay of 257 Rf. Qian et al. [20] observed seven γ-ray events in coincidence with a delayed electron event, but could only identify two counts associated with K-shell X-rays. Our data supports the findings of Qian et al. [20] and adds further information to the level scheme of 257 Rf. The differences in rotational energy levels built on the [725]11/2 − state were calculated using the simple rotational model. Possible γ lines matching these rotational energy differences were found within the γ-ray energy spectrum in Fig. 2 and labeled with a red circle. On this basis, we present a postulated decay scenario, which is shown in Fig. 3. Additional support for the decay scenario comes from looking at the total excitation energy for r-e-α( 257 Rf) events, which is the sum of the electron and γ-ray energies for each event. We observe an energy spectrum that ends at a maximum energy of ≈1050 keV. The energy difference between the [725]11/2 − state and the 134 µs isomeric state is 1080 keV based on our proposed decay scenario, which is comparable to the observed excitation energy.  
Nuclear spectroscopy of the heaviest elements: Studies of 254No, 257Rf, and 261Sg
  • Article
  • Full-text available

September 2011

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81 Reads

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2 Citations

Journal of Physics Conference Series

Recently it has become possible to perform detailed spectroscopy on nuclei beyond Z = 100 with the aim of understanding the underlying single-particle structure of superheavy elements. A number of such experiments have been performed at the 88-Inch Cyclotron of the Lawrence Berkeley National Laboratory using the Berkeley Gas-filled Separator (BGS), coupled with delayed γ-ray and electron-decay spectroscopy. Experiments have been performed on 254No (Z = 102), 257Rf (Z = 104), and 261Sg (Z = 106). The results provide new information on the properties of transactinide nuclei, which is important for testing models of the heaviest elements.

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High-K multi-quasiparticle states in 254No

June 2010

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51 Reads

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70 Citations

Physics Letters B

We report results from an experiment on the decay of the high-K isomers in 254No. We have been able to establish the decay from the known high-lying four-quasiparticle isomer, which we assign as a Kπ=16+ state at an excitation energy of Ex=2.928(3) MeV. The decay of this state passes through a rotational band based on a previously unobserved state at Ex=2.012(2) MeV, which we suggest is based on a two-quasineutron configuration with Kπ=10+. This state in turn decays to a rotational band based on the known Kπ=8− isomer, which we infer must also have a two quasineutron configuration. We are able to assign many new gamma-rays associated with the decay of the Kπ=8− isomer, including the identification of a highly K-forbidden ΔK=8 E1 transition to the ground-state band. These results provide valuable new information on the orbitals close to the Fermi surface, pairing correlations, deformation and rotational response, and K-conservation in nuclei of the deformed trans-fermium region.


High-K multi-quasiparticle states and rotational bands in _ {103}^{255} Lr

September 2009

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33 Reads

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33 Citations

Physical Review C

Two isomeric states have been identified in 255Lr. The decay of the isomers populates rotational structures. Comparison with macroscopic-microscopic calculations suggests that the lowest observed sequence is built upon the [624]9/2+ Nilsson state. However, microscopic cranked relativistic Hartree-Bogoliubov (CRHB) calculations do not reproduce the moment of inertia within typical accuracy. This is a clear challenge to theories describing the heaviest elements.


Multi-quasiparticle states in Rf256

February 2009

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28 Reads

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55 Citations

Physical Review C

Excited states in Rf256 were populated via the Pb208(Ti50,2n) fusion-evaporation reaction. Delayed γ-ray and electron decay spectroscopy was performed and three isomeric states in Rf256 have been identified. A fourth low-energy nonyrast state was identified from the γ-ray decay of one of the higher lying isomers. The states are interpreted as multi-quasiparticle excitations.



Determination of the position resolution of a segmented HPGe detector using a collimated source

October 2008

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6 Reads

New techniques in the use of highly-segmented HPGe detectors enable the tracking of the path of a scattered gamma ray in the detector. This enables precision Doppler correction of gamma rays emitted from fast-moving sources for high-resolution spectroscopy at radioactive beam facilities. Critical to these applications is a knowledge of the position resolution to which the scattering points can be determined. We directly measured the position resolution of using a highly collimated Cs source. Signal decomposition was used to determine the position and charge deposition of the interaction points from the scattered gamma ray in the crystal, followed by tracking to identify the first interaction point. The set of first interaction points form a line through the detector and their dispersion gives the position resolution of the crystal in two dimensions. Such a measurement was performed with the 36-way segmented GRETINA P3 prototype detector the position resolution was found to be sigmax = 1.5 mm and sigmay = 1.7 mm.


Intruder excitations in^{35} P

September 2008

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20 Reads

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19 Citations

Physical Review C

The structure of the neutron-rich N=20 nucleus 35P has been investigated through nucleon transfer experiments using the 208Pb(36,Xγ) reaction at 230 MeV. The level structure, of mainly 1ℏω excitations in 35P, has been significantly expanded. The measurements are compared with shell model calculations. Experimental branching ratio limits are reported for predicted transitions to the 2ℏω bandheads in 35P and 34Si.


Citations (49)


... U is generally renormalized to U −2∆ p , where 2∆ p , known as the backshift parameter, takes the pairing interaction into account. Recently, however, detailed analyses [153,172] have suggested that the magnitude of ∆ p should be much smaller than usually used, or neglected entirely. This, then, is an additional factor which adds uncertainty to current knowledge of Γ N . ...

Reference:

Dephasing and decoherence in open quantum systems: A Dyson's equation approach
Quasicontinuous decay spectra of superdeformed bands in 192,194Pb and energy gaps in level density at moderate angular momenta
  • Citing Article
  • March 2000

... Zirkonyum diborür (ZrB 2 ), pota ve termokupl astarı yapımında, alüminyum elektrolizinde katot kaplamasında, kesme ve aşındırma takımlarında, hipersonik uçakların ve roket atış sistemlerinin termal korumasında, nozullarda, zırh uygulamalarında ve nükleer reaktörlerde durdurucu olarak kullanılmakta veya kullanıma aday görülmektedir [3][4][5]. Ayrıca zirkonyum diborürün süperiletkenlik davranışları literatürde incelenmiş ve güncel olarak da incelenmeye devam etmektedir [6][7]. Çeşitli oksit ya da karbür katkıları ile geliştirilen zirkonyum borür esaslı kompozit malzemeler (ZrB 2 -ZrC, ZrB 2 -ZrO 2 , ZrB 2 -SiC, ZrB 2 -SiO 2 , ZrB 2 -B 4 C, vb.) mükemmel fiziksel ve mekanik özellikler göstermektedirler [8]. ...

Band structure of 235U
  • Citing Article
  • December 2012

Physical Review C

... Numerous studies were performed within the surrogate approach [23,[25][26][27][28][29][30][31] yielding encouraging results in a few particular cases: neutron capture, fission, and, recently, also the (n, p) channel [32]. The surrogate method generates the nucleus of interest that undergoes fission or γ decay through a direct reaction induced by a high-energy charged particle. ...

Deducing the 237U(n,f) cross section using the surrogate ratio method
  • Citing Article
  • May 2006

Physical Review C

... The rotational band resulting from this mechanism possesses increasing B(M1)/B(E 2) ratio, and decreasing B(M1) value with increasing rotational frequency. While the presence of the MR band is a very common phenomenon around the neutron-deficient Pb region [5][6][7], the observation of the MR band [8][9][10][11] in the above Pb region (Z = 82) around N = 126 neutron shell closure is rare due to insufficient experimental data at the high spin. The presence of the MR band in this region has already been reported for 203,204 At (Z = 85) [12,13], 202 Bi (Z = 83) [14], 201,202 Pb (Z = 82) [15], and 206 Fr (Z = 87) [16]. ...

Magnetic rotation in 197Pb and 198Pb
  • Citing Article
  • February 2001

Nuclear Physics A

... It has been demonstrated that the additional spectral line widening due to charge trapping depends not only on CCE but also on the electronic and Fano noises, so that higher causes a higher excess line widening for the same CCE [55]. Effects of charge trapping have been observed both in detectors made with compound semiconductors as with germanium and silicon, due to several different causes as: significant defect or impurity density both native as due to radiation damage, presence of volumes with low electric field [56][57][58][59][60][61][62] ...

Effects of neutron damage on the performance of large volume segmented germanium detectors
  • Citing Article
  • June 2005

Nuclear Instruments and Methods in Physics Research Section A Accelerators Spectrometers Detectors and Associated Equipment

... Most tracking algorithms attempt to reconstruct the tracks of photons, which have been fully absorbed in the Ge detectors (there is the notable exception of the TANGO algorithm [9], which also identifies Compton escape events, see section 4). There are two categories of tracking algorithms: forward-tracking algorithms [10], which start from the known position of the source and reconstruct the track of photons as they interact in the detector and back-tracking algorithms [11], which start from the potential photoelectric interaction point and reconstruct the track backwards to the source. Forward-tracking algorithms have been demonstrated to be more efficient than back-tracking algorithms [12] and are therefore used both at AGATA [1] and GRETINA [13]. ...

A ??-ray tracking algorithm for the GRETA spectrometer
  • Citing Article
  • June 1999

Nuclear Instruments and Methods in Physics Research Section A Accelerators Spectrometers Detectors and Associated Equipment

... As the mass number increases in these Pd nuclei, the deformation is expected to gradually change toward an oblate shape beyond 111 Pd [3]. However, past experiments have shown that the yrast structures in 113,115,117 Pd nuclei correspond to rotational bands arising from a prolate deformation [4][5][6]. The present experiment investigates these bands with very high statistics data to better determine the energy levels of odd-A Pd nuclei in this region. ...

vh11/2 bands in 113Pd and 115Pd
  • Citing Article
  • August 1999

Physical Review C

... The energy-level staggering in γ-bands in the chain of the Pd isotopes was analyzed in Ref. [7]. The levels of the γ-bands in 108 Pd [7], 110 Pd [7], 112 Pd [8] are grouped as 2 + , (3 + ,4 + ), (5 + ,6 + ) and etc., which is consistent with γ-soft behavior accordingly to the model of Wilets and Jean [9]. While the γ-bands are not so well developed in 102,104,106 Pd as in the heavier Pd isotopes, the amplitude of the staggering effect decreases in 114 Pd and 116 Pd with respect to that in 108,110,112 Pd, where it reaches its maximum [7]. ...

Spectroscopy of 112 Pd using heavy-ion-induced fission
  • Citing Article
  • February 2001

European Physical Journal A

... Custom readout electronics provided amplified, differential pulses from the HPGe detector charge collection process [29]. These signals were recorded by digitizers developed for the GRETINA experiment [30,31] which were read out using the Object-oriented Real-time Control and Acquisition (ORCA) software package [32][33][34]. ...

GRETINA: A gamma ray energy tracking array
  • Citing Article
  • December 2004

Nuclear Physics A