Natural radioactivity and radon exhalation rate in Brazilian igneous rocks
This paper reports the natural radioactivity of Brazilian igneous rocks that are used as dimension stones, following the trend of other studies on the evaluation of the risks to the human health caused by the rocks radioactivity as a consequence of their use as cover indoors. Gamma-ray spectrometry has been utilized to determine the (40)K, (226)Ra and (232)Th activity concentrations in 14 rock types collected at different quarries. The following activity concentration range was found: 12.18-251.90 Bq/kg for (226)Ra, 9.55-347.47 Bq/kg for (232)Th and 407.5-1615.0 Bq/kg for (40)K. Such data were used to estimate Ra(eq), H(ex) and I(γ), which were compared with the threshold limit values recommended in literature. They have been exceeded for Ra(eq) and H(ex) in five samples, where the highest indices corresponded to a rock that suffered a process of ductile-brittle deformation that caused it a microbrecciated shape. The exhalation rate of Rn and daughters has also been determined in slabs consisting of rock pieces ~10 cm-long, 5 cm-wide and 3 cm-thick. It ranged from 0.24 to 3.93 Bq/m(2)/h and exhibited significant correlation with eU (=(226)Ra), as expected. The results indicated that most of the studied rocks did not present risk to human health and may be used indoors, even with low ventilation. On the other hand, igneous rocks that yielded indices above the threshold limit values recommended in literature may be used outdoors without any restriction or indoors with ample ventilation.
Available from: Şeref Turhan
- "Volcanic tuff stones consisting of consolidated volcanic ash, and large and small pieces ejected from vents during a volcanic eruption, with a porous structure in different colours, are used as covering materials for insulating and ornamental purposes on the exterior and interior of buildings in Turkey. Up until now, several studies on the radiometric, petrographic and mineralogical properties of natural stone samples have been reported (Anjos et al., 2005; Xinwei et al., 2006; El-Arabi, 2007; Asghar et al., 2008; Kitto et al., 2009; Koornneef et al., 2010; Lanzo et al., 2010; Moura et al., 2011; Abd El-Ghafour et al., 2012; Capaccioni et al., 2012; Trevisi et al., 2012; Turhan, 2012). However, according to our literature survey, a comprehensive study related to the radiometric properties of volcanic tuff samples collected from Turkey has not yet been conducted, except one study in which eight volcanic tuff samples were considered (De˘ gerlier, 2013). "
Available from: Isam Salih
- "The new types of building materials are brought from various places around the world, and some may be extracted from areas with high background radiation . The contribution of building materials to indoor radon has been investigated in some previous studies in different regions   . "
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ABSTRACT: Radon levels and radioactivity were measured in 50 shops and storage areas for building materials in Sudan. Charcoal canister and gamma spectrometry systems were used to measure radon in 55 types of natural material, and concentrations of 71-292 Bq/m3 (mean, 154 ± 38 Bq/m3) were found. The concentration of radium (226Ra) ranged from 2.8 to 182.5 Bq/kg, of thorium (232Th) from 1.2 to 302 Bq/kg and of potassium (40K) from 82.3 to 1413.3 Bq/kg. Porcelain, ceramic and marble showed high values, while gravel types had low radioactivity. Radium in building materials was well correlated with radon (r2 = 0.77). The average annual dose of workers at these sites due to inhalation of radon was estimated to be 2.8 mSv. The activity index of building materials ranged between 0.33 and 1.97 (mean, 0.77).
Available from: Csaba Szabo
- "and they are widely used in recent publications for presenting the radioactive hazard of building materials (e.g. Al-Sulaiti et al., 2011; Damla et al., 2011; Moura et al., 2011). "
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ABSTRACT: Building materials and their additives contain radioactive isotopes, which can increase both external and internal radioactive exposures of humans. In this study Hungarian natural (adobe) and artificial (brick, concrete, coal slag, coal slag concrete and gas silicate) building materials were examined. We qualified 40 samples based on their radium equivalent, activity concentration, external hazard and internal hazard indices and the determined threshold values of these parameters. Absorbed dose rate and annual effective dose for inhabitants living in buildings made of these building materials were also evaluated. The calculations are based on (226)Ra, (232)Th and (40)K activity concentrations determined by gamma-ray spectrometry. Measured radionuclide concentrations and hence, calculated indices and doses of artificial building materials show a rather disparate distribution compared to adobes. The studied coal slag samples among the artificial building materials have elevated (226)Ra content. Natural, i.e. adobe and also brick samples contain higher amount of (40)K compared to other artificial building materials. Correlation coefficients among radionuclide concentrations are consistent with the values in the literature and connected to the natural geochemical behavior of U, Th and K elements. Seven samples (coal slag and coal slag concrete) exceed any of the threshold values of the calculated hazard indices, however only three of them are considered to be risky to use according to the fact that the building material was used in bulk amount or in restricted usage. It is shown, that using different indices can lead to different conclusions; hence we recommend considering more of the indices at the same time when building materials are studied. Additionally, adding two times their statistical uncertainties to their values before comparing to thresholds should be considered for providing a more conservative qualification. We have defined radon hazard portion to point to the limitations of the internal hazard considerations based on only measured (226)Ra activity concentrations without direct radon measurements. Our data are compared to those obtained in other countries and they provide a good basis to expand the database of radioactivity of building materials and gives information about the safety and situation of the building material industry in this central region of Europe.
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