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Lateral and axisymmetric ferrofluid oscillations in a cylindrical
tank in microgravity
Álvaro Romero-Calvo
Department of Aerospace Engineering Sciences, University of Colorado Boulder, Boulder, CO, United States
Antonio J. García-Salcedo, Francesco Garrone, Inés Rivoalen§, and Filippo Maggi
Department of Aerospace Science and Technology, Politecnico di Milano, Milan, Italy
I. Introduction
Magnetic polarization forces are becoming increasingly popular in space technology as a means of controlling
multiphase flows in reduced gravity environments. Applications include mass transfer [
1
5
], spacecraft propulsion
[
6
8
], thermomagnetic convection [
9
,
10
], phase separation [
11
], sample holding [
12
], or diamagnetically-enhanced
electrolysis [
13
], among others. The polarization force can be induced on natural liquids and magnetically-enhanced
substances, which are classified as diamagnetic, paramagnetic, or ferromagnetic. Although the dia/paramagnetic force is
so weak that terrestrial applications are almost nonexistent, in microgravity even the slightest disturbance can determine
the behavior of a fluid system [
14
]. The same force acting on a highly-susceptible ferrofluid can be dominant both on
Earth and in space [15].
The simulation of low-gravity multiphase flows subject to inhomogeneous polarization forces is severely complicated
by the coupling between fluid and magnetic problems and the presence of strong capillary forces [
16
]. However, some
of the most important space applications can still be addressed by means of efficient quasi-analytical tools. Following
the track of classical low-gravity fluid mechanics research [
17
,
18
], recent works have focused on the study of the
equilibrium, stability, and free surface oscillations of inviscid magnetic liquid interfaces [
19
]. The latter is of particular
importance for the development of novel magnetic liquid sloshing control devices, which have been recently proposed to
complement or substitute traditional capillary propellant management devices [
16
]. The final goal of such systems is to
transform a highly unpredictable propellant sloshing problem into a simple and reliable superposition of analogous
linear oscillators.
Even though low-gravity liquid sloshing and its interactions with spacecraft dynamics continue to be very active
fields of research [
20
26
] and a number of publications have explored the magnetic positioning of liquid oxygen and
low-susceptibility ferrofluids in microgravity [
27
35
], the study of highly susceptible ferrofluids for space applications
Graduate Research Assistant, Department of Aerospace Engineering Sciences, University of Colorado Boulder,
alvaro.romerocalvo@
colorado.edu, AIAA Student Member.
Graduated student, Department of Aerospace Science and Technology, Politecnico di Milano.
Graduated student, Department of Aerospace Science and Technology, Politecnico di Milano.
§Graduated student, Department of Aerospace Science and Technology, Politecnico di Milano.
Associate Professor, Department of Aerospace Science and Technology, Politecnico di Milano, AIAA Senior Member.
Accepted Manuscript
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is still in its infancy. The accurate determination of the modal shapes and frequencies of oscillating ferrofluid surfaces
in low-gravity is, however, critical for magnetic sloshing control devices. In order to cover this fundamental gap, the
European Space Agency (ESA) Drop Your Thesis! 2017 [
36
,
37
] experiment studied the axisymmetric oscillations
of water-based ferrofluids in cylindrical tanks when subjected to an inhomogeneous magnetic field in microgravity.
The results show that the theoretical model presented in Ref.
19
overestimates the axisymmetric magnetic frequency
response, pointing to the existence of unaccounted physical effects such as viscous damping or a complex magnetic
influence on the contact line hysteresis process [
38
]. Lateral oscillations, which have an intrinsic technical value as main
sources of attitude disturbances, remained unexplored. The United Nations Office for Outer Space Affairs (UNOOSA)
DropTES 2019 StELIUM experiment, whose design is described in Refs. [
39
41
], was subsequently launched at the
drop tower of the Center of Applied Space Technology and Microgravity (ZARM) to complement the analysis initiated
in Ref. 38 with the lateral sloshing case.
This technical note presents the final results of the UNOOSA DropTES 2019 StELIUM experiment and addresses the
influence of the magnetic field generated by a circular coil on the fundamental axisymmetric and lateral frequencies of an
oscillating ferrofluid located in a cylindrical tank in microgravity. Predictions from the aforementioned quasi-analytical
free surface oscillations model are compared with the experiments under different regimes. The framework of analysis
introduced in Ref.
19
is summarized in Sec. II, followed by a description of the experimental methods in Sec. III and the
discussion of results in Sec IV.
Fig. 1 Geometry of the system under study.
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II. Magnetic free surface oscillations model
The system under study, represented in Fig. 1, consists of an upright cylindrical tank with radius
𝑎
that contains a
volume
𝑉
of a water-based ferrofluid in microgravity. The liquid is incompressible and Newtonian, and has density
𝜌
,
surface tension
𝜎
, and static wall contact angle
𝜃𝑐
. The free space is filled by air at pressure
𝑝𝑔
. In microgravity, a coil
located at the base of the vessel generates an inhomogeneous axisymmetric magnetic field
𝑯
that interacts with the
magnetic fluid with magnetization
𝑀
(
𝐻
), with
𝐻
and
𝑀
being the modules of their corresponding vector fields. In
Fig. 1,
𝑠
is a curvilinear coordinate along the meniscus with origin in the vertex
𝑂
, and the local vertical coordinates
are given by
𝑤
(fluid surface - vertex),
𝑓
(meniscus - vertex) and
(fluid surface - meniscus). The dynamic (
𝑆
) and
static (
𝑆0
) fluid surfaces meet the wall
𝑊
of the vessel at the contact lines
𝐶
and
𝐶0
, respectively. The set of cylindrical
coordinates {𝑟, 𝜃 , 𝑧}, centered at the vertex of the meniscus, is considered in the analysis.
The oscillations of free liquid surfaces in microgravity have traditionally been studied through modal analysis [
42
,
43
]
and then validated using microgravity experiments [
44
52
] already since the development of the first non-magnetic
low-gravity free surface oscillation model by Satterlee and Reynolds in 1964 [
53
]. One of the main reasons for adopting
this approach is the complete analogy between the modal decomposition process and the superposition of linear
spring-mass-damper systems employed to model liquid sloshing [
14
,
18
,
54
,
55
]. The framework here presented for
magnetic liquids, summarized from Ref.
19
, is not an exception. It assumes an inviscid, potential, isothermal, and
magnetically dilluted flow to which the ferrohydrodynamic Bernoulli equation [
56
] is applied. After linearizing the
equations of motion around the meniscus, the variational principle
(1a)
𝐽
=
𝑆0"H2
𝑅
1 + 𝐹2
𝑅3/2
+
1
𝑅2
H2
𝜃
1 + 𝐹2
𝑅1/2
+
𝐵𝑜
+
𝐵𝑜mag
(
𝑅
)
H2
Ω
2
Φ
H#𝑅𝑑𝑅 𝑑𝜃
Ω
2𝑊
Φ
𝐺𝑅𝑑𝑅𝑑𝜃
Γ
Z𝐶0"H2
1 + 𝐹2
𝑅3/2#𝑅=1
d
𝜃
=
extremum
is obtained, subjected to
2Φ= 0 in 𝑉 , (1b)
H=Φ𝑍𝐹𝑅Φ𝑅on 𝑆0,(1c)
𝐺=Φ𝑍𝑊𝑅Φ𝑅on 𝑊, (1d)
H𝑅=ΓHon 𝐶0,(1e)
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where the subindices denote the partial derivatives. The magnetic Bond number is defined as
𝐵𝑜mag (𝑅) = 𝜇0𝑎2
𝜎𝑀𝜕𝐻
𝜕𝑧 + M𝑛
𝜕M𝑛
𝜕𝑧 𝐹(𝑅)
,(2)
and describes the ratio between magnetic and surface tension forces. The dimensionless cylindrical coordinates
𝑅
=
𝑟/𝑎
,
𝑍
=
𝑧/𝑎
, vertical coordinates
𝐹
=
𝑓 /𝑎
,
𝜙
(
𝑅, 𝜃 , 𝑍, 𝑡
) =
p𝑔0𝑎3
Φ(
𝑅, 𝜃, 𝑍
)
sin
(
𝜔𝑡
),
(
𝑅, 𝜃 , 𝑡
) =
p𝑎𝑔0/𝜔2H
(
𝑅, 𝜃
)
cos
(
𝜔𝑡
),
circular frequency Ω
2
=
𝜌𝑎3𝜔2/𝜎
, and hysteresis parameter Γ=
𝑎𝛾
are employed with
𝑔0
= 9
.
81
𝑚/𝑠2
being the
gravitational acceleration at ground level,
𝜙
the dimensional perturbed velocity potential, and
𝜔
the dimensional circular
frequency.
𝐺
is a function defined by Eq. 1d that accounts for the non-penetration wall boundary condition and that
arises naturally after reducing a volume integral in the original form of Eq. 1a to a surface integral using Green’s
theorem, as described in Ref.
43
. The hysteresis parameter Γin Eq. 1e can be regarded as the dynamic equivalent of the
static contact angle
𝜃𝑐
, and describes how the dynamic surface interacts with the walls of the container. The limiting
cases Γ= 0 and Γ
→ ∞
lead to the free-edge and stuck-edge conditions, respectively. In other words, Γdescribes how
freely the contact line
𝐶
slides over the walls of the tank, and has consequently a large influence on the shape of the
eigenmodes and their associated eigenfrequencies [38].
The system described by Eqs. 1a-e is solved in two steps. First, the axisymmetric meniscus
𝐹
(
𝑅
)is computed with an
iterative algorithm that accounts for the fluid-magnetic coupling. The algorithm solves the meniscus balance equations
(derived in Ref.
19
) for a given magnetic field, and then the magnetic field is recomputed in Comsol Multiphysics
employing the new interface. The process is repeated until the vertex of the meniscus converges with an error of
±
0
.
1
mm. In a second step, Eqs. 1a-e are transformed into an eigenvalue problem by using Ritz’s method with a set of
admissible functions that enforce the boundary conditions given by Eqs. 1b-e. The process relies on the previously
computed axisymmetric meniscus
𝐹
(
𝑅
)and
𝐵𝑜mag
(
𝑅
)number, and takes the geometry and magnetic environment, the
physical properties of the liquid (
𝜌
,
𝜎
,
𝑀
(
𝐻
)), and the wall boundary conditions (
𝜃𝑐
,Γ) as inputs. The solution of the
eigenvalue problem is the eigenvalue
𝜔𝑛
and eigenmode
(𝑛)
for the axisymmetric or lateral mode
𝑛
. Further details on
the formulation and operation of this method can be found in Ref.
19
. Its implementation is fully equivalent (excluding
liquid and geometrical properties) to that described in Ref. 38.
III. Materials and methods
A. Experimental setup
The experimental setup of StELIUM, depicted in Fig. 2, is designed to operate in a 9.3 s catapult launch at ZARM’s
drop tower [
57
]. The system, that is thoroughly described in Ref.
39
, is subdivided into two identical assemblies that
contain a cylindrical Plexiglas container, a surrounding electromagnetic coil, and an horizontal linear slider that imposes
a lateral oscillation to the fluid in the middle of the flight. This oscillation induces a lateral sloshing wave that is
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Detection system
Container assembly
Drop tower capsule
ZARM’s drop tower
953 mm
200 mm
Fig. 2 Experimental setup (not in scale).
complemented with the axisymmetric wave induced by the initial launch acceleration. A restoring polarization force is
applied to the ferrofluid during this process by operating the coils with constant current intensities
𝐼
ranging from 0 to
20 A. The 20 A level generates an inhomogeneous magnetic force distribution with characteristic meniscus magnetic
Bond number and accelerations values of 35 and 0.71 m/s2, respectively.
The evolution of the free surface is captured by a custom device located on top of each container. A laser line
is pointed at the surface of the ferrofluid while a camera records its projection. The deformation of the line is then
correlated with the height of the surface, and the 3D liquid surface profile is extracted. The system is able to compute the
axisymmetric meniscus, from which the apparent contact angles
𝜃𝑐
are derived, and the evolution of the axisymmetric
and lateral waves along the direction of excitation. A modal projection is subsequently applied to compute the hysteresis
parameter Γfrom the lateral waves, while a Fast Fourier Transform of the movement of the laser line is employed to
extract the modal frequencies. Γis here assumed to be the same for axisymmetric and lateral modes. This assumption is
motivated by the difficulty in extracting Γin the axisymmetric case, where magnetic and non-magnetic modal shapes
are very similar [
38
]. Further details on the design and operation of the detection system can be found in Refs. [
40
,
41
].
B. Liquid properties
The liquid tank has 11 cm diameter and 20 cm height, and is filled up by a 1:5 volume solution of the Ferrotec
EMG-700 water-based ferrofluid. Oil-based options are discarded to avoid the visualization issues reported in previous
works [
27
]. The ferrofluid has a density of 1058 kg/m
3
, surface tension of 55
.
6mN/m, a viscosity of 1.448 mPa
·
s,
employs an anionic surfactant, and contains a 1.16% vol concentration of 10 nm magnetic nanoparticles. The
magnetization curve of the solution, that determines its magnetic response, was measured with a MicroSense EZ-9
Vibrating Sample Magnetometer, resulting in an initial magnetic susceptibility 𝜒= 0.39 and saturation magnetization
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Table 1 Experimental results for contact angle, fundamental oscillation frequency and damping ratios for
axisymmetric and lateral waves, and lateral hysteresis parameter
I
[A]
𝜃𝑐
[deg]
Γ
[-]
𝜔𝑎,1
[rad/s]
𝜉𝑎,1
[-]
𝜔𝑙,1
[rad/s]
𝜉𝑙,1
[-]
Upper
0 60.52 16.75 4.52 0.19 2.58 0.21
10 59.87 7.23 5.82 0.15 3.62 0.16
15 62.36 7.11 7.05 0.14 4.60 0.12
20 65.67 4.41 7.60 0.13 5.30 0.11
Lower
0 47.52 15.27 3.62 0.23 2.21 0.22
10 53.07 4.88 5.41 0.16 3.36 0.17
15 58.15 5.44 5.98 0.17 4.18 0.15
20 * * * * 4.90 *
*
Not available due to a malfunction of the primary detection
system.
𝑀𝑠= 4160 ±100 A/m. The curve is fitted with a function of the form
𝑀(𝐻) = 2
𝜋[𝜅1arctan (𝜅3𝐻)+𝜅2arctan (𝜅4𝐻)] ,(3)
where 𝜅1= 1120.25 A/m, 𝜅2= 3103.56 A/m, 𝜅3= 8.49 ·106m/A, and 𝜅4= 1.94 ·104m/A.
IV. Results and discussion
Estimations for the fundamental axisymmetric and lateral frequencies
𝜔𝑎/𝑙
, fundamental damping ratios
𝜉𝑎/𝑙
,
contact angle
𝜃𝑐
, and lateral hysteresis parameter Γare obtained after analyzing the laser line projection as described
in Sec. III.A. Results are shown in Table 1 as a function of current intensity
𝐼
for upper and lower containers. Data
for the lower container at the 20 A drop is recovered from a time-of-flight sensor. Even though they share the same
geometry and a very similar magnetic environment, each container has significantly different values of
𝜃𝑐
(two-sample
t-test
𝑡
(5) = 3
.
07,
𝑝
= 0
.
03), revealing dissimilar wettability conditions. An analogous bias is observed with Γ, although
in this case it is not statistically significant (
𝑡
(3) = 0
.
90,
𝑝
= 0
.
43). These effects may be attributed to the potentially
uneven application of the hydrophobic treatment over the internal walls of the tanks and to the large sensitivity of water
to surface contamination [58, 59].
Microgravity facilities are expensive to operate and their access is generally limited. Having only 4 launch
opportunities, the StELIUM team decided to favor the derivation of statistical trends rather than statistical repetitions.
The comparative analysis between individual data points shall thus be treated with care since data dispersion may impair
accuracy. Nevertheless, there seems to be a strong dependence between Γand
𝐼
when switching between non-magnetic
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Lower:
Upper: Experimental
Experimental
Interpolated Γ, θ
Interpolated Γ, θ
Mean Γ, θ
Mean Γ, θ
Free edge
Free edge
Stuck edge
Stuck edge
Axisymmetric Freq. [rad/s]
4
6
8
10
Coils current intensity [A]
0 5 10 15 20
Lateral Freq. [rad/s]
2
3
4
5
6
Coils current intensity [A]
0 5 10 15 20
Fig. 3 Axisymmetric (left) and lateral (right) fundamental frequencies as a function of the coils current
intensity.
(
𝐼
= 0 A) and magnetic (
𝐼
= 10 A) regimes. A 56.3% and 68.0% drop in Γis observed for upper and lower containers,
respectively, suggesting the existence of a shift from surface-tension-dominated to magnetic-force-dominated regimes.
To the best knowledge of the authors, this effect has not been reported before and should be confirmed by future studies.
In spite of the aforementioned limitations, solid statistical conclusions can be drawn through the application of
appropriate statistics to the variables of interest, as discussed in Ref.
38
. Figure 3 shows the fundamental axisymmetric
and lateral free surface oscillation frequencies as a function of current intensity. Experimental values, whose error
bands are derived by identifying the FFT resolution with the
±
3
𝜎
Gaussian interval, are superposed with free edge
(Γ= 0) and stuck edge (Γ
→ ∞
) estimations from the model described in Sec. II using mean contact angle values of
62.15°
and
52.91°
for upper and lower containers, respectively. The use of mean contact angle values is motivated by
the absence of a significant linear correlation between
𝐼
and
𝜃𝑐
for upper (
𝑟
(2) = 0
.
79,
𝑝
= 0
.
21) and lower (
𝑟
(1) = 0
.
99,
𝑝
= 0
.
10) containers
. From a technical perspective, reducing the number of inputs simplifies the characterization and
simulation of the system. The free edge condition is associated with the lowest free surface frequency, while the stuck
edge case sets the maximum possible value. Although experimental lateral frequencies fall withing those boundaries,
the same does not seem to happen in the axisymmetric case.
Two more theoretical predictions are superposed in Fig. 3: a first one that considers a linear interpolation of the
contact angle
𝜃𝑐
and hysteresis Γvalues reported in Table 1, and a second that assumes average
𝜃𝑐
and magnetic Γ
(upper: 6.25, lower: 5.16) results. Both curves are practically identical, exemplifying the small effect of the contact angle
variability, but diverge by
0.2 rad/s for
𝐼
= 0. This effect is attributed to the large increase of Γin the non-magnetic case.
The most remarkable feature of these predictions is, however, the excellent agreement with experimental results observed
for the lateral frequencies. While the interpolation of Γand
𝜃𝑐
results in an adjusted coefficient of determination
However, previous works [
60
62
] have reported a dependence between the apparent contact angle and the applied magnetic field of ferrofluid
droplets, an effect that should be explored with larger datasets for the setup employed in this work.
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𝑅2
adj
= 0
.
983 (with 3 explanatory variables, Γ,
𝜃𝑐
, and
𝐼
) and a mean-squared error of
𝑀𝑆𝐸
= 0
.
01 rad/s, the use of
averaged values returns
𝑅2
adj
= 0
.
976 with a single explanatory variable
𝐼
and an
𝑀𝑆𝐸
= 0
.
02 rad/s. Both models lead
to normally distributed residuals according to the Saphiro-Wilk test (
𝑝
= 0
.
075,
𝑊
= 0
.
84 and
𝑝
= 0
.
49,
𝑊
= 0
.
93 for
the fitted and averaged models, respectively). Interestingly, if the frequencies are computed with a restoring inertial
acceleration equivalent to the mean magnetic acceleration at the interface (which, for
𝐼
= 20 A, is
0.71 m/s
2
), the
deviation at 20 A is just
0.3 rad/s for both the free and stuck lateral cases. The reasons are that (i)
𝐵𝑜mag
(
𝑅
)remains
almost constant along the meniscus for this setup [
38
], and (ii) the meniscus profile is only slightly deformed by the
magnetic field. In other words, when these two conditions apply, the frequencies can be roughly estimated by assuming
a low-gravity interface subject to an equivalent inertial acceleration.
Results for lateral oscillations are in sharp contrast with the axisymmetric case, where the free-edge model
(
𝑅2
adj
= 0
.
873) performs much better than the rest (e.g. the averaged alternative,
𝑅2
adj
= 0
.
486). This is consistent with
the analysis reported in Ref.
38
, that assumes the free-edge condition, and with the fact that the Γvalues are derived
from the shape of the lateral sloshing waves. The magnetic response of the model (i.e. its current-frequency slope)
cannot be robustly assessed because, unlike in Ref.
38
, the small sample size prevents any meaningful comparison.
Furthermore, an
𝑅2
adj
coefficient of just 0.873 is far from acceptable for confirming or denying the conclusions of said
reference, where the analytical framework in Sec. II is shown to overestimate the axisymmetric free surface oscillation
frequencies. This effect is attributed to unmodeled physical effects, like the potential coupling between Γand
𝐼
reported
in Tab. 1, that may be addressed in a future work.
The damping ratios reported in Table 1 are computed by means of the half-power bandwidth method as
𝜉𝑎/𝑙 =1
2
Δ𝜔3𝑑𝐵
𝜔𝑎/𝑙
,(4)
where Δ
𝜔3𝑑𝐵
is the frequency peak width between the -3 dB points on the FFT spectrum. The division by
𝜔𝑎/𝑙
justifies
the decrease of
𝜉𝑎/𝑙
with
𝐼
. Most importantly, the excellent agreement between inviscid theoretical and experimental
lateral frequencies confirms the negligible impact of fluid viscosity and magnetically-induced viscosity [
56
,
63
] on the
sloshing problem for the system under study.
From a technical perspective, this analysis shows that, given an educated estimate of
𝜃𝑐
and Γand an appropriate
characterization of the geometric and magnetic environments, the inviscid model first introduced in Ref.
19
and
summarized in Sec. II is able to predict the lateral sloshing parameters of a highly-susceptible low-viscosity magnetic
liquid in microgravity. This is important for future space applications involving magnetic positive positioning or
magnetic liquid sloshing [
16
] since lateral oscillations represent the largest fuel-induced attitude control disturbance.
Furthermore, the results confirm the importance of coupling the magnetic and fluid problems for the study of the
dynamics of highly susceptible ferrofluids: if the simplified uncoupled model introduced in Ref.
38
was considered
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instead, the frequencies at 20 A would be underestimated by 1.37 rad/s and 0.74 rad/s for the axisymmetric and lateral
cases, respectively, falling well beyond the error bands. The excellent agreement between experimental results and
the averaged model, that operates employing a global estimation of
𝜃𝑐
and Γ, makes basic science discussions on
the dependence of such parameters on the applied magnetic field less relevant for most applications, at least for the
configuration here considered. The same can be said about axisymmetric oscillations, which have a weaker impact on
the spacecraft dynamics [14, 18].
V. Conclusions
The final results of the UNOOSA DropTES StELIUM experiment, that studies the axisymmetric and lateral
oscillations of a ferrofluid solution in a series of drop tower experiments, validate the quasi-analytical magnetic sloshing
model presented in Ref.
19
for the study of lateral oscillations. The small dependence of the contact angle and hysteresis
parameter with the applied magnetic field is shown to have an almost negligible impact on the frequency response of the
system under study, which simplifies the development of magnetic sloshing control devices. Although the presence
of unmodeled physical effects reported in Ref.
38
for the axisymmetric free surface oscillations problem cannot be
confirmed due to the small sample size, existing results indicate that the axisymmetric frequencies follow a free-edge
behavior rather than the measured lateral hysteresis parameter. The results highlight the importance of accounting for
the fluid-magnetic coupling in applications involving highly susceptible ferrofluids.
Competing Interests
The authors declare no competing interests.
Funding Sources
This work was supported by the United Nations Office for Outer Space Affairs (UNOOSA), the Center of Applied
Space Technology and Microgravity (ZARM) and the German Space Agency (DLR) in the framework of the UNOOSA
DropTES Programme 2019. Further financial and academic support was obtained from Ferrotec Corporation, Politecnico
di Milano, the University of Seville, the European Space Agency (ESA) and the European Low Gravity Research
Association (ELGRA). A.R.C. acknowledges the financial support offered by the La Caixa Foundation (ID 100010434),
under agreement LCF/BQ/AA18/11680099.
Acknowledgments
We acknowledge the financial, technical, and academic support offered by UNOOSA, DLR, ZARM, Ferrotec
Corporation, Politecnico di Milano, and the University of Seville. We also thank ESA and ELGRA for financing
the presentation of this work at the 70th International Astronautical Congress (IAC) and the 26th ELGRA Biennial
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Symposium and General Assembly. We are in debt with ZARM’s drop tower engineers Jan Siemer and Fred Oetken,
ZARM’s point of contact Dr Thorben Könemann and UNOOSAs point of contact Ayami Kojima for their endless
support. We would like to thank the technicians Giovanni Colombo, Alberto Verga and the PhD student Riccardo Bisin
from the Space Propulsion Laboratory (SPLab) of Politecnico di Milano for their academic and technical assistance, as
well as the rest of members of this research group for contributing to the creation of an extraordinary professional and
human environment. Finally, we acknowledge the support offered by Prof. Elena Castro-Hernández, Prof. Gabriel
Cano-Gómez, and Prof. Miguel Herrada in the early stages of the StELIUM project.
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12
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... Subsequent publications presented refined numerical models and numerical results of technical relevance [154,[164][165][166][167][168][169][170][171]. The axisymmetric and lateral sloshing of water-based ferrofluids was characterized in microgravity when subjected to an inhomogeneous magnetic field as part of the ESA Drop Your Thesis! 2017 [77,172,173] and UNOOSA DropTES 2019 [174][175][176][177] campaigns reported in Chapter 9. ...
... The magnetic field modifies the effective gravity acceleration of the system and shifts its natural frequencies, as reported in normal-gravity works [160,311]. If the magnetic term was approximately constant in R, like in the case of a linear magnetic field and a flat surface, the problem would be equivalent to the nonmagnetic system [162,177]. In this analysis, however, an inhomogeneous magnetic field is being considered. ...
Thesis
Full-text available
The commercialization of the sub-orbital environment, the ambition to make humans a multi-planetary species, and the urgent need for sustainable space operations are driving the development of a new generation of space systems. The use of electromagnetic forces (and electromagnetism, in general) is proposed in this dissertation to enable mid-distance, contactless actuation and sensing for space technology development. Following this paradigm, two applications are explored: electron-based touchless spacecraft potential sensing, and low-gravity magnetohydrodynamics. The electron-based touchless potential sensing method was recently introduced to characterize the electrostatic state of non-cooperative objects in GEO and deep space. Applications span from arcing prevention to space debris removal. Although the fundamentals of this approach were studied in previous works, several open questions remained regarding the effect of complex geometries and differential charging on the sensing process. Such questions are here addressed with efficient numerical tools and vacuum chamber experiments, providing key insights into the behavior of realistic spacecraft formations. In addition, new active photoelectron-based sensing strategies are proposed that overcome some of the challenges of previous implementations. The concept of low-gravity magnetohydrodynamics is also introduced as a way to actuate low-gravity fluid mechanics systems using magnetic forces. The theoretical foundations of the field are established from the analytical, numerical, and experimental perspectives with particular attention to the equilibrium, stability, and modal response of gas-liquid interfaces. Specific features of bubbles and droplets are also explored. Finally, the use of magnetic polarization and Lorentz forces in low-gravity fluid systems is discussed together with some of their applications, which include phase separation, magnetic positive positioning, and low-gravity electrolysis. The development of such technologies is initiated with support from microgravity research campaigns at ZARM's drop tower and Blue Origin's New Shepard suborbital rocket.
... An exception is the European Space Agency (ESA) Drop Your Thesis! 2017 The Ferros project, that studied the axisymmetric sloshing of water-based ferrofluids when subjected to an inhomogeneous magnetic field in microgravity [39][40][41]. Although the axisymmetric and lateral sloshing of ferrofluids were also studied during the United Nations Office for Outer Space Affairs (UNOOSA) DropTES 2019 experiment StELIUM [42][43][44], statistical significance was not achieved for the axisymmetric modes [45]. Therefore, the configuration of the Drop Your Thesis! 2017 experiment is adopted in this work. ...
... A quasi-analytical model was recently introduced to study the equilibrium and modal response of ferrofluid interfaces in microgravity [22]. The model has been shown to offer an excellent estimation of the lateral modal frequencies in the aforementioned UNOOSA DropTES 2019 campaign [45], but over-predicted the axisymmetric sloshing frequencies of the ESA Drop Your Thesis! 2017 experiment [41]. An additional (technical) motivation for this work is thus to shed light on this disagreement and develop a tool that provides the equilibrium, global stability, modal response, and time-dependent evolution of the capillary ferrohydrodynamic interfaces that may find application in space propulsion. ...
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Full-text available
A coupled ferrohydrodynamic interface-tracking model is introduced for the analysis of the equilibrium, linear stability, and modal response of magnetic liquid interfaces in surface tension-dominated axisymmetric multiphase flows. The incompressible viscous mass and momentum balances are solved together with the steady-state Maxwell equations by following a monolithic solution scheme. The method is fully implicit, allowing to reach a steady-state solution in a single time step. In addition, the time-dependent evolution of the interface subject to variable external inputs can also be simulated. The geometry is particularized for the study of the free surface oscillations of a ferrofluid in a cylindrical tank under the influence of an inhomogeneous magnetic field in microgravity. Five regions are used to discretize the simulation domain, which combines analytical and elliptic mappings. Magnetic field-free results are validated by the literature. The modal response of the fluid-magnetic system agrees with measurements from the European Space Agency (ESA) Drop Your Thesis! 2017 The Ferros experiment and improves previous quasi-analytical estimations. This new framework of analysis can be applied to the study of a wide variety of microfluidic and low-gravity fluid systems. Copyright by Elsevier. Downloaded papers are for personal use only, and are not to be sold in any way or included in any commercial package.
... Subsequent publications by Marchetta and coworkers presented refined numerical models and results of technical relevance for the development of liquid oxygen magnetic positioning devices [46][47][48][49][50][51][52][53][54]. Recent works have also explored the free surface oscillations of ferrofluids in microgravity, which may be relevant for slosh control and the development of novel PMDs [55][56][57][58][59][60]. A comprehensive review of the field can be found in Ref. 28. Significant advances have been made in the modeling and fundamental understanding of MP 2 devices during the last two decades. ...
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The active deorbiting and passivation of launch vehicles has become key for the implementation of modern space debris mitigation guidelines. Appropriate engine restart conditions must be provided as part of this process. Ullage motors have been traditionally employed to induce active settling and ensure a gas-free propellant supply to the engines. Although robust and reliable, ullage rockets are also heavy, which motivates the study of alternative approaches to the problem. Classic propellant management devices could potentially be employed in this context, but they are hardly applicable to high flow rate cryogenic liquid systems. This paper explores several novel propellant settling strategies that are particularly well suited for cryogenic propellants. In particular, three distinct Magnetic Positive Positioning concepts, a hydrogen-peroxide-based Propellant Gasification System, and a hybrid device that combines both approaches are introduced. The preliminary technical analysis indicates that the successful development of these technologies could lead to mass savings of hundreds of kilograms and economic gains of several hundred thousand dollars per launch.
... In modern literature the manifestations of several different capillary, hydrostatic, electro-and magnetostatic instabilities that take place at the interface of magnetic colloid (magnetic fluid) with other media under the influence of external force fields are known and intensively studied [1][2][3][4][5][6][7][8][9]. In the development of physics of magnetic colloids, much attention is traditionally paid to the problems of equilibrium shapes of their limited volumes determined by the action of magnetic interaction forces and surface tension. ...
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This paper presents experimental studies of the influence of an alternating magnetic field on the separation of magnetic liquid droplets from a capillary hole. The formation of waves on the surface of capillary volumes of a magnetic fluid flowing out of a capillary hole in a horizontal non-magnetic plate under the action of gravity in external alternating magnetic field is detected. Spherical, dumbbell-shaped, jet-shaped, and comb-shaped droplet geometries were observed. It is established that the shape of the waves formed could vary from waves running and standing on the surface of a growing drop to bending oscillations of a vertical fluid jet. The magnetic field parameters at which different instability patterns are observed were determined.
... [35][36][37][38][39][40][41][42][43] Recent works have also explored the free surface oscillations of ferrofluids in microgravity, which may be relevant for slosh control and the development of novel propellant management devices (PMDs). [44][45][46][47][48][49] A comprehensive review of the field can be found in Ref. 19. ...
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The active deorbiting and passivation of launch vehicles has become key for the implementation of modern space debris mitigation guidelines. Appropriate engine restart conditions must be provided as part of this process. Ullage motors have been traditionally employed to induce active settling and ensure a gas-free propellant supply to the engines. Although robust and reliable, ullage rockets are also heavy, which motivates the study of alternative approaches to the problem. This paper explores for the first time several high-risk-high-return propellant settling strategies that may result in significant benefits for future space systems. In particular, three distinct Magnetic Positive Positioning concepts, a hydrogen-peroxide-based Propellant Gasification System, and a hybrid device that combines both approaches are introduced. The preliminary feasibility analysis indicates that the successful development of these technologies may lead to mass savings of hundreds of kilograms and economic gains of several hundred thousand dollars per launch. However, the robustness of some of these methods may be compromised by complex fluid-structure interactions that require a careful numerical and/or experimental analysis.
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In this study, numerical simulations were conducted to explore the best possible magnetic field arrangement that can maximize the heat exchange performance of Fe3O4-water magnetic nanofluid. Orientation of magnets poles, number of magnets, and the distribution of magnetic field intensity over the flow path are studied to obtain the optimum design which is then tested at various values of magnetic nanoparticles volume fraction, magnetic flux density, and Reynolds number. Results indicated that the optimum design is achieved by placing magnets with N–N orientation and adjusting the magnetic flux density to increase by a rate of 100% between each two successive magnets along the path of the flow. Results also revealed that the average Nusselt number and pressure drop increase when the magnetic flux density is increased. Furthermore, it was found that the effect of increasing magnetic nanoparticles volume fraction on the heat transfer performance is higher at low Reynolds number. An increase of the average Nusselt number in the range of 16.44%–24.46% compared to the design without magnetic field was achieved when using the optimum design with an average magnetic flux density of 1000 Gauss, and magnetic nanoparticles volume fraction of 4%.
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This paper describes an inexpensive, non-invasive, and highly adaptable surface reconstruction device for opaque liquids. The instrument was developed to study the lateral sloshing of ferrofluids in microgravity as part of the UNOOSA DropTES 2019 StELIUM project. Its design is driven by the geometrical and mechanical constraints imposed by ZARM’s drop tower, where the experiment was launched in November 2019. The launch catapult and deceleration systems impose strong axial g-loads to a system that is confined in the reduced capsule environment. Redundant procedures are implemented to measure the first two lateral sloshing frequencies and damping ratios of the magnetic liquid, as well as its equilibrium surface in microgravity. Ideal vertical resolutions between 0.25 and 0.4 mm/px can be achieved with the configuration here proposed. The final performance depends, among other factors, on the correct application of the robust calibration procedure that is documented in this work.
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The management of fluids in space is complicated by the absence of relevant buoyancy forces. This raises significant technical issues for two-phase flow applications. Different approaches have been proposed and tested to induce phase separation in low-gravity; however, further efforts are still required to develop efficient, reliable, and safe devices. The employment of diamagnetic buoyancy is proposed as a complement or substitution of current methods, and as a way to induce the early detachment of gas bubbles from their nucleation surfaces. The governing magnetohydrodynamic equations describing two-phase flows in low-gravity are presented with a focus on bubble dynamics. Numerical simulations are employed to demonstrate the reachability of current magnets under different configurations, compare diamagnetic and Lorentz forces on alkaline electrolytes, and suggest scaling up procedures. The results support the employment of new-generation centimeter-scale neodymium magnets for electrolysis, boiling, and phase separation technologies in space, that would benefit from reduced complexity, mass, and power requirements.
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The sloshing of liquids in low-gravity entails several technical challenges for spacecraft designers due to its effects on the dynamics and operation of space vehicles. Magnetic settling forces may be employed to position a susceptible liquid and address these issues. Although proposed in the early 1960s, this approach remains largely unexplored. In this paper, the equilibrium meniscus and axisymmetric oscillations of a ferrofluid solution in a cylindrical tank are studied for the first time while subject to a static inhomogeneous magnetic field in microgravity. Coupled fluid-magnetic simulations from a recently developed inviscid magnetic sloshing model are compared with measurements collected at ZARM's drop tower during the ESA Drop Your Thesis! 2017 campaign. The importance of the fluid-magnetic interaction is explored by means of an alternative uncoupled framework for diluted magnetic solutions. The coupled model shows a better agreement with experimental results in the determination of the magnetic deformation trend of the meniscus, but the uncoupled framework gives a better prediction of the magnetic frequency response which finds no theoretical justification. Although larger datasets are required to perform a robust point-by-point validation, these results hint at the existence of unmodeled physical effects in the system.
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This paper addresses the operation in microgravity of the surface reconstruction device whose design is detailed in the first part of the manuscript. The system, employed during the drop tower campaign of the UNOOSA DropTES 2019 StELIUM experiment, studies the axisymmetric and lateral oscillations of a ferrofluid solution in microgravity. The free liquid surface is reconstructed in a cylindrical tank and relevant metrics of the magnetic sloshing problem, such as contact angles, hysteresis parameters, natural oscillation frequencies, or damping ratios, are derived. The result is a rich and unique database where several phenomena of scientific and technological interest are reported for the first time. The dependence of the fundamental axisymmetric and lateral modal frequencies with the applied magnetic field is consistent with the literature and past experiments. Although the detection system was designed and built using low-cost hardware, high-quality results are obtained.
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The sloshing of liquids in low-gravity entails several technical challenges for spacecraft designers and operators. Those include the generation of significant attitude disturbances, the uncontrolled displacement of the center of mass of the vehicle or the production of gas bubbles, among others. Magnetic fields can be used to induce the reorientation of magnetically susceptible propellants and improve the controllability of a fluid system. Despite being proposed in the early 1960s, this approach remains largely unexplored. This paper provides new insight into the prospects and challenges of using magnetic control of space propellants. Key unanswered theoretical and technical questions are identified, highlighting the importance of developing appropriate analytical tools and fluid-magnetic simulation frameworks. New results associated with the reachability, scaling, long-term thermal and radiation stability, and efficiency of paramagnetic and ferromagnetic propellants are presented. Magnetic settling forces are shown to enhance the stability and speed up the oscillatory response of the liquid, leading to more predictable propellant management systems for different scales and filling ratios. These effects are particularly relevant for ferrofluids, whose enhanced magnetic properties make them excellent candidates for active sloshing control applications in space.
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Liquid sloshing represents a major challenge for the design and operation of space vehicles. In low-gravity environments, a highly non-linear movement can be produced due to the lack of stabilizing forces. This gives rise to significant disturbances that impact on the propulsion and attitude control systems of the spacecraft. The employment of magnetically susceptible fluids may open an interesting avenue to address this problem, but their dynamics in low gravity remain practically unexplored. The UNOOSA DropTES StELIUM project aims at filling this gap by studying the lateral sloshing of a ferrofluid solution subjected to an inhomogeneous magnetic field in microgravity. This paper describes the design process, challenges and preliminary results of the experiment, which was successfully launched at ZARM's drop tower in November 2019. The outcomes will be employed to validate the quasi-analytical models developed by the authors and set the path for the design of magnetic propellant positioning devices in space.
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The formulation of the total force exerted by magnetic fields on ferrofluids has historically been a subject of intense debate and controversy. Although the theoretical foundations of this problem can now be considered to be well established, significant confusion still remains regarding the implementation of the associated expressions. However, the development of future applications in low-gravity environments is highly dependent on the correct modeling of this force. This paper presents a contextualized analysis of different proposed calculation procedures and validation in a space-like environment. Kinematic measurements of the movement of a ferrofluid droplet subjected to an inhomogeneous magnetic field in microgravity are compared with numerical predictions from a simplified physical model. Theoretical results are consistent with the assumptions of the model and show an excellent agreement with the experiment. The Kelvin force predictions are included in the discussion to exemplify how an incomplete modeling of the magnetic force leads to significant errors in the absence of gravity.
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The sloshing of liquids in microgravity is a relevant problem of applied mechanics with important implications for spacecraft design. A magnetic settling force may be used to avoid the highly non-linear dynamics that characterize these systems. However, this approach is still largely unexplored. This paper presents a quasi-analytical low-gravity sloshing model for magnetic liquids under the action of external inhomogeneous magnetic fields. The problems of free and forced oscillations are solved for axisymmetric geometries and loads by employing a linearized formulation. The model may be of particular interest for the development of magnetic sloshing damping devices in space, whose behavior can be easily predicted and quantified with standard mechanical analogies. Copyright 2019 by ASME. Downloaded papers are for personal use only, and are not to be sold in any way or included in any commercial package.
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A concept design of a novel orbit control system is presented. It is based on the acceleration and subsequent ejection of magnetofluid droplets. Overall, the Gauss gun principle is investigated and extended on the utilisation of ferrofluids. Based on results of the student experiment PAPELL (Pump Application Using Pulsed Electromagnets for Liquid reLocation), the development of this acceleration concept is performed. PAPELL is a technology demonstrator that has been conducted on the International Space Station in 2018. A non-mechanical pumping mechanism has been realised with it, utilising single ferrofluid droplets as working medium to be transported by changing local magnetic fields. A low-maintenance and high-lifetime system can be achieved by the removal of mechanical components, leading to a possible innovative technology for future space transportation systems. With PAPELL, it has been demonstrated that ferrofluid droplets can be transported, split and merged in a microgravity environment. Considering these results, the concept design of the in-orbit propulsion system is based on a multistage Gauss gun. Working with coils acting as magnetic field sources, switched on and off successively to accelerate ferrofluid droplets utilised as propellant, a novel propulsion system is achieved. In detail, the magnetic flux density of each coil generates an accelerating force acting on the propellant. An equation for the estimation of the exhaust velocities for the droplets is derived depending on the ferrofluid type, the coil parameters and the acceleration or respective system length. Possibilities of increasing the exhaust velocity and thus the specific impulse of the propulsion systems are discussed. Additionally, the power supply system for the coils as well as the coil switching control are investigated and a thermal control for the propulsion system is discussed. A storage and feeding concept for the ferrofluid as well as a concept for the formation of droplets for acceleration are presented. A subsequent performance analysis is conducted showing theoretical results of specific impulses in a range of competing electric propulsion systems. However, the specific impulses are limited due to technical feasibility which is investigated further in this paper. Additionally, application limits are discussed to assess future applications. The theoretically promising results of the performance analysis lead to the expectation of an extended and more detailed analysis as well as practical tests of the acceleration concept and further validation activities.
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