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6TheiaX, HZDR Innovation, Bautzner Landstraße 400, 01328 Dresden, Germany
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1. Introduc tion
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S.T. Thiele et al. Ore Geology Reviews xxx (xxxx) 104252
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2. Geological setting
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3. Photogrammetric survey
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4. Hyperspectral data pr oces sing with hylite
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4.1. Laboratory acquisition
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S.T. Thiele et al. Ore Geology Reviews xxx (xxxx) 104252
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S.T. Thiele et al. Ore Geology Reviews xxx (xxxx) 104252
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5B8 C6@=EI9 J=9K =B; 5B ;@9GC: H<9 9B=L =A5; 9FM H<9 HK C 85H5 G9HG K9F9
A9F;98 IG=B; DC=BH 5J9F5;9G K=H< 5 K9=;<H=B; :57HC F 9EI5@ HC H<9 N
7CADCB9BH C: 957< DC=BH’G BCFA5@ J97HCF -<IG GD97HF5 CB <CF=NCBH5@
D@5B9G 5F9 8CA=B5BH @M 89F=J98 :FCA H< 9 <=;< F9GC@IH=CB +=?C@5 =A5; 9FM
5B8 GD97HF5 CB J9FH=75@ D@5B9G :FCA H<9 9B=L =A5;9FM
5. Results: Data analysis and integration
?9M 89G=;B :95HIF9 C: hylite =G =HG IG9 C: DC@MACFD<=7 GHFI7HIF9G HC
F9DF9G9BH J5F=CIG <MD9FGD97HF5@ 85H5 9; GD97HF5@ @=6F5F=9G =A5;9G
<MD9F7@CI8G =B 5 IB=:CFA K5 M !9B79 GH5B85F8 5B5@MG=G H97<B=EI9G
GI7< 5G A=B=AIA K5J9@9B;H< A5DD=B; CF <I@@ 7CFF97H=CB 75B 69 >IGH 5G
95G=@M 5D D@=98 HC 5 GD97HF5@ @=6F5FM 5G 5 <M D9F7@CI8 -<=G =G :IB85A9BH5@
HC :5 7=@=H5H=B; 85H5 =BH9;F5H=CB 69HK 99B :CF 9L5AD@9 GD97HF5 57EI=F98
IG=B; 5 ]9@8 GD97HFCA9H9F 5 ;FCIB865G98 <MD9F7@CI8 5B8 59F=5@ =A
5;9FM
"B H<9 :C @@CK=B; G97H=CB K9 89ACBGHF5H9 H<=G 5DDFC57< 5B8 H<9 J5
F=9HM C: 5B5@MG=G HCC@G =AD@9A9BH98 =B hylite 6M =BH9;F5H=B; ,=GI+($
=A5;9FM C: <5B8G5AD@9G K=H< 5 <MD9F7@CI8 89F=J98 :FCA H9FF9GHF=5@
5B8 ./ =A5;9FM HC A5D H<9 ;9C@C;M C: H<9 CD9BD=H
5.1. Qualitative analysis and visualisation
G 5 DF9@=A=B5FM 85H5 9LD@CF5H=CB GH9D hylite K5G IG98 HC 7F95H9 5
G9F=9G C: HFI9 =; 5 5B8 :5 @G97C@CIF J=GI5@=G5H=CBG C: H<9 G75BB98
<5B8 G5AD@9G 5B8 <MD9F7@CI8 5@G97C@CIF F9DF9G9BH5H=CBG K9F9
7F95H98 IG=B; K5 J9@9B;H<G =B H<9 ,0"+ 5B8
BA H<5H 5F9 G9BG=H=J9 HC 7@5M 7<@CF=H9 5B8 A=75 A=B9F5@C;M
=; 6 /9889F 5B8 &7CB5@8 %C< )CBHI5@ 9H 5@
%5I?5AD 9H 5@ 5B8 IG=B; H<9 K=89@M 5DD@=98 A=B=AIA BC=G9
:F57H=CB &' F99B 9H 5@ 8=A9BG=CB5@=HM F98I7H=CB H97<B=EI9
=; 7 :C@@CK=B; H<9 =AD@9A9BH5H=CB =B SPy C;; G "BH9F57
H=J9 J=GI5@=G5H=CBG C: H<9 <MD9F7@CI8 5B8 =HG J5 F=CIG 89F=J5H=J9G 75 B
69 J=9K98 5H <HHDGH=BMIF@7CA75<MD9F7@CI8
0=H< H<9G9 J=GI5@=G5H=CBG 5G 5 F9:9F9B79 957< <5B8 G5AD@9 K5G 7@5G
G=]98 =BHC B=B9 GD97HF5@ @=H<C@C;=9G =; 65G98 CB =BH9FDF9H5H=CBG C:
=B8=J=8I5@ D=L9@ GD97HF5 -5 6@9 -<9G9 @=H<C@C;=9G K9F9 75F9:I@@M 7<C
G9B GI7< H<5H H<9M 5F9 GD97HF5@@M 8=GH=B;I=G<56@9 5B8 ;9C@C;=
75@@M A95B=B;:I@ !9B79 H<9M 5F9 @5F;9@M 89]B98 6M H<9 56IB85B79 C:
GD97HF5@@M 57H=J9 D<5G9G GI7< 5G 7@5M A=75 7<@CF=H9 5B8 =FCB CL=89
9B9F5@ F9^97H5B79 7<5F57H9F=GH=7G GI7< 5G 6F=;<HB9GG 5B8 ^5HB9GG K9F9
5@GC 7CBG=89F98 K<9B 8=GH=B;I=G<=B; @=H<C@C;=9G K=H<CIH 8=5; BCGH=7 56
GCFDH=CB :95HIF9G 9; G<5@9 5B8 A5GG=J9 GI@D<=89 1F5M 8=::F57H=CB
A=B9F5@C;M K5 G 5@GC D9F:CFA98 CB G9@97H98 G5AD@9G HC J5 @=85H9 CIF
GD97HF5@ =BH9FDF9H5H=CBG DD9B8=L 5B8 7@5F=:M H<9 A=B9F5@ 5GGC7=5
H=CBG H<5H 75IG9 H<9 C6G9FJ98 GD97HF5@ :95HIF9G
5.2. Quantitative measurem ent and feature extraction
=F97H 7CAD5 F=GCB C: GD97HF5 57 EI=F98 6M 8=: :9F9BH G9BGCFG 5B8CF =B
8=GD5F5H9 9BJ=FCBA9BHG 9; @5 6CF5HCFM JG CIH8CCFG F9A5=BG 5 G=;B=:=
75BH 7<5@@9B;9 !CK9J9F GCA9 GD97HF5@ 89F=J5H=J9G GI7< 5G GD97HF5@ =B
8=79G 9; 65B8 F5H=CG 5B8 A=B=AIA K5J9@9B;H< A5DG 5F9 F9A5F?
56@M FC6IGH HC J5F=5H=CBG =B G75@9 57EI=G=H=CB A9H<C8 5B8 =@@IA=B5H=CB
09 H5?9 58J5 BH5;9 C: H<9G9 DFC8I7HG 9; I85<M 9H 5@
,CBBH5; 9H 5@ !59GH 9H 5@ J5 B +I=H9B699? 9H 5@
!97?9F 9H 5@ J5B 89F &99F 9H 5@ 5B8 7CBGHFI7H 5 :95HIF9
G9H H<5H 75B 69 IG98 HC 8=F97H@M 7CAD5F9 GD97HF5@ 7<5F57H9F=GH=7G 69
HK99B <5 B8G5AD@9 5B8 CD9BD=H G75@9G K=H< H<9 DF=B7=D5@ 5=A C: HF5=B
=B; 5 GID9FJ=G98 7@5GG=]9F CB @569@@98 <5B8G5AD@9G 5B8 5DD@M=B; =H HC
A5D @=H<C@C;M =B H<9 <MD9F7@CI8
S.T. Thiele et al. Ore Geology Reviews xxx (xxxx) 104252
Fig. 3. C@CIF 7CADCG=H9G C: H<9 <MD9F7@CI8 7F95H98 IG=B; <M@=H9 5B8 G<CK=B ; 5 HFI97C@CIF + BA BA BA
J=GI5@=G5H=CB 5 :5@G97C@CIF J=GI5@=G5H=CB + BA BA BA <= ;<@=;< H=B; J5F=5H=CBG =B 7@ 5M 7< @CF=H9 5B8 A=75
7CBH9BH 6 5B8 H<9 ]FGH H<F99 &' 65B8 G 7 J=GI 5@=G5H=CBG C: H<9G9 85H5 75B 69 :CIB 8 5H <HHDGH=BMIF @7CA75 <MD9 F7@CI8
K=89 J5F=9HM C: GD97HF5@ =B8=79G <5J9 699B 89J9@CD98 :CF 9LHF57H
=B; ;9C@C;=75@ =B:CFA5H=CB :FCA AI@H= 5B8 <MD9FGD97HF5@ 85H5 G
H<9G9 5F9 HMD=75@@M 5DD@=98 CB F9ACH9@M G9BG98 G5H9@@=H9 85H5 H<9M 5J C=8
GD97HF5@ 65B8G G9BG=H=J9 HC 5HACGD<9F=7 9::97HG 5B8 GC 75B 69 5D D@=98 CB
6CH< CIH8CCF 5B8 @56CF5HCFM 85 H5 F6=HF5F=@M 7CAD@9L GD97HF5@ =B8=79G
75B 69 75@7I@5H98 IG=B; hylite IG=B; =B6I=@H HCC@G :CF GD97HF5@ F9G5AD@=B;
5B8 7CA6=B5H=CB CF H<FCI;< 8=F97H A5B=DI@5H=CB C: H<9 IB89F@M=B;
85H5 5FF5M IG=B; numpy !5FF=G 9H 5@ 09 9LHF57H ;9C@C;=
75@@M G9BG=H=J9 GD97HF5@ =B8=79G -56@9 :FCA H<9 7CF9G75BB9F =A5;9FM
5B8 <MD9F7@CI8 85H5 -<9G9 =B8=79G K9F9 89J9@CD98 6M I85<M 9H 5@
HC A5D H<9 ;9C@C;M C: H<9 &H "G5 F9;=CB IG=B; ,-+ 5B8 5=F
6CFB9 <MD9FGD97HF5@ 85H5 5B8 5F9 G9BG=H=J9 HC A=75 7@5M 75F6CB5H 9
5B8 =FCB CL=89 A=B9F5@G -<9 F9GI@HG =; DD9B8=L 5F9 8=F97H@M
7CAD5F56@9 69HK99B H<9 @56CF5HCFM 5B8 CIH8CCF 85H5G9HG 5B8 <=;<
@=;<H G=A=@5F=H=9G 5B8 8=::9F9B79G 69HK99B H<9 J5 F=CIG GD97HF5@
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&=B=AIAK5 J9@9B;H< &0% A5DG 5F9 5@GC 7CAACB@M 5DD@=98 HC
A5D H<9 8=GHF=6IH=CB C: GD97=]7 A=B9F5@G IG=B; <MD9FGD97HF5@ 85H5
!97?9F 9H 5@ CF 9L5AD@9 H<9 DCG=H=CB C: GD97=]7 56GCFDH=CB
:95HIF9G =B H<9 G<CFHK5J9 =B:F5F98 F9;=CB 5F9 J9FM G9BG=H=J9 HC H<9
@9B;H< C: @(! 9(! 5B8 &;(! 6CB8G =B G=@=75H9 A=B9F5@G 5@@CK=B;
577IF5H9 8=G7F=A=B5H=CB 69HK 99B 5 J5F=9HM C: 7@5M A=75 7<@CF=H9 75F
6CB5H9 5B8 5AD<=6C@9 A=B9F5@G !97?9F 9H 5@ J5 B 89F &99F 9H
5@ J5B +I=H9B699? 9H 5@ &=B=AIA K5J9@9B;H< A5DG
K9F9 75@7I@5 H98 :CF H<9 85 H5G9HG =; DD9B8=L 6M ]HH=B; H<F99
;5IGG=5B :IB7H=CBG HC 5 <I@@ 7CFF97H98 GD97HF5 :FCA HC BA
G G<CKB 6M =;G 5B8 5B8 DD9B8=L H<9 GD97HF5@ =B8=79G 5B8
&0% A5DG :CF H<9 @56CF5HC FM 5B8 CIH8CCF 85H5G9HG 5F9 EI5BH=H5 H=J9@M
7CAD5F56@9 !9B79 K9 DFCDCG9 H<5H H<9M F9DF9G9BH 5 G9H C: ;9C@C;=
75@@M F9@9J5BH :95HIF9G H<5H 5F9 5H @95GH =B H<=G 75 G9 GHI8M =BJ5F=5BH HC
G75@9 5B8 57 EI=G=H=CB A9H<C8
5.3. Automa ted ge ological mapping
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DFCJ=89 5 A9H<C8 :C F 8=F97H@M 7CAD5 F=B; GD97HF5 57EI=F98 IB89F ]9@8
5B8 @56CF5HCFM 7CB8=H=CBG -<=G CD9BG H<9 DCGG=6=@=HM C: HF5=B=B; 5 GI
D9FJ=G98 7@5GG=]9F IG=B; H<9 @=6F5FM C: 7@5GG=]98 <5B8 G5AD@9G =;
5B8 H<9B 5D D@M=B; =H HC 5IHCA5H=75@@M A5D H<9 ;9C@C;M C: H<9 CD9B
D=H "B H<9 :C @@CK=B; G97H=CB K9 9LD@CF9 H<=G CDH=CB 89J9@CD=B; 5 <5B8
H5=@CF98 897=G=CB HF99 H<5H 75B 8=GH=B;I=G< 69HK99B H<9 A5=B 5@H9F5H=CB
A=B9F5@G 5H 5B8 HF5=B=B; 5 F5B8CA :CF9GH 5@;CF=H<A H<5H 75B D9F
:CFA @=H<C@C;=75@ A5DD=B;
5.3.1. Alteration ma pping using a decision tree
,=A=@5F HC DF9J=CIG GHI8=9G =BJ9GH=;5H=B; A=B9F5@ 5@H9F5H =CB 9;
I85<M 9H 5@ @5F? 9H 5@ K9 A5DD98 H<9 8=GHF=6IH=CB C:
G9F=7=H9 5B8 7<@CF=H9 =; K<=7< 5F9 C: H9B 5GGC7=5H 98 K=H< <M
8FCH<9FA5@ 5@H9F5H=CB =B /!&, 89DCG=HG IG=B; 5 897=G=CB HF99 65 G98 CB
8=GH=B7H=J9 GD97HF5@ 7<5F57H9F=GH=7G C: 957< A=B9F5@ -<9 DF9G9B7956
G9B79 C: 8=5;BCGH=7 GD97HF5@ 56 GCFDH=CBG 5H 5B8 BA
7: )CBHI5@ 9H 5@ K5G A5DD98 IG=B; 5 89DH< 7IHC:: C: 5B 8
H<9 897=G=CB HF99 IG98 HC G9D5F5H9 ?5 C@=B=H=7 7@5M :95HIF9 5H BA
S.T. Thiele et al. Ore Geology Reviews xxx (xxxx) 104252
Fig. 4. ,D97HF5@ @=6F 5FM DF9G9BH=B ; <I@@ 7CFF97H98 A9 8=5BGD 97HF5 ;F9 9B 5B8 5GGC7=5H98 =BH9FEI5 FH=@9 5F95 ;F9M 75@7I @5H98 CB 5@@ D=L9@G C: H<9 <5B8 G5A
D@9G 7 : =;G F9D F9G9 BH=B; 957< C: H<9 GD97 HF5@ @=H<C@C;=9G =B H9FDF 9H98 5H (L=8=G98 (L A5 GG=J9 GI@D< =89 &, HKC J5F=9H=9G C: 7<@CF=H9 <@
5B8 HKC G9F=7= H=7 IB =HG ,9F 5B 8 G<5@9 5B 8 DI FD@ 9 G<5@9 ), -<9 5D DFCL=A5H9 DCG=H=CB C: 7<5F57 H9F=GH=7 56 GCFDH=CB :95HIF9G )CBHI5@ 9H 5@
5F9 5@GC D@CHH98 :CF F9:9F9B79 ,99 -56@9 :CF 89H5=@98 GD97HF5@ 89 G7F=DH=CBG
Table 1
,D97 HF5@ 89 G7 F=DH=CBG C: H<9 7< 5F57 H9F=GH=7 :95HIF9G 7: )CBHI5@ 9H 5@ %5I?5A D 9H 5@ C: 957< GD97 HF5@ @= H<C@C;M IG98 8I F=B ; GID9 FJ=G9 8 7@ 5GG=]75 H=CB
,97H=CB ,D97 HF5 :CF 957< C: H<9G9 @=H<C@C;=9G 5F9 D@CHH98 =B =;
@(! :95H IF 9 9(!
:95HIF 9
&;(!
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9]B= B; 7<5F 57 H9F= GH=7 G ,D97HF 5@ @=H< C@C; M
BA 99D =F CB 56 GCFD H=CB :95H IF9G 5B 8 GA 5@@ 8CI6 @9@(! :95H IF9 8I9 HC 5GGC7= 5H98 ?5 C@=B =H9 (L =8=G98 ( L
@5H GD 97HF5 K=H< 6FC58 K5H9F :95H IF9 5H BA &5 GG =J9 GI @D <=89
&,
OBA OBA C I6@9 56 GCFDH= CB 5H 5B 8 BA HMD=75@ C: 7<@CF= H9 @=A= H98 @(! 56 GCFDH=CB 5H BA 5B 8 @CK
=BH9BG =HM 6F C5 8 K5 H9F :95H IF9 69HK99B 5B 8 BA
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OBA OBA G K=H< < @ 6IH K= H< 899D9F K5 H9F :95HIF 9G 5F CIB8 BA @=?9@M 8I9 HC H< 9 DF9G 9B79 C: A= BCF G9F=7= H9
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8=_9F9B79 =B 89DH< C: @(! 5B 8 K5H9F :95H IF 9 7FMGH5@@= B= HM
,9F= 7=H9 ,9F
BA O BA &IG7CJ =H 9HF 5B G=H= CB=B ; HC K5F8 G D< 9B;= H9 @( ! :95H IF9 @C 75H98 5H Z 9DH< C: K5H9F :95HIF 9 F9@5 H=J9 HC
@(! :95HIF 9 GI ;; 9GHG =B7F 95G9 8 K5 H9F 7C BH9BH 7FM GH 5@ @=B= HM
,9F= 7=H9 , 9F
@5H GD 97HF5 6IH 8=GH =B7H :F CA &, 8I9 HC GA 5@ @9F B5FF CK 9F K5 H9F :95HIF 9 69HK99B 5B 8 BA BA @CK
@(! 5B8 9(! 56GCFD H=CB :95HIF9 5B8 GH99D9F G@ CD 9 69HK99B 5B 8 BA
,<5@ 9
G 56 CJ9 6IH K=H< @CK9F G@ CD9 69HK99B 5B 8 BA 5B8 G@=; <H@M 899D9F @(! :95HIF 9 )IFD@9 G<5@9 ),
K<=H9 A=75 :95HIF9 5H BA 6IH BCH BA 7<@CF=H9 :95HIF9 5H
BA 6IH BCH BA 5B8 7<@CF=H9K<=H9 A=75 A=LHIF9G :95HIF9
5H 5B8 BA 88=H=CB5@@M A=75 5B8 7<@CF=H9 7CADCG=H=CB
K5G GD@=H 65G98 CB H<9 DCG=H=CB C: H<9 BA 5B8 BA 56GCFD
H=CBG F9GD97H=J9@M 5@@CK=B; 8=G7F=A=B5H=CB C: 7CADCG=H=CB5@ 9B8A9A
69FG "AD@9A9BH5H=CB 89H5=@G C: H<=G 897=G=CB HF99 5F9 =B7@I898=B DD9B
8=L
5.3.2. Litholog y mapping using rand om fo rests
-<9 ;9C@C; M C: H<9 D=H K5 G 5@GC =BJ9GH=;5H98 IG=B; 5 F5 B8CA :CF
9GH 7@5GG=]9F =AD@9A9BH98 IG=B; ,7=?=H@95FB )98F9;CG5 9H 5@
!MD9FGD97HF5@ =A5;9G C: @569@@98 <5B8 G5AD@9G ,97H=CB K9F9 IG98
5G HF5=B=B; 85H5 5B8 H<9 F9GI@H=B; AC89@ 5DD@=98 HC A5D @=H<C@C;=9G =B
H<9 <MD9F7@CI8 C: H<9 D=H 7: DD9B8=L G 89G7F=698 =B ,97H=CB
H<9 IG9 C: FC6IGH 5B8 ;9C@C;=75@ A95B=B;:I@ :95HIF9G GI7< 5G GD97
HF5@ =B8=79G 5B8 A=B=AIA K5J9@9B;H< A5DG =G ?9M HC H<=G 5DDFC57< 5G
=H 5@@CK98 EI5BH=H5H=J9 7CAD5F=GCB 69HK99B <5B8G5AD@9 G75@9 GD97HF5
57EI=F98 =B 5 @56CF5HCFM 5B8 CIH7FCD G75@9 GD97HF5 57 EI=F98 CIH8CCFG
-<9 F5B8CA :CF9GH A9H<C8 =G 5B 9BG9A6@9 @95FB=B; 7@5GG=]9F 5 @5F;9
G9H C: 897=G=CB HF99 7@5GG=]9FG 5F9 HF5=B98 GI7< H<5H H<9=F =B8=J=8I5@ F9
GI@HG 7CA6=B9 HC ;=J9 5 7CBG9BGIG 7@5GG=]75H=CB 57< HF99 7CBHF=6IH9G 5
IB=H JCH9 5B8 H<9 ]B5@ 7@5GG=]75H=CB @569@ =G 5@@C75H98 65 G98 CB H<9
7@5GG K=H< H<9 ACGH JCH9G -<9G9 9BG9A6@9G C: HF99 7@5GG=]9FG 5F9 9L
D97H98 HC D9F:CFA ACF9 FC6IGH@M 5B8 577IF5H9@M H<5B 5B =B8=J=8I5@ 89
7=G=CB HF99 7@5GG=]9F F9=A5B
S.T. Thiele et al. Ore Geology Reviews xxx (xxxx) 104252
Table 2
,D97 HF5@ =B8=79G IG98 HC 7<5F57H9F=G9 5B8 7CAD5 F9 G5A D@9 5B8 CIH7FCD
A=B 9F5@C;M -<9 7C@CB =B 8=75H9G H<5H 5B 5J9F 5;9 F9^97 H5B7 9 K5G 75 @7I
@5H98 :CF 5@@ 65 B8 G K=H<=B H<9 GD 97=]98 F5B; 9 @ @ K5J9@9 B;H<G 5F 9 =B
B5BCA9H9FG
"B89L 9]B=H=CB
@(! FCID 7C BH9BH
@(! FCID
7CAD CG =H=C B
&;(! FCI D 7CBH 9BH
&;(! FCI D
7CAD CG =H=C B
9(! F CID 7C BH9BH
9FF CIG "F CB "B89L
9FF =7 (L =89 7CBH9BH
9FF =7 (L =8 9
7CAD CG =H=C B
$5 C@=B FCID =B 89L
(D5EI9 =B 89L
+9;C @=H< "B89L
+9;C @=H< "B89L
G K=H< A5BM A57<=B9 @95FB=B; A9H<C8G F9GI@HG C6H5=B98 IG=B;
F5B8CA :CF9GHG 75B 69 G9BG=H=J9 HC <MD9FD5F5A9H9FG H<5H 7CBHFC@ :CF 9L
5AD@9 HF99 GHFI7HIF9 5B8 89DH< G =G GH5B85F8 DF57H=79 F9=A5B
K9 D9F:CFA98 5 ]J9:C@8 7FCGG J5@=85H=CB HC CDH=A=G9 H<9G9 <M
D9FD5F5A9H9FG HCH5@ C: 7CA6=B5H=CBG C: <MD9FD5F5A9H9FG K9F9
H9GH98 IG=B; 5 :CF9GH C: HF99G -<9 F5B;9 C: <MD9FD5F5A9H9F J5@I9G
H<5H K9F9 H9GH98 5B8 H<9=F CDH=AIA J5@I9 =G GIAA5F=G98 =B -56@9
IF=B; H<9 HF5=B=B; D<5G9 H<9 7@5GG=]9F 57<=9J98 577IF57=9G C: Z
CB 6CH< HF5=B=B; 5B8 H9GH=B; GI6G9HG C: H<9 <5B8G5AD@9 =A5;9 'CH9
H<5H H<9G9 577IF57=9G 5F9 BCH F9DF9G9BH5H=J9 C: H<9 5@;CF=H<AG 5DD@=75
H=CB HC H<9 <MD9F7@CI8 85H5 5G :CF H<=G 85H5G9H H<9 ;FCIB8 HFIH< =G BCH
?BCKB
-<9 F9GI@HG C: H<9 F5B8CA :CF9GH 7@5GG=]75H=CB 5F9 GIAA5F=G98 5G
J=GI5@=G5H=CBG C: H<9 7@5GG=]98 <MD9F7@CI8 =B =; -<9 8=GHF=6IH=CB
C: @=H<C@C;=9G G<CK 9L79@@9BH GD5H=5@ 7CBG=GH9B7M 9J9B H<CI;< BC GD5
H=5@ ]@H9F=B; <5G 699B 5DD@=98 5B8 CIH@=B9 ;9C@C;=75@@M F95GCB56@9
;9CA9HF=9G H<5H ;9B9F5@@M A5H7< K=H< DF9J=CIG A5DD=B; =; 98
8=B; A95GIF9A9BHG 9LHF57H98 IG=B; H<9 CAD5GG D@I;=B =B @CI8CA
D5F9 -<=9@9 9H 5@ 5@CB; 7CBH5 7HG C: H<9 7@95F@M :C@898 G<5@9 IB=H
CIH7FCDD=B; =B H< 9 BCFH<95GH C: H<9 D=H H<9 “CFH5 H5@5M5 7CB;@CA9F
5H9” 89]B9 5 :C@8 5L=G D@IB;=B; X HCK5F8G X 5B8 5L=5@ GIF:579 8=D
D=B; 5H X HCK5 F8G X -<9G9 A95GIF9A9BHG 5F9 6FC58@M 7CBG=GH9BH
K=H< H<9 ;9B9F5@ GHFI7HIF9 C: H<9 F9;=CB5@ ;9C@C;M S9N&CBH9G 5B8
5F7S5F9GDC 5B8 5@@CK98 IG HC 89J9@CD 5B ID85H98 =BH9FDF9
H5H=CB C: H<9 GHFI7HIF9 C: =;
6. Discussion
CAD@9L ;9CA9HF=9G 5B8 =@@IA=B5H=CB 9::97HG A5?9 F9ACH9 G9BG=B;
C: 7@=::G 5B8 CD9BD=H A=B9G K=H< <MD9FGD97HF5@ =A5;=B; 5 G=;B=:=75BH
7<5@@9B;9 #5?C6 9H 5@ %CF9BN 9H 5@ -<9 KCF?^CK DF9
G9BH98 =B H<=G 7CBHF=6IH=CB 5B8 =AD@9A9BH98 =B H<9 CD9BGCIF79 hylite
DMH<CB D5 7?5;9 <9@DG 5A9@=CF5H9 H< 9G9 =GGI9G 6M DFCJ=8=B; A9H<C8G :C F
657? DFC>97H=B; 7CFF97H=B; 5B8 :IG=B; <MD9FGD97HF5@ 5B8 ;9CA9HF=7
85H5 :FCA 5 J5 F=9HM C: G9BGCFG -<9 F9GI@H=B; F9^97H5B79 GD97HF5 5F9
GHCF98 =B 5 ^9L=6@9 <MD9F7@CI8 :CFA5H GI7< H<5H 85H5 :FCA <IB8F98G C:
=B8=J=8I5@ <MD9FGD97HF5@ =A5; 9G 75B 69 =BH9;F5H 98 =BHC 5 G=B;@9 DFC8I7H
:CF J=GI5@=G5H=CB =BH9FDF9H5 H=CB 5B8 5B5@M G=G -<9 B5 HIF9 C: H< =G 5D
DFC57< A=H=;5H9G C77@IG=CB 5B8 8=GHCFH=CB =GGI9G H<5H @=A=H 5DDFC57<9G
F9@M=B; CB CFH<C;F5D<=7 DFC>97H=CB 5B8 :57=@=H5H9G 7FI7=5@ 7CFF97H=CBG
C: =@@IA=B5H=CB 5B8 5HACGD<9F=7 9::97HG =B H<9 <MD9FGD97HF5@ 85H5
-<9 75G9 GHI8M =@@IGHF5H9G H<9 DCH9BH=5@ C: H<=G 5DDFC57< 5D D@=98
HC EI5BH=H5H=J9 ;9C@C;=75@ A5DD=B; C: 5B CD9BD=H A=B9 <@CF=H=7 5B8
G9F=7=H=7 5@H9F5H =CB 5GGC7=5H 98 K=H< A=B9F5@=G5H=CB 7CI@8 69 A5DD98 IG
=B; 5 G=AD@9 897=G=CB HF99 =; K<=@9 GHF5H=;F5D<=75@@M =ADCFH5BH
<CF=NCBG GI7< 5G H<9 DIFD@9 G<5@9 K9F9 GI779GG:I@@M A5DD98 IG=B; F5B
8CA :CF9GHG =; ,=;B=:=75BH@M 6CH< A5DG 8=GH=B;I=G< GI6H@9
J5F=5H=CBG =B A=B9F5@ 7<9A=GHFM =B7@I8=B; H<9 HF5BG=H=CB HCK5 F8G AIG
7CJ=H=7 G9F=7=H9 7@CG9 HC H<9 A5GG=J9 GI@D<=89 A=B9F5@=N5H=CB 5B8 @=H<C
@C;=75@ J5 F=5H=CBG =B 7<@CF=H9 7CADCG=H=CB -<9G9 DFCJ=89 IG9:I@ 5B5
@C;I9G :CF A=B9F5@=N5H=CB J97HCFG 8IF=B; :IHIF9 9LD@CF5H=CB DFC>97HG
5B8 <=BH 5H H<9 DCH9BH=5@ :C F AI@H=G75@9 <MD9FGD97HF5@ =BJ9GH=;5H=CBG
H<5H =BH9;F5H9 85H5 :FCA F9;=CB5@ A=B9 5B8 8F=@@ 7CF9 G75@9G
-<9 7CAD@9L 6IH ;9C@C;=75@@M F95GCB56@9 ;9CA9HF=9G 89@=B95H98 6M
H<9 F5B8CA :C F9GHG A5DD=B; F9GI@H :FCA H<9 G9F=9G C: H97HC B=7 89:CFA5
H=CBG H<5H H<9 <CGH FC7?G <5J9 699B GI6>97H98 HC 5B8 DFCJ=89 =ADCFH5BH
=BG=;<H =BHC H<9 GHFI7HIF9 C: H<9 89DCG=H CF 9L5AD@9 CIF F9GI@HG 7@95F@M
G<CK H<5H H<9 7FMDH=7 “CFH5 H5@5M5 7CB;@CA9F5H9”IB=H <5G 699B
:C@898 =BHC 5B 5BH=:C FA5@ GHFI7HIF9 =; -< =G K5G A=GG98 8IF=B; DF9
Fig. 5. 5@G9 7C@CIF 7CA DCG=H9 J=GI5@=G5H=CB ;9B 9F5H98 6M A5 DD= B; H<9 @ (! 9FFCIG 5B 8 (D5EI9 =B8=79G 89]B9 8 =B -56@9 HC F98 6@I9 5B 8 ;F99B F9GD 97
H=J9@M :CF H<9 @56CF5HCFM <5B8 G5AD@ 9 G75BG 5 5B 8 <MD9F7@CI8 6 J=GI5@=G5H=CBG C: H<9G9 85H5 75B 69 :CIB 8 5H <HHDGH=BMIF @7CA75<MD9 F7 @CI8
S.T. Thiele et al. Ore Geology Reviews xxx (xxxx) 104252
Fig. 6. &=B =AI A K5 J9@9B; H< A5D C: H<9 899D 9GH 56GCFDH=CB :95HIF9 69HK99B 5B 8 BA 75@7I@5H98 6M ]HH=B; H<F9 9 ;5IGG=5B :95HIF9 G HC H<=G F5B;9
5B8 G9@97H=B; H<9 899D9G H CB9 +9GI@HG :CF <5B8 G5A D@ 9G 5 5B 8 CD 9B D=H <MD9 F7@CI8 6 G<CK 9L79@@9BH 5;F99A9 BH C@CIF F9 DF9G9BHG :95HIF9 DCG=H=CB 5B 8
6F=;<HB9GG H<9 :95HIF9 89 DH< <@CF=H=7 FC7? G K=H< 5 899D 9(! :95HIF9 5F9 <=;< @=;<H98 =B ;F99B K< =@9 A= 75 CF 7@5M F=7< @=H<C@C;=9G K=H< 5 899D @(! :95HIF9
5DD9 5F =B DI FD@9 5B8 6@I9 6 6F 9J=5H=CBG 7CFF9 GDCB8 HC H<CG9 89]B98 =B =; 5B8 -56@9 J=GI5@=G5H=CBG C: H<9G9 85H5 75B 69 :CIB8 5H <HHDGH=BMIF@
7CA 75<MD9F7 @CI8
Fig. 7. =G HF=6IH=CB C: 5@H9F5H=CB A= B9F 5@G K= H< 8=GH=B7 H=J9 5@H9F5H=CB :95HIF9 G =B H< 9 ,0"+ ;9 B9F5H98 6M D5 GG=B; H<9 AI @H=:95HIF9 A= B=AI A K5J9 @9B;H<
A5DG =; H<FCI; < 5 897=G=CB HF99 -<9 F9 GI@HG <= ;<@=;<H H<9 AIG7CJ=H=7 G9F=7=H9 5@H9F5H=CB DF CL=A5 @ HC H<9 A5GG=J9 GI@D< =89 A=B 9F5@=G5H=CB &;F=7< F9
;=CB5@ 7<@CF=H=7 5@H9F5H=CB 5B8 AC F9 9F=7< 7< @CF=H9G 5GGC7= 5H98 K=H< 5@H9F5H=CB 5@CB; :5I@HG 5B8 K=H<=B H<9 GHC7?KCF? NCB9 C: H<9 89DCG=H A=75 5B8 7@ 5M
F=7< NCB9 B9 5F H<9 GIF:579 =G 5@GC 9J=89BH K<=7 < K9 =B H9FDF 9H HC F9GI@H :FCA F979BH K9 5H<9F=B; -<=G A5D 75B 69 J=9K98 =B 5H <HHDG H=BMIF @7CA
75<MD9F7 @CI8
J=CIG A5DD=B; 75AD5=;BG 9; S9N&CBH9G 5B8 5F7S5F9GDC
DF9GIA56@M 8I9 HC H<9 8=:]7I@H=9G 8=GH=B;I=G<=B; H<=G @=H<C@C;M
5B8 5779GG=B; H<9 F9@9J5BH CIH7FCDG -<9 <MD9F7@CI8 A5DD=B; F9GI@HG
5B8 5GGC7=5H98 GHFI7HIF5@ A95GIF9A9BHG =;G 5B8 <5J9 H<IG 5@
S.T. Thiele et al. Ore Geology Reviews xxx (xxxx) 104252
Table 3
!MD9FD5 F5A9 H9F J5@I9 G H9GH98 8I F=B; <MD9 FD5F5A9 H9F CDH=A= G5H=CB 5B 8
H<9=F 7CFF9GDCB8=B ; J5@I9G CF 5 89H5=@98 89G7 F=D H=CB C: 957< <MD9FD5F5
A9H9F D@95G9 F9:9F HC H<9 G7=?=H @95FB 8C7 IA9 BH5H=CB
!M D9FD 5A 9H9F -9GH98 F5 B; 9 (DH= AIA J5 @I 9
&5 L= AIA :95H IF9G D9F HF 99 –
&5 L= AIA HF 99 89DH< –
&=B= AI A G5 AD @9G GD @=H –
&=B= AI A G5 AD @9G @95: –
CCHGH F5 D -FI9 5 @G9 -FI9
@CK98 IG HC 7CA9 ID K=H< 5 F9J=G98 GHFI7HIF5@ =BH9FDF9H5H=CB C: =;
:IFH<9F <=;<@=;<H=B; H<9 J5@I9 C: CIF 5DDFC57< LD@CF5H=CB ;9C@C
;=GHG 5H <5J9 G=B79 J5@=85H98 5GD97HG C: H<=G GD97HF5@ =BH9FDF9H5H=CB
H<FCI;< H5 F;9H98 ]9@8 A5DD=B; C: H<9 DIFD@9 G<5@9 IB=H 5B8 :C@898
7CB;@CA9F5H9
-<9 + F9GI@HG 5@GC <=;<@=;<H GCA9 7<5@@9B;9G H<5H 7CI@8 69 58
8F9GG98 =B :IHIF9 GHI8=9G =FGH@M 5 7CAD5F=GCB C: H<9 7@5GG=]75H=CB F9
GI@HG K=H< H<9 ;9C@C;M A5D C: S9N&CBH9G 5B8 5 F7S5F9GDC
GI;;9GHG H<5H H<9 F5B8CA :C F9GH 7@5GG=]9F =G BCH 56@9 HC 577IF5H9@M 8=G
H=B;I=G< 69HK99B 6@57? G<5@9G 5B8 A5GG=J9 GI@D<=89G -<=G =G IBGIFDF=G
=B; 5G 6CH< IB=HG 5F9 7<5F57H9F=G98 6M ^5H 5B8 ;9B9F5@@M @CK
F9^97H5B79 GD97HF5 =B H<9 /'"+ 5B8 ,0"+ !CK9J9F =H =G DCGG=6@9 H<5H
H<9G9 IB=HG 7CI@8 69 GI779GG:I@@M 8=GH=B;I=G<98 IG=B; :95HIF9G H<5H <=;<
@=;<H GI6H@9 8=::9F9B79G =B H<9 J=G=6@9 5B8 /'"+ D5 FHG C: H<9 GD97HFIA 7:
=; CF 6M 75DHIF=B; 5B8 =BH9;F5H =B; @CB;K5 J9 =B:F5F98 =A5;9FM
H<5H 75 B 69HH9F 8=G7F=A=B5H9 G=@=75H9 A=B9F5@G 5GGC7=5H98 K=H< H<9 A=B9F
5@=N5H=CB 9; EI5FHN
,97CB8@M K9 5@GC =BH9FDF9H H<5H H<9 ,9F=7=H9 IB=H 5GGC7=5H98 K=H<
CL=8=G98 5B8 K95H <9F98 A5H9F=5@ 5@CB; H<9 BCFH<9FB F=A C: H<9 D=H F9
GI@HG :FCA GID9F;9B9 7@5M A=B9F5@G :CFA=B; =B K95H <9F98 7<@CF=H9 JC@
75B=7G .B:CFHIB5H9@M <5B8G5AD@9G :FCA H<9G9 @C75H=CBG 7CI@8 BCH 69
Fig. 8. &5D 5 7F CGGG97H=CB 6 5B8 @CB;G97H=CB 7 J=9KG C: H<9 + 7@5GG=]75H=CB -<9 <5 B8 G5AD @9G IG98 HC HF5=B H<9 + 5F9 CJ9F@5=B =B 5 IG=B ; 5DDF CL=
A5H9 @C75H=CBG A95GIF98 K=H< 5 <5B8<9 @8 ), 5B8 7C@CIF98 6M H<9=F @569 @ 7 : -56@9 ,5A D@9G G9@97H98 :CF 1+ 5B5@MG9G DD9B8=L 5F9 5@GC <=;<
@=;<H98 J=GI 5@=G5H=CBG C: H<=G 7@5GG=]75H=CB 75 B 69 :CIB8 5H <HHDGH=BMIF@ 7CA 75<MD9F7 @CI8
Fig. 9. ,7<9 A5H=7 GHFI7HIF5@ 7FCGG G97H=CB C: H<9 CFH5 H5@5M5 CD9B D=H 65G98 CB 5B =B H9FDF 9H5H=CB C: H<9 <MD9FGD97 HF5@ A5DD= B; F9GI @HG 5B8 GHFI 7HIF5@ A95
GIF9A9BHG 9LHF57H98 :FCA H<9 <MD9 F7@CI8 .B =HG 5F9 @569 @@98 57 7CF8=B; HC =;G 5B8 5B 8 8F 5D98 CB H<9 &' J=GI5@=G5H=CB DF9G9BH98 =B =; 9 8
8=B; A9 5GI F9A9 BHG 9LHF57H98 65 G98 CB H<9G9 A5DD= B; F9GI @HG 5B8 H<9 HCDC;F5D< M 5F9 CJ9F@5=B CB 5 5B 8 D@ CHH98 CB 5 @CK9F <9 A=GD<9 F9 9EI5@5F95
GH9F9C;F5D <=7 DFC>97H=CB 6 IG=B; ,H9F9CB9H @ @A9B8= B;9F CBHCIFG =B 6 K9F9 75@7I@5H98 IG =B; H<9 $5A6 A9 H<C8 @ @A9B8= B;9F 9H 5@
5B8 IG 98 HC 89]B9 H<9 5J9F5;9 CF=9BH5H=CB C: 957< :C@8 @=A6 5B8 <9 B7 9 9GH=A5 H9 H<9 CF=9BH5H=CB C: H<9 :C@8’G 5L=5@ D@5B 9
S.T. Thiele et al. Ore Geology Reviews xxx (xxxx) 104252
F9HF=9J98 8I9 HC 5779GG @=A=H5H=CBG 5B8 GC K9F9 BCH =B7@I898 =B CIF
HF5=B=B; 85H5G9H "H =G @=?9@M H<5H =: G5AD@9G 7CI@8 69 F9HF=9J98 H<9B H<=G
GID9F;9B9 NCB9 7CI@8 69 A5DD98 5G 5 8=GH=B7H @=H<C@C;M 6M H<9 + ,=A=
@5F@M 7<@CF=H=7 G<5@9G CIH7FCDD=B; 5@CB; H<9 GCIH<9FB A5F;=B C: H<9 D=H
7CI@8 BCH 69 8=GH=B;I=G<98 :FCA 7<@CF=H=G98 JC@75B=7G =B H<9 BCFH< 8I9 HC
5 @57? C: G5AD@9G :FCA H<=G IB=H =B H<9 HF5=B=B; 85H5G9H 7: =;
9GD=H9 H<9G9 @=A=H5H=CBG CIF F9GI@HG 5F9 5 7@95F 89ACBGHF5H=CB H<5H
K=H< 589EI5H9 7CFF97H=CBG 5B8 75F9:I@ :95 HIF9 G9@97H=CB <MD9FGD97HF5@
=B:CFA5H=CB 75B 69 EI5BH=H5H=J9@M 7CAD5F98 69HK99B @56CF5HCFM 5B8
CIH7FCD G75@ 9G J9B H<CI;< H<9 F5 B8CA :CF9GH 7@5GG=]9F K5 G HF5=B98 9L
7@IG=J9@M CB @56CF5HCFM57EI=F98 GD97HF5@ =A5;9FM C: =B8=J=8I5@ <5B8
G5AD@9G =H K5G 56@9 HC GI779GG:I@@M 7@5GG=:M H<9 <MD9F7@CI8 5B8 9L
HF57H A95B=B;:I@ ;9C@C; =75@ =B:CFA5H=CB -<=G 5DDFC5 7< <5G G=;B=:=75BH
DF57H=75@ 58J5BH5;9G CJ9F HF58=H=CB5@ A9H<C8G 6975IG9 H<9 B998 :CF
GI6>97H=J9 @56CIF=BH9BG=J9 5B8 DCH9BH=5@@M IBG5:9 ]9@8A5DD=B; HC
7F95H9 HF5=B=B; @569@G =G F98I798
-<=G 5DDFC57< =G A589 DCGG=6@9 6M H<9 =BH=A5H9 =BH9;F5H=CB C: ;9C
A9HF=7 5B8 GD97HF5@ 85H5 J=5 5 <MD9F7@CI8 )F9J=CIG GH5H 9C:H<95FH 5D
DFC57<9G 9; $FIDB=? 5B8 $<5B 5F9 @=A=H98 6M 7CB:C IB8=B; 5H
ACGD<9F=7 5B8 =@@IA=B5H=CB 9::97HG K<=7< F98I79 H<9 577IF57M C: 5IHC
A5H=7 A5DD=B; A9H<C8G -<9 =BH9;F5H=CB C: <=;<F9GC@IH=CB ;9CA9HFM
=BHC H<9 GD97HF5@ DFC79GG=B; KCF?^CK 5@@CKG G=;B=:=75BH@M 69HH9F 7CF
F97H=CB C: H<9G9 9::97H G 5B8 H<IG ACF9 57 7IF5H9 GD97HF5@ 89F=J5 H=J9G 5B8
7@5GG=]75H=CBG )F9J=CIG A9H<C8G :CF 7CF9;=GH9F=B; ;9CA9HFM K=H<
GD97HF5@ 85H5 9; #5?C6 9H 5@ <5J9 699B @=A=H98 6M =B577IF5H9
5B8 @56CF=CIG A9H<C8G :CF 9GH=A5H=B; H<9 DCG=H=CB 5B8 CF=9BH5H=CB C:
H<9 <MD9FGD97HF5@ G9BGCF -<9 )B) GC@IH=CB =AD@9A9BH98 =B hylite 7=F
7IAJ9BHG H<9G9 =GGI9G 5B8 5@ @CKG A5BM 8=::9F9BH <MD9FGD97HF5@ 85 H5G9HG
HC 69 657?DFC>97H98 5B8 :IG98 =BHC 5 <MD9F7@CI8 -<9 J5 @I9 C: H<9G9
85H5 =G :I FH<9F 9B<5B798 6M H<9 5GGC7=5H98 <=;< F9GC@IH=CB ;9CA9HFM 5G
H<=G =B:C FA5H=CB =G 7F=H=75@ :CF =BH9FDF9H=B; H<9 ;9CA9HFM C: ;9C @C;=
75@ 6C8=9G -<=G =G 9L9AD@=]98 6M CIF 56 =@=HM HC A5D :C @898 IB=HG 5H
J=GI5@=G9 H<9 F9GI@HG =B 5B8 9LHF57H GHFI7HIF5@ A95GIF9A9BHG H<5H
7CBGHF5=B H<9 :C @8’G 5L =5@ D@5B9 =;
=B5@@M CIF F9GI@HG 5@GC GI;;9GH H<5H GCA9 <MD9FGD97HF5@ 89F=J5H=J9G
9; A=B=AIA K5J9@9B;H< A5DG 5B8 65B8 F5H=CG 5F9 F9@5H=J9@M G75@9
=BJ5F=5BH :C F DFCD9F@M 7CFF97H98 85H5G9HG -<=G F5=G9G H<9 =BH9F9GH=B;
DCGG=6=@=HM H<5H &% 5@;CF=H<AG HF5=B98 CB @=6F5F=9G C: <5B8G5AD@9G
7CI@8 5=8 A5DD=B; 57 H=J=H=9G 5H @5F;9F G75@9G 5B8 697CA9 “8=;=H5@ ;9C@C
;=GHG”H<5H 5GG=GH =BH9FDF9H5H=CB 9::CFHG 6M C6>97H=J9@M 7CBJ9FH=B; !,"
85H5 :FCA 8F=@@ 7CF9 CIH7FCD A=B9:5 79 5B8 5=F6CFB9 75AD5=;BG =BHC
@=H<C@C;=75@ A5 DG 5B8 @C;G -<=G KCI@8 DFCJ=89 5 IB=]98 5D DFC57< H<5H
5A9@=CF5H9G =GGI9G K=H< =B7CBG=GH9BH @C;;=B; 5B8 A5DD=B; K<=7< 7CA
ACB@M D@5;I9 A=B9F5@G 9LD@CF5H=CB 5B8 =B 8C=B; GC :5 7=@=H5H9 9::CFHG HC
GMBH<9G=G9 5B8 <CAC;9B=N9 F9;=CB5@ 85H5 G9HG "H 5@GC DFCJ=89G 5 A97<5
B=GA :CF ;9B9F5H=B; H<9 @5 F;9 5B8 FC6IGH HF5=B=B; 85H5 G9HG H<5H 5F 9 7F=H=
75@ :CF H<9 GI779GG:I@ 5DD@=75H=CB C: AC89FB A57<=B9 @95FB=B; A9H<C8G
7. Conclusion
-<9 CD9BGCIF79 hylite D57?5; 9 DFCJ=89G 5 IB=:CFA KCF?^CK :C F
:IG=B; F5K <MD9FGD97HF5@ 85 H5 :FCA AI@H=D@9 G9BGCFG 5B8 57EI=G=H=CB
;9CA9HF=9G =BHC F58=CA9HF=75@@M 5B8 ;9CA9HF=75@@M 7CFF97H98 <MD9F
7@CI8G -<9 D57?5;9 75 B H<9B 69 IG98 HC 89F=J9 ;9C@C;=75@@M F9@9J5BH
85H5 DFC8I7HG GI7< 5G A=B=AIA K5J9@9B;H< A5DG 65B8 F5H=CG 5B8
GD97HF5@ 7@5GG=]75H=CBG -C 89ACBGHF5H9 H<=G K9 IG98 hylite HC 7CA6=B9
;FCIB865G98 5B8 ./6CFB9 <MD9FGD97HF5@ =A5;9G =BHC 5 G=B
;@9 F9^97H5B79 <MD9F7@CI8 -<=G K5G IG98 HC A5D @=H<C@C;M 5B8 5@H9F
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Decl aration of Competing Interest
-<9 5IH<CFG 897@5F9 H<5H H<9M <5J9 BC ?BCK B 7CAD9H=B; ]B5B7=5@
=BH9F9GHG CF D9FGCB5@ F9@5H=CBG<=DG H<5H 7CI@8 <5J9 5DD95F98 HC =B^I
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Acknowledgem ents
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Append ix A. Suppleme ntary data
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