Article

Modelling the Spatio-Temporal Distribution of Ambient Nitrogen Dioxide and Investigating the Effects of Public Transit Policies on Population Exposure

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Abstract

Estimating the future state of air quality associated with transport policies and infrastructure investments is key to the development of meaningful transportation and planning decisions. This paper describes the design of an integrated transportation and air quality modelling framework capable of simulating traffic emissions and air pollution at a refined spatio-temporal scale. For this purpose, emissions of Nitrogen Oxides (NOx) were estimated in the Greater Montreal Region at the level of individual trips and vehicles. In turn, hourly Nitrogen Dioxide (NO2) concentrations were simulated across different seasons and validated against observations. Our validation results reveal a reasonable performance of the modelling chain. The modelling system was used to evaluate the impact of an extensive regional transit improvement strategy revealing reductions in NO2 concentrations across the territory by about 3.6% compared to the base case in addition to a decrease in the frequency and severity of NO2 hot spots. This is associated with a reduction in total NOx emissions of 1.9% compared to the base case; some roads experienced reductions by more than half. Finally, a methodology for assessing individuals’ daily exposure is developed (by tracking activity locations and trajectories) and we observed a reduction of 20.8% in daily exposures compared to the base case. The large difference between reductions in the mean NO2 concentration across the study domain and the mean NO2 exposure across the sample population results from the fact that NO2 concentrations dropped largely in the areas which attract the most individuals. This exercise illustrates that evaluating the air quality impacts of transportation scenarios by solely quantifying reductions in air pollution concentrations across the study domain would lead to an underestimation of the potential health gains.

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... In the common industrial practice, air quality studies are usually carried out by employing large scale models (Bezyk et al., 2021;Isakov et al., 2017;Shekarrizfard et al., 2017), which can predict pollutants dispersion in large areas where environmental impact assessment should be performed. However, these models can have accuracy issues when dealing with the assessment of dispersion in the local scale of urban districts. ...
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The use of Computational Fluid Dynamics (CFD) for environmental studies is continuously growing. In this context, simulations are usually carried out solving Reynolds-averaged Navier–Stokes (RANS) equations that require an appropriate implementation of the Atmospheric Boundary Layer (ABL). This paper proposes a framework based on the Shear Stress Transport (SST) k−ω turbulence model, which is highly recommended for microclimate analysis, since it is known to well reproduce homogeneous ABL flows in the context of RANS simulations. Besides, a new blending approach is developed to account for the presence of obstacles in the domain. The model is implemented in the open-source OpenFOAM code and validated against well-known benchmark cases spanning different configurations, i.e., an empty fetch, a single building and an array of buildings. The performance of the proposed model is very satisfactory. For instance, the Factor-of-2 validation metric is FAC2>0.8 for both velocity and turbulent kinetic energy in nearly all cases.
... In the common industrial practice, air quality studies are usually carried out by employing large scale models (Bezyk et al., 2021;Isakov et al., 2017;Shekarrizfard et al., 2017), which can predict pollutants dispersion in large areas where environmental impact assessment should be performed. 10 However, these models can have accuracy issues when dealing with the assessment of dispersion in the local scale of urban districts, since they are characterized by a low level of turbulence treatment. ...
... Concerns over population exposure to air pollution have grown with an increasing number of health studies reporting links between combustion-related air pollutants and adverse health effects (Sevik et al., 2020;Tobías et al., 2018;Vette et al., 2013;Weichenthal, 2012). Near-road air quality, especially pollutants such as ultrafine particles (UFP) and black carbon (BC), varies significantly over small distances and short periods in urban environments (Parvez & Wagstrom, 2019;Shekarrizfard et al., 2017;Wang et al., 2016;Weichenthal et al., 2014;. Mobile measurements of air pollution using high-time-resolution portable instruments on mobile platforms have gained popularity in recent years due to their ability to characterize the spatiotemporal variability of nearroad air quality in urban areas (W. ...
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... Ewing and Cevero (2010) performed a meta analysis of studies on travel and the built environment with the primary objective of providing planners with data in the form of elasticities that could be used to estimate the effects of built environment factors on mode choice and travel demand. Most recently, Shekarrizfard et al. (2017) designed an integrated transportation and air quality modeling framework capable of simulating traffic emissions and air pollution at a refined spatio-temporal scale. This complex modeling system was used to evaluate the impact of an extensive regional transit improvement strategy revealing reductions in NO 2 concentrations across the territory by about 3.6% compared to the base case in addition to a decrease in the frequency and severity of NO 2 hot spots. ...
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... The most common approach is to consider home location as a proxy of population location [19][20][21][22][23][24] and constitutes the basis for most air quality health impact assessment studies [25,26]. However, several studies have reported important discrepancies between personal exposure and exposure at residence [27][28][29]. It has been demonstrated that travel behavior significantly influences on exposure to air pollution [30][31][32][33]. ...
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... Although transport has been identified as one of the key sectors for a long time (Colvile et al., 2001) most of air quality exceedances in Europe are still related to road traffic (EEA, 2017). Traffic-related policies have been shown particularly relevant for NO 2 exposure (Shekarrizfard et al., 2017) since this is the main contributor to ambient air levels in many urban areas worldwide including Madrid (Spain). According to Borge et al. (2014), road traffic is responsible for up to 90% of NO 2 concentration levels in the city centre. ...
... Although transport has been identified as one of the key sectors for a long time (Colvile et al., 2001) most of air quality exceedances in Europe are still related to road traffic (EEA, 2017). Traffic-related policies have been shown particularly relevant for NO 2 exposure (Shekarrizfard et al., 2017) since this is the main contributor to ambient air levels in many urban areas worldwide including Madrid (Spain). According to Borge et al. (2014), road traffic is responsible for up to 90% of NO 2 concentration levels in the city centre. ...
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Air pollution continues to be one of the main issues in urban areas. In addition to air quality plans and emission abatement policies, additional measures for high pollution episodes are needed to avoid exceedances of hourly limit values under unfavourable meteorological conditions such as the Madrid's short-term action NO2 protocol. In December 2016 there was a strong atmospheric stability episode that turned out in generalized high NO2 levels, causing the stage 3 of the NO2 protocol to be triggered for the first time in Madrid (29th December). In addition to other traffic-related measures, this involves access restrictions to the city centre (50% to private cars). We simulated the episode with and without measures under a multi-scale modelling approach. A 1 km2 resolution modelling system based on WRF-SMOKE-CMAQ was applied to assess city-wide effects while the Star-CCM+ (RANS CFD model) was used to investigate the effect at street level in a microscale domain in the city centre, focusing on Gran Vía Avenue. Changes in road traffic were simulated with the mesoscale VISUM model, incorporating real flux measurements during those days. The corresponding simulations suggest that the application of the protocol during this particular episode may have prevented concentrations to increase by 24 μg·m-3 (14% respect to the hypothetical no action scenario) downtown although it may have cause NO2 to slightly increase in the city outskirts due to traffic redistribution. Speed limitation and parking restrictions alone (stages 1 and 2 respectively) have a very limited effect. The microscale simulation provides consistent results but shows an important variability at street level, with reduction above 100 μg·m-3 in some spots inside Gran Vía. Although further research is needed, these results point out the need to implement short-term action plans and to apply a consistent multi-scale modelling assessment to optimize urban air quality abatement strategies.
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Near-road exposures of traffic-related air pollutants have been receiving increased attention due to evidence linking emissions from high-traffic roadways to adverse health outcomes. To date, most epidemiological and risk analyses have utilized simple but crude exposure indicators, most typically proximity measures, such as the distance between freeways and residences, to represent air quality impacts from traffic. This paper derives and analyzes a simplified microscale simulation model designed to predict short- (hourly) to long-term (annual average) pollutant concentrations near roads. Sensitivity analyses and case studies are used to highlight issues in predicting near-road exposures. Process-based simulation models using a computationally efficient reduced-form response surface structure and a minimum number of inputs integrate the major determinants of air pollution exposures: traffic volume and vehicle emissions, meteorology, and receptor location. We identify the most influential variables and then derive a set of multiplicative submodels that match predictions from "parent" models MOBILE6.2 and CALINE4. The assembled model is applied to two case studies in the Detroit, Michigan area. The first predicts carbon monoxide (CO) concentrations at a monitoring site near a freeway. The second predicts CO and PM2.5 concentrations in a dense receptor grid over a 1 km2 area around the intersection of two major roads. We analyze the spatial and temporal patterns of pollutant concentration predictions. Predicted CO concentrations showed reasonable agreement with annual average and 24-hour measurements, e.g., 59% of the 24-hr predictions were within a factor of two of observations in the warmer months when CO emissions are more consistent. The highest concentrations of both CO and PM(2.5) were predicted to occur near intersections and downwind of major roads during periods of unfavorable meteorology (e.g., low wind speeds) and high emissions (e.g., weekday rush hour). The spatial and temporal variation among predicted concentrations was significant, and resulted in unusual distributional and correlation characteristics, including strong negative correlation for receptors on opposite sides of a road and the highest short-term concentrations on the "upwind" side of the road. The case study findings can likely be generalized to many other locations, and they have important implications for epidemiological and other studies. The reduced-form model is intended for exposure assessment, risk assessment, epidemiological, geographical information systems, and other applications.
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The development and use of dispersion models that simulate traffic-related air pollution in urban areas has risen significantly in support of air pollution exposure research. In order to accurately estimate population exposure, it is important to generate concentration surfaces that take into account near-road concentrations as well as the transport of pollutants throughout an urban region. In this paper, an integrated modelling chain was developed to simulate ambient Nitrogen Dioxide (NO2) in a dense urban neighbourhood while taking into account traffic emissions, the regional background, and the transport of pollutants within the urban canopy. For this purpose, we developed a hybrid configuration including 1) a street canyon model, which simulates pollutant transfer along streets and intersections, taking into account the geometry of buildings and other obstacles, and 2) a Gaussian puff model, which resolves the transport of contaminants at the top of the urban canopy and accounts for regional meteorology. Each dispersion model was validated against measured concentrations and compared against the hybrid configuration. Our results demonstrate that the hybrid approach significantly improves the output of each model on its own. An underestimation appears clearly for the Gaussian model and street-canyon model compared to observed data. This is due to ignoring the building effect by the Gaussian model and undermining the contribution of other roads by the canyon model. The hybrid approach reduced the RMSE (of observed vs. predicted concentrations) by 16%–25% compared to each model on its own, and increased FAC2 (fraction of predictions within a factor of two of the observations) by 10%–34%.
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This research is motivated by the need to improve transportation policy analysis through the development of a holistic framework to evaluate transportation externalities. Traditionally, transportation planning has been focused primarily on the improvement of transportation infrastructure and network performance and little attention has been paid to the resulting externalities that negatively impact public health. The paper presents a holistic analysis framework that enables policy makers analyze the chain effect of transportation demand on air quality and population health exposure. Holism is achieved by incorporating the interactions between transportation demand, network performance measurement, vehicular emissions, air quality modeling and population exposure assessment. The eventual impact of vehicular emissions on population is measured through the use of an intake fraction metric, which measures the fraction of pollutant inhaled by an exposed population over a defined period of time. The proposed framework takes advantage of the existing state-of-the-art domain specific models so there is no need to re-invent the wheels. Instead, the focus of the this research is to provide a prescriptive process of addressing data gaps and resolution matching between these models as well as other models alike. The proposed population exposure assessment incorporates key parameters including different microenvironments and inhalation rates not accounted for in the existing literature of exposure assessment. The entire framework is evaluated with the three city sub-region of Maricopa County in Arizona. Further investigations demonstrate the importance of differentiating microenvironments and inhalation rates to properly capturing population exposure.
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A dynamic city-wide air pollution exposure assessment study has been carried out for the urban population of Rome, Italy, by using time resolved population distribution maps, derived by mobile phone traffic data, and modelled air pollutants (NO2, O3 and PM2.5) concentrations obtained by an integrated air dispersion modeling system. More than a million of persons were tracked during two months (March and April 2015) for their position within the city and its surroundings areas, with a time resolution of 15 minutes and mapped over an irregular grid system with a minimum resolution of 0.26x0.34 Km2. In addition, demographics information (as gender and age ranges) were available in a separated dataset not connected with the total population one. Such BigData were matched in time and space with air pollution model results and then used to produce hourly and daily resolved cumulative population exposures during the studied period. A significant mobility of population was identified with higher population densities in downtown areas during daytime increasing of up to 1000 people/Km2 with respect to nigh-time one, likely produced by commuters, tourists and working age population. Strong variability (up to ±50% for NO2) of population exposures were detected as an effect of both mobility and time/spatial changing in pollutants concentrations. A comparison with the correspondent stationary approach based on National Census data, allows detecting the inability of latter in estimating the actual variability of population exposure. Significant underestimations of the amount of population exposed to daily PM2.5 WHO guideline was identified for the Census approach. Very small differences (up to a few μg/m3) on exposure were detected for gender and age ranges population classes.
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Advances in micro-sensor technologies for air pollution monitoring encourage a growing use of portable sensors. This study aims at testing their performance in the development of exposure surfaces for nitrogen dioxide (NO2) and ozone (O3). In Montreal, Canada, a data collection campaign was conducted across three seasons in 2014, for 76 sites spanning the range of land-uses and built environments of the city; each site was visited 6 to 12 times, for 20 minutes, using NO2 and O3 sensors manufactured by Aeroqual. Land use regression models were developed achieving R(2) values of 0.86 for NO2 and 0.92 for O3, when adjusted for regional meteorology - to control for the fact that all the locations were not monitored at the same time. Two exposure surfaces were then developed for NO2 and O3 - as averages over spring, summer and fall. Validation against fixed station data and previous campaigns suggests that Aeroqual sensors tend to overestimate the highest NO2 and O3 concentrations thus increasing the range of values across the city. However, the sensors suggest a good performance with respect to capturing the spatial variability in NO2 and O3 and are very convenient to use, with great potential for capturing temporal variability.
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Microsimulation is becoming more popular in transportation research. This research explores the potential of microsimulation by integrating an existing activity-based travel demand model, TASHA, with a dynamic agent-based traffic simulation model, MATSim. Differences in model precisions from the two models are resolved through a series of data conversions, and the models are able to form an iterative process similar to previous modeling frameworks using TASHA and static assignment using Emme/2. The resulting model is then used for light-duty vehicle emission modeling where the traditional average-speed modeling approach is improved by exploiting agent-based traffic simulation results. This improved method of emission modeling is more sensitive to the effect of congestion, and the linkage between individual vehicles and link emissions is preserved. The results have demonstrated the advantages of the microsimulation approach over conventional methodologies that rely heavily on temporal or spatial aggregation. The framework can be improved by further enhancing the sensitivity of TASHA to travel time.
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Exposure to fine particulate matter from vehicle exhaust is associated with increased health risk. This study develops a new approach for creating spatially detailed regional maps of fine particulate matter concentration from vehicle exhaust using a dispersion model to better evaluate these risks. The spatial extent, diurnal, and seasonal patterns of concentration fields across Los Angeles County, California are evaluated and population exposure and exposure equity by race and income are investigated. The results demonstrate how this modeling approach can create new knowledge about vehicle emissions exposure. This approach also provides a method for proactively screening out regional plans, or specific projects within these plans, that are likely to cause air quality concerns. A proactive and regional air quality assessment can identify potential problems earlier in the planning process and a wider range of solutions, saving time, money and protecting public health. The detailed concentration maps can also be used to improve the siting of regulatory air quality monitors and provide more accurate exposure data for epidemiology studies.
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Modelling approaches for simulating air and stormwater pollution due to on-road vehicles are reviewed and discussed. Models for traffic, emissions, atmospheric dispersion, and stormwater contamination are studied with particular emphasis on their couplings to create a modelling chain. The models must be carefully selected according to the requirements and level of detail of the integrated modelling chain. Although a fair amount of research has been conducted to link air pollution and road traffic, many questions related to spatio-temporal scales, domains of validity, consistency among models, uncertainties of model simulation results, and interfaces between models remain open. The aim of this work is to review the current status of the relationships between traffic, emissions, air quality, and water quality models, to recommend modelling approaches and to propose some directions for improving the state of the science. The difficulties and challenges associated with model coupling are illustrated with specific examples.
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In developed countries such as Canada and United States, a significant number of individuals depend on automobile as their main mode of transport. There has been a stronger push towards analyzing travel behavior at the individual level so that transportation agencies can formulate appropriate strategies to reduce the auto dependency. Towards this pursuit of enhancing our understanding on travel behavior, we examine individual home to work/school commute patterns in Montreal, Canada with an emphasis on the transit mode of travel. The overarching theme of this paper is to examine the effect of the performance of the public transportation system on commuter travel mode and transit route choice (for transit riders) in Montreal. We investigate two specific aspects of commute mode choice: (1) the factors that dissuade individuals from commuting by public transit and (2) the attributes that influence transit route choice decisions (for those individuals who commute by public transit). This study employs a unique survey conducted by researchers as part of the McGill University Sustainability project. The survey collected information on commute patterns of students, faculty and staff from McGill University. In addition, detailed socio-demographic and residential location information was also collected. The analysis was undertaken using multinomial logit model for the travel mode choice component and a mixed multinomial logit model for the transit route choice component. The model estimation results were employed to conduct policy sensitivity analysis that allows us to provide recommendations to public transportation and metropolitan agencies.
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There is often a large discrepancy between the questions raised by policy makers and the responses offered by scientists. Current modeling approaches do not answer some of the typical questions that decision-makers face, as they do not provide solutions to policy-makers dealing with concrete political negotiation and decisions. In this paper, we try to bridge the gap by creating an integrated model chain that can respond to such concrete policy questions. The paper describes a model chain consisting of an activity-based transport model, a road traffic emission model, a bi-gaussian atmospheric dispersion model and a concentration measurement interpolation model. Subsequently results are compared to observations, in order to test its usability for simulating air quality and assessing dynamic exposure. The model is shown to represent the main cycles governing air quality, such as the intra-daily, the intra-weekly and the intra-annual cycle. Finally, this paper provides an example of the use of such a model chain by assessing the impact of different trip motives on the intra-daily NO2 cycle.
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Objectives: We quantified health benefits of transportation strategies to reduce greenhouse gas emissions (GHGE). Methods: Statistics on travel patterns and injuries, physical activity, fine particulate matter, and GHGE in the San Francisco Bay Area, California, were input to a model that calculated the health impacts of walking and bicycling short distances usually traveled by car or driving low-emission automobiles. We measured the change in disease burden in disability-adjusted life years (DALYs) based on dose-response relationships and the distributions of physical activity, particulate matter, and traffic injuries. Results: Increasing median daily walking and bicycling from 4 to 22 minutes reduced the burden of cardiovascular disease and diabetes by 14% (32,466 DALYs), increased the traffic injury burden by 39% (5907 DALYS), and decreased GHGE by 14%. Low-carbon driving reduced GHGE by 33.5% and cardiorespiratory disease burden by less than 1%. Conclusions: Increased physical activity associated with active transport could generate a large net improvement in population health. Measures would be needed to minimize pedestrian and bicyclist injuries. Together, active transport and low-carbon driving could achieve GHGE reductions sufficient for California to meet legislative mandates.
Article
Transportation policy measures often aim to change travel behaviour towards more efficient transport. While these policy measures do not necessarily target health, these could have an indirect health effect. We evaluate the health impact of a policy resulting in an increase of car fuel prices by 20% on active travel, outdoor air pollution and risk of road traffic injury. An integrated modelling chain is proposed to evaluate the health impact of this policy measure. An activity-based transport model estimated movements of people, providing whereabouts and travelling kilometres. An emission- and dispersion model provided air quality levels (elemental carbon) and a road safety model provided the number of fatal and non-fatal traffic victims. We used kilometres travelled while walking or cycling to estimate the time in active travel. Differences in health effects between the current and fuel price scenario were expressed in Disability Adjusted Life Years (DALY). A 20% fuel price increase leads to an overall gain of 1650 (1010–2330) DALY. Prevented deaths lead to a total of 1450 (890–2040) Years Life Gained (YLG), with better air quality accounting for 530 (180–880) YLG, fewer road traffic injuries for 750 (590–910) YLG and active travel for 170 (120–250) YLG. Concerning morbidity, mostly road safety led to 200 (120–290) fewer Years Lived with Disability (YLD), while air quality improvement only had a minor effect on cardiovascular hospital admissions. Air quality improvement and increased active travel mainly had an impact at older age, while traffic safety mainly affected younger and middle-aged people. This modelling approach illustrates the feasibility of a comprehensive health impact assessment of changes in travel behaviour. Our results suggest that more is needed than a policy rising car fuel prices by 20% to achieve substantial health gains. While the activity-based model gives an answer on what the effect of a proposed policy is, the focus on health may make policy integration more tangible. The model can therefore add to identifying win–win situations for both transport and health.
Article
By focussing on air pollutant concentration levels only, the variation in population mobility is not taken into account when assessing the exposure. Transportation policies have an impact on both concentration levels and mobility patterns. The impact of a fuel price increase policy on population exposure to elemental carbon (EC) was evaluated and compared to the base scenario (current situation), taking into account time-activity patterns e including time in commute. We assessed the effect on exposure of both the change in concentrations and whereabouts. The decrease in exposure due to the fuel price increase using residential information only was limited to areas near highways and urban centres. Integrating population movement, exposures to EC were higher and the decrease in exposure was no longer limited to areas near traffic hotspots. For inhabitants of urban areas, the exposure integrating time-activity patterns was more similar to the residential exposure, as they spent more time in their own neighbourhood. For people living further away from traffic hotspots, the estimated impact of the policy was higher than expected for residential exposure. These people profited both from the higher decrease in concentrations at their work/shop/leisure destinations in more urban areas and, as they have to travel longer, also had a larger gain from the high decrease in concentrations during transport. Therefore, the impact of changing concentrations is underestimated when using residential exposure only. These results show the importance of taking into activity-travel patterns when planning future actions
Article
Cohort studies designed to estimate human health effects of exposures to urban pollutants require accurate determination of ambient concentrations in order to minimize exposure misclassification errors. However, it is often difficult to collect concentration information at each study subject location. In the absence of complete subject-specific measurements, land-use regression (LUR) models have frequently been used for estimating individual levels of exposures to ambient air pollution. The LUR models, however, have several limitations mainly dealing with extensive monitoring data needs and challenges involved in their broader applicability to other locations. In contrast, air quality models can provide high-resolution source–concentration linkages for multiple pollutants, but require detailed emissions and meteorological information. In this study, first we predicted air quality concentrations of PM2.5, NOx, and benzene in New Haven, CT using hybrid modeling techniques based on CMAQ and AERMOD model results. Next, we used these values as pseudo-observations to develop and evaluate the different LUR models built using alternative numbers of (training) sites (ranging from 25 to 285 locations out of the total 318 receptors). We then evaluated the fitted LUR models using various approaches, including: 1) internal “Leave-One-Out-Cross-Validation” (LOOCV) procedure within the “training” sites selected; and 2) “Hold-Out” evaluation procedure, where we set aside 33–293 tests sites as independent datasets for external model evaluation. LUR models appeared to perform well in the training datasets. However, when these LUR models were tested against independent hold out (test) datasets, their performance diminished considerably. Our results confirm the challenges facing the LUR community in attempting to fit empirical response surfaces to spatially- and temporally-varying pollution levels using LUR techniques that are site dependent. These results also illustrate the potential benefits of enhancing basic LUR models by utilizing air quality modeling tools or concepts in order to improve their reliability or transferability.
Article
This paper describes the development of an integrated approach for assessing ambient air quality and population exposure as a result of road passenger transportation in large urban areas. A microsimulation activity-based travel demand model for the Greater Toronto Area – the Travel Activity Scheduler for Household Agents – is extended with capabilities for modelling and mapping of traffic emissions and atmospheric dispersion. Hourly link-based emissions and zone-based soak emissions were estimated. In addition, hourly roadway emissions were dispersed at a high spatial resolution and the resulting ambient air concentrations were linked with individual time-activity patterns derived from the model to assess person-level daily exposure. The method results in an explicit representation of the temporal and spatial variation in emissions, ambient air quality, and population exposure.
Article
Concentrations of traffic-related air pollution can be highly variable at the local scale and can have substantial seasonal variability. This study was designed to provide estimates of intra-urban concentrations of ambient nitrogen dioxide (NO2) in Montreal, Canada, that would be used subsequently in health studies of chronic diseases and long-term exposures to traffic-related air pollution. We measured concentrations of NO2 at 133 locations in Montreal with passive diffusion samplers in three seasons during 2005 and 2006. We then used land use regression, a proven statistical prediction method for describing spatial patterns of air pollution, to develop separate estimates of spatial variability across the city by regressing NO2 against available land-use variables in each of these three periods. We also developed a “pooled” model across these sampling periods to provide an estimate of an annual average. Our modelling strategy was to develop a predictive model that maximized the model R2. This strategy is different from other strategies whose goal is to identify causal relationships between predictors and concentrations of NO2.Observed concentrations of NO2 ranged from 2.6 ppb to 31.5 ppb, with mean values of 12.6 ppb in December 2005, 14.0 ppb in May 2006, and 8.9 ppb in August 2006. The greatest variability was observed during May. Concentrations of NO2 were highest downtown and near major highways, and they were lowest in the western part of the city. Our pooled model explained approximately 80% of the variability in concentrations of NO2. Although there were differences in concentrations of NO2 between the three sampling periods, we found that the spatial variability did not vary significantly across the three sampling periods and that the pooled model was representative of mean annual spatial patterns.
Article
Recent air quality studies have highlighted that important differences in pollutant concentrations can occur over the day and between different locations. Traditional exposure analyses, however, assume that people are only exposed to pollution at their place of residence. Activity-based models, which recently have emerged from the field of transportation research, offer a technique to micro-simulate activity patterns of a population with a high resolution in space and time. Due to their characteristics, this model can be applied to establish a dynamic exposure assessment to air pollution.This paper presents a new exposure methodology, using a micro-simulator of activity–travel behaviour, to develop a dynamic exposure assessment. The methodology is applied to a Dutch urban area to demonstrate the advantages of the approach for exposure analysis. The results for the exposure to PM10 and PM2.5, air pollutants considered as hazardous for human health, reveal large differences between the static and the dynamic approach, mainly due to an underestimation of the number of hours spent in the urban region by the static method.We can conclude that this dynamic population modelling approach is an important improvement over traditional methods and offers a new and more sensitive way for estimating population exposure to air pollution. In the light of the new European directive, aimed at reducing the exposure of the population to PM2.5, this new approach contributes to a much more accurate exposure assessment that helps evaluate policies to reduce public exposure to air pollution.
Article
Speed reduction measures rank among the most common schemes to improve traffic safety. Recently many urban streets or entire districts were converted into 30 kph zones and in many European countries the maximum permissible speed of trucks on motorways is under discussion. However, besides contributing to traffic safety, reducing the maximum speed is also seen as beneficial to the environment due to the associated reduced fuel consumption and lower emissions. These claims however are often unsubstantiated. To gain greater insight into the impact of speed management policies on emissions, this paper examines the impact on different traffic types (urban versus highway traffic) with different modelling approaches (microscopic versus macroscopic). Emissions were calculated for specific types of vehicles with the microscopic VeTESS-tool using real-world driving cycles and compared with the results obtained using generalized Copert-like macroscopic methodologies. We analyzed the relative change in pollutants emitted before and after the implementation of a speed reduction measure for passenger cars on local roads (50–30 kph) and trucks on motorways (90–80 kph). Results indicate that emissions of most classic pollutants for the research undertaken do not rise or fall dramatically. For the passenger cars both methods indicate only minor changes to the emissions of NOx and CO2. For PM, the macroscopic approach predicts a moderate increase in emissions whereas microscopic results indicate a significant decrease. The effects of specific speed reduction schemes on PM emissions from trucks are ambiguous but lower maximums speed for trucks consistently result in lower emissions of CO2 and lower fuel consumption. These results illustrate the scientific uncertainties that policy makers face when considering the implementation of speed management policies.
Article
Compact city forms are associated with minimal consumption of land and energy, hence, they are often promoted as being the more sustainable thus preferred mode of urban development. In this context, numerical simulations were performed to evaluate the effect of urban sprawl on air quality and associated human exposure. Working on a highly urbanised area in the German Ruhrgebiet, models dealing with satellite data processing, traffic flows, pollutant emission and atmospheric dispersion were applied in an integrated fashion, under conditions representative of the urbanised area as it is today. A fair agreement was obtained between simulated and observed meteorological variables, as well as between simulated and observed concentrations of ozone and particulate matter. Simulated atmospheric pollution fields were found to closely reflect urbanisation patterns. In a companion paper [De Ridder, K., Lefebre, F., Adriaensen, S., Arnold, U., Beckroege, W., Bronner, C., Damsgaard, O., Dostal, I., Dufek, J., Hirsch, J., IntPanis, L., Kotek, Z., Ramadier, T., Thierry, A., Vermoote, S., Wania, A., Weber, C., 2008. Simulating the impact of urban sprawl on air quality and population exposure in the German Ruhr area. Part II: Development and evaluation of an urban growth scenario], the results of this base case simulation will be compared with those of a scenario simulation, designed to mimic urban sprawl, so as to allow the evaluation of the latter on air quality and associated human exposure.
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Based on wind tunnel experiments, theoretical considerations and measurements, the dispersion model CAR (calculation of air pollution from road traffic) has been developed for determining air quality in city streets. CAR International, which is a simple parameterized model using readily available input data, calculates annual percentile values and average concentrations close to streets (at the kerbside) for non-reactive air pollutants and NO2. The accuracy of the model has proved to be good and is within the limits set by Dutch air quality decrees. CAR International can be used for a quick survey of city street air quality. It is also a valuable tool for judging the effects of traffic management plans and for scenario studies.
Article
Nowadays urban pollution exposure from road transport has become a great concern in major cities throughout the world. A modelling framework has been developed to simulate Personal Exposure Frequency Distributions (PEFDs) as a function of urban background and roadside pollutant concentrations, under different traffic conditions. In this paper, we present a technique for classifying roads, according to their traffic conditions, using the traffic characteristics and fleet compositions. The pollutant concentrations data for 2001 from 10 Roadside Pollution Monitoring (RPM) units in the city of Leicester were analysed to understand the spatial and temporal variability of the pollutant concentrations patterns. It was found that variability of pollutants during the day can be associated with specific road traffic conditions. Statistical analysis of two urban and two rural Automated Urban and Rural Network (AURN) background sites for particulates suggests that PM2.5 and PM10 are closely related at urban sites but not at rural sites. The ratio of the two pollutants observed at Marylebone was found to be 0.748, which was applied to Leicester PM10 data to obtain PM2.5 profiles. These results are being used as an element in the PEFDs model to estimate the impact of urban traffic on exposure.
Article
Local air quality management requires the use of screening and advanced modelling tools that are able to predict roadside pollution levels under a variety of meteorological and traffic conditions. So far, more than 200 air pollution hotspots have been identified by local authorities in the UK, many of them associated with NO2 and/or PM10 exceedences in heavily trafficked urban streets that may be classified as street canyons or canyon intersections. This is due to the increased traffic-related emissions and reduced natural ventilation in such streets. Specialised dispersion models and empirical adjustment factors have been commonly used to account for the entrapment of pollutants in street canyons. However, most of the available operational tools have been validated using experimental datasets from relatively deep canyons (H/W⩾1) from continental Europe. The particular characteristics of low-rise street canyons (H/W<1), which are a typical feature of urban/sub-urban areas in the UK, have been rarely taken into account.The main objective of this study is to review current practice and evaluate three widely used regulatory dispersion models, WinOSPM, ADMS-Urban 2.0 and AEOLIUS Full. The model evaluation relied on two comprehensive datasets, which included CO, PM10 and NOx measurements, traffic information and relevant meteorological data from two busy street canyons in Birmingham and London for a 1-year period. The performance of the selected models was tested for different times of the day/days of the week and varying wind conditions. Furthermore, the ability of the models to reproduce roadside NO2/NOx concentration ratios using simplified chemistry schemes was evaluated for one of the sites. Finally, advantages and limitations of the current regulatory street canyon modelling practice in the UK, as well as needs for future research, have been identified and discussed.
Article
Studies on the health effects of long-term average exposure to outdoor air pollution have played an important role in recent health impact assessments. Exposure assessment for epidemiological studies of long-term exposure to ambient air pollution remains a difficult challenge because of substantial small-scale spatial variation. Current approaches for assessing intra-urban air pollution contrasts include the use of exposure indicator variables, interpolation methods, dispersion models and land-use regression (LUR) models. LUR models have been increasingly used in the past few years. This paper provides a critical review of the different components of LUR models.
Article
Children are particularly vulnerable to the health effects of climate change, the biggest global health threat of the 21st century. However, the worst effects on child health can be avoided, and well-designed climate policies can have important benefits for child health and equity. We call on child health professionals to seize opportunities to prevent climate change, improve child health and reduce inequalities, and suggest useful actions that can be taken. © 2011 Paediatrics and Child Health Division (Royal Australasian College of Physicians).