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Anomalous Radiation Produced by Glow Discharge in Deuterium Containing Oxygen

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ElectroMagnetic Radiation (EMR) and anomalous radiation (potentially produced by nuclear reactions, involving high energy particles), in a low-voltage discharge in a gas containing deuterium was measured using a Geiger counter located within the apparatus. This radiation is found to consist of energetic particles that are produced only when the voltage is above a critical value. In addition, the emission is very sensitive to the presence of oxygen in the gas. The intensity of the reaction producing the radiation could be fit by a power function when compared to the applied voltage. The effect of EMR and other sources of noise that might be attributed to the anomalous radiation are discussed.
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1
Storms, E. and B. Scanlan. Radiation Produced By Glow Discharge In Deuterium. in 8th
International Workshop on Anomalies in Hydrogen / Deuterium Loaded Metals. 2007. Sicily,
Italy. From: http://www.iscmns.org/catania07/index.htm
RADIATION PRODUCED BY GLOW DISCHARGE IN DEUTERIUM
Edmund Storms and Brian Scanlan
KivaLabs, LLC
ABSTRACT
Radiation produced by low-voltage discharge in a gas containing deuterium was measured
using a Geiger counter located within the apparatus. This radiation was found to consist of
energetic particles that were produced only when the voltage was above a critical value. In
addition, the emission was very sensitive to the presence of oxygen in the gas. In the
presence of the required conditions, emission occurred reliably with reaction rates in excess
of 10
8
events/second.
I. INTRODUCTION
Evidence for the LENR effect was and still is based to a large extent on production of
anomalous energy. Many of the observations imply nuclear reaction rates in excess of 10
12
events/sec. In addition, the presence of detectable helium, tritium, and transmutation products
show that nuclear products are, in fact, produced. Absence of expected conventional radiation,
consisting of neutrons and gamma, has long since been acknowledged. Nevertheless, such a high
reaction rate is expected to produce detectable X-ray emission even if the primary radiation
cannot penetrate the surrounding wall. Failure in the past to detect any kind of radiation has led
some theoreticians to propose a direct coupling of energy to the lattice, without need for
emission of radiation or energetic particles of any kind.
With increasing frequency, as proper detectors are used, researchers are observing several
types of radiation, as summarized in a recent book [1]. These emissions consist of X-ray, gamma
ray, and various charged particles. Although the intensity of these emissions cannot explain the
high levels of heat observed during some experiments, the mere existence of such energetic
radiation raises important questions, such as the following.
1. Does the detected radiation result from one nuclear reaction or do several energetic
processes occur at the same time?
2. Is any of the energy generated by these nuclear reactions coupled to the lattice? If so,
why is the energy associated with the detected emissions not coupled?
3. Does the primary nuclear reaction produce the reported X-radiation or does it result when
emitted energetic particles are absorbed by the surrounding material?
This study was initiated in an attempt to answer these questions using low-voltage gas
discharge in low-pressure deuterium containing gas. A Geiger-Müller (GM) detector and a
silicon barrier detector were located within the apparatus near the discharge. In the process, very
2
energetic electron and particle emission were detected and characterized. These emissions occur
at very high intensity and occur reliably within the appropriate voltage, current, pressure, and gas
composition. This work is preliminary and is presented only to demonstrate that such radiation
can be produced without making claims about its source or the mechanism of its production.
II. EXPERIMENTAL
The apparatus is shown in Fig 1. A turbomolecular pump is located below the table on which
the apparatus is supported. This pump can produce a vacuum of less than 10
-6
Torr in the
discharge cell prior to adding deuterium-containing gas. Gas pressure within the cell during
discharge is measured by Baratron gauges (0-10 and 0-100 Torr) located at the rear. To the left
of the cell are connections for the GM detector, which has an end-window of mica (1.7-2.2
mg/cm
2
, LND 712). To the right are connections to the water-cooled cathode, which is grounded
to the apparatus. Connection to the anode is made out of sight at the rear of the cell. A residual
gas analyzer (RGA) is provided to allow gas in the discharge chamber to be analyzed up to
mass/charge of 50. Figure 2 shows the anode, which is a 2 mm diameter palladium wire and the
cathode, which is surrounded by an insulating shroud. This arrangement allows the radiation
detector, located at the left, a clear view of the cathode surface, as can be seen in the cathode-eye
view in Fig. 3. The cathode is a thin metal disc directly cooled by flowing water, a design that
allows the cathode surface to be easily examined. Details of cathode assembly are shown in Fig.
4. This design can dissipate power in excess of 300 watts, permitting a wide range of current and
voltage to be used. A collection of absorbers of different thickness can be placed between the
cathode and detector to allow the energy and type of the radiation to be determined. These are
moved by magnets from outside the vacuum, as shown in Fig. 5.
FIGURE 2. View of anode (left) and cathode
(right).
FIGURE 1. Overall view of the apparatus.
3
Discharge is produced using a power supply rated at 1.5 A and 2000 V running under current
control. Voltage is supplied to the anode through a forced-air cooled resistor of 300 ohm. The
supplied current and the voltage at the anode are measured and stored approximately every 6 to
60 sec. Although calorimetry could be done using this apparatus, none was attempted during this
study.
A Geiger counter alone or combined with a silicon barrier detector was used to measure
radiation. During the first part of the study, the amount of radiation was proportional to a voltage
produced by the GM counting circuit that averaged the count rate. A maximum count rate of
approximately 5000 counts/sec on scale 10 was limited by the circuit becoming saturated. Later,
the count rate was measured directly by counting individual pulses produced by the GM tube,
which permitted much greater values to be determined. This design allowed particle production
rates in excess of 10
6
/sec to be measured, a limit that was imposed only by unwanted electrical
discharge to the body of the cell. The energy and type of radiation was determined by placing
absorbers of varying thickness between the GM tube and the discharge. Later in the study, the
output of the Si barrier detector, shown in Fig. 6, allowed the energy of radiation to be
determined directly.
FIGURE 3. Cathode-eye view of the GM radiation
detector. One of the copper absorbers is seen on the left.
The anode is one of several designs using 2 mm wire
covered by a glass insulator. The large tube from which it
emerges is a glass-filled insulator.
FIGURE 4. Exploded view of the cathode
showing the insulating shroud. The cathode
disc can be removed and is sealed using a
rubber O-ring.
4
Energetic electrons and charged particles, having several energies, were detected. As yet, these
charged particles have not been sorted into proton, triton, or alpha, although the energetic
electrons have been clearly identified. Which of these emission, if any, is produced depends
critically on small impurities in the deuterium gas and the nature of the glow discharge including
its voltage and current.
Before discussing the observed radiation, understanding the nature of a glow discharge is
necessary. A discharge consists of three parts; the cathode bright zone, the dark zone, and the
anode bright zone. The bright zones occur where sufficient energy is available to cause
ionization as electrons move from the cathode to the anode. In this study, the cathode bright zone
grows in thickness as applied voltage is increased until it engulfs the anode. Ions created in the
bright zones bombard the cathode causing changes in the cathode surface. The resulting
sputtering of cathode material causes growth of cones, shown in Fig. 7. As a result, thickness of
the cathode increases while its weight decreases. Consequently, material is being lost from
regions between the cones while it is deposited on their tops. In addition, any material sputtered
from the shroud also deposits on the tops, as indicated by the dark regions seen in Fig. 7. Shroud
materials consisting of Al
2
O
3
, BN, mica-based ceramic, or Teflon were used. All except Teflon
worked well. Teflon caused the electron radiation to decay away over about 10 minutes during
glow-discharge when it was used with a previously active cathode. When sufficient oxygen is
present in the gas in any chemical form, detectable oxide also forms in these regions. The cones
are proposed to be the radiation source.
During the first part of the study, only D
2
at a pressure of about 30 Torr was used in the cell to
generate the radiation described below. Subsequent work suggested that the presence of a small
amount of carbon-containing impurity in the gas was required for success. Too much
FIGURE 6. Si barrier detector (Ortec TB-016-
050-1000) and GM tube (2.2-2.6 mg/cm
2
).
FIGURE 5. View of the mechanism used to move
absorbers of varying thickness in front of the GM tube
with magnets. Each assembly has two different
thickness and an open position, which allows 8
combinations of thickness. The GM tube can be seen
on the left.
5
hydrocarbon in the gas impedes the discharge as carbon is deposited on the cathode surface. On
the other hand, a system that is too clean will not produce energetic electrons having an energy
described here. Once the discharge become stable and uniform over the cathode surface, the
relationship shown in Fig. 8 is obtained. Although variations in this behavior are seen, in all
cases this radiation is sensitive to applied current but not to cell voltage. Little change in
behavior was found when copper, copper plated with palladium, palladium, Sterling silver, or a
Pd+Pt alloy are used as the cathode for producing this type of radiation. The anode is a 2 mm
diameter palladium wire in all cases. A distance of 6 mm to 10 mm between the anode and
cathode was used, all of which successfully produced the effect.
A combination of copper foils of varying thickness were placed between the GM tube and the
glow discharge using a cathode made from an alloy of Pd + Pt, surrounded by a mica-based
ceramic The result is shown in Fig. 9. As absorber thickness is increased, the amount of radiation
reaching the GM tube decreases. However, near the limit, the amount of radiation abruptly
increases. This increase is caused by X-radiation, generated by the absorption process
(Bremsstrahlung), adding to the remaining electron radiation. Above the limit, only X-radiation
remains, which is slowly reduced as thickness is increased. This limit shows that the electrons
have nearly a single energy of 0.8±0.1 MeV based on the equation given by Katz and Penfold.[2]
Because these electrons are monoenergetic, they do not result from beta decay. Also, when cell
current is stopped, the reaction stops abruptly without an apparent decay.
When oxygen containing gas, such as O
2
, D
2
O, or H
2
O is added to the D
2
, a different kind of
emission is produced. This radiation is completely stopped by an absorber having 1.74 mg/cm
2
added to the absorption produced by the GM counter window of 2.0 mg/cm
2
for a total of ~3.74
FIGURE 7. Surface of a Pd+Pt alloy after being
subjected to gas discharge in D
2
using a ceramic
shroud containing the oxides of Mg, Al, Na, Si
and K. The black regions contain shroud material
that is not present elsewhere.
0.00
0.0100
0.0200
0.0300
0.0400
0.0500
0.0600
0 0.05 0.1 0.15 0.2 0.25
(4-30-07)Pt+Pd#1c
GM COUNTER, Scale 10
APPLIED CURRENT, A
Y = M0 + M1*x + ... M8*x
8
+ M9*x
9
-0.00010608M0
0.00990175M1
0.914962M2
0.997724R
FIGURE 8. Effect of cell current on output of GM
counter.
6
mg/cm
2
. The radiation could be protons with an energy of at least 0.7 MeV but less than about
1.2 MeV or alphas with an energy of at least 2.9 MeV but less than 4.7 MeV. The low value of
this range is required for the particle to pass through the window of the GM tube and a particle
having the upper value is stopped by the sum of the window and absorber. Onset of this emission
was very sensitive to applied voltage, with a critical voltage below which no radiation was
detected. In addition, this behavior was altered by changing the D/O ratio in the gas. Least
squares lines drawn through the data were used to obtain values for the slope and the critical
voltage at which no radiation was detected. Examples of these effects are shown in Fig. 10 where
various isotopes of oxygen are used as the source of oxygen. The effect is not sensitive to the
isotopic composition of oxygen. When all measurements are compared, the maximum effect is
found to occur when the D/O ratio in the gas is near 0.1, as shown in Fig. 11. In other words,
once voltage is increased above the critical value, the voltage has a maximum effect on emission
when about 10 atoms of O are present for each atom of D in the gas. When oxygen is added in
the form of H
2
O, the behavior is the same as when D
2
O or O
2
are used. This effect only applies
to relatively low emission rates. When the system was designed to measure higher rates and
greater voltage was applied, the emission rate is found to increase in a nonlinear way, as shown
in Fig. 12, but with the expected effect of increased oxygen.
0.00
0.500
1.00
1.50
2.00
0 0.2 0.4 0.6 0.8 1 1.2 1.4
(4-30-07)Pt-Pd
RELATIVE GM COUNT
THICKNESS COPPER, g/cm
2
Electron+X-ray
Energy limit
X-ray
FIGURE 9. Effect of copper absorbers on the amount
of radiation reaching the GM tube from a Pd+Pt
cathode.
0.0
0.1
0.2
0.3
0.4
0.5
0.6
0.7
560 570 580 590 600 610
620
(7-21-07)
D/O(17)=0.19
D/O(17)=4.46
D/O(17)=0.089
D/O(18)=0.051
D/O(18)=0.44
D/O(18)=2.31
D/O(18)=19.33
D/O(16)=20.14
D/O(16)=0.11
GM COUNTER, Scale 10
APPLIED VOLT
FIGURE 10. Effect of voltage on emission at various
D/O atom ratios and with various isotopic
compositions of oxygen.
7
The GM tube is stated by the supplier to have a window with an area density of 1.5-2.0
mg/cm
2
. Because this window limits the energy of detected radiation, its value must be known
more accurately. For this measurement, a Po
210
alpha source was moved at various distances
from the tube in air and the distance at which no counts were detected was determined. Counts
stopped between 2.42 mg/cm
2
and 2.91 mg/cm
2
, based on the density of laboratory air. The
range of the 5.30 MeV alpha in air is 4.57 mg/cm
2
. Consequently, the thickness of the GM
window is equivalent to 1.7 mg/cm
2
to 2.2 mg/cm
2
. A value of 2.0 mg/cm
2
was used to calculate
the absorption characteristics of the GM counter using published values.[3]
IV. CONCLUSION
Energetic emissions are produced during gas discharge that cannot be detected outside of the
apparatus. Nevertheless, their energy is so large that they can only result from nuclear reactions.
If conditions are appropriate, the emissions are easily reproduced and imply a reaction rate at the
cathode in excess of 10
9
reactions/sec, limited only by the design of the apparatus. Consequently,
these energetic emissions are completely anomalous, are produced at high rates that can be
increased to the rates associated with anomalous heat production, and are not difficult to
generate. The observations show that energetic electrons make up part of this emission and
energetic particles that might be protons and/or alpha particles add to the radiation, depending on
the chemical composition of the cathode and gas. The type of radiation, its energy, and the rate
are all sensitive to the presence of certain elements in the environment.
This work indicates that when nuclear reactions are generated at the cathode surface using
glow discharge, the energy is not coupled to the lattice, but appears as very energetic charged
particles. Because the particles cannot escape most apparatus and their presence can only be
-2.40
-2.20
-2.00
-1.80
-1.60
-1.40
-1.20
-1.00
-2.0 -1.0 0.0 1.0 2.0 3.0
log S, log D-O, +H
D + O
D + O + H
Log (Slope)
Log (D/O)
FIGURE 11. Relationship between log slope produced
by changing the applied voltage above the critical value
vs log D/O atom ratio in the gas. Oxygen was supplied
0.0
2.0 10
7
4.0 10
7
6.0 10
7
8.0 10
7
1.0 10
8
560 580 600 620 640 660 680
(7-27-07)Fe
D/O=6.3
D/O=8.9
D/O=2.8
REACTION RATE, c/s
APPLIED VOLT, V
Previous range
200 W applied power
count=-3.438e9+1.9787e7*V-3.794e4*V^2+24.23*V^3
FIGURE 12. Reaction rate, corrected for
detector size and distance, vs applied voltage at
various D/O atom ratios.
8
discovered when certain kinds of detectors are used, their presence has not been detected before
at the rates generated in this study.
If these observations apply to LENR in general, the chemical composition of the environment
in which the nuclear reactions are initiated would play a significant role in permitting nuclear
reactions to take place and would determine the resulting nuclear products.
References
[1] Storms, E., “The Science of Low Energy Nuclear Reaction”, World Scientific Publishing Co., 2007.
[2] Katz, L and Penfold, A.S., Rev. Mod. Phys., 24 (1952) 28.
[3] Radiological Health Handbook, U.S. Dept. of Health, Education and Welfare, Washington, DC. 1970.
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  • Katz
  • A S Penfold
Katz, L and Penfold, A.S., Rev. Mod. Phys., 24 (1952) 28.