About
243
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Introduction
Current institution
Additional affiliations
December 2014 - present
October 2007 - November 2014
January 2006 - September 2007
Education
August 1998 - September 2002
August 1998 - September 2002
August 1993 - July 1998
Publications
Publications (243)
The large (26-fold over the past 25 years) increase in the on-road vehicle fleet in China has raised sustainability concerns regarding air pollution prevention, energy conservation, and climate change mitigation. China has established integrated emission control policies and measures since the 1990s, including implementation of emission standards f...
Hydrogen has the potential to contribute to a clean, secure, and affordable energy future. It can provide distributed energy storage for intermittent renewable energy resources and support hydrogen-based transportation. This study reports well-to-wheels greenhouse gas (GHG) and criteria air pollutant emissions and levelized cost of driving (LCD) fo...
Significance
On-road vehicles have become a significant source of air pollution in Chinese cities. Air pollution in China has substantial impacts on public health and is thought to be responsible for millions of deaths each year. The government has implemented comprehensive control measures to mitigate vehicle emissions since the late 1990s. In thi...
https://www.nature.com/articles/s41893-019-0398-8
China has emerged as a leading electric vehicle (EV) market, accounting for approximately half of the global EV sales volume. We employed an atmospheric chemistry model to evaluate the air quality impacts from multiple scenarios by considering various EV penetration levels in China and assessed the...
Mass adoption of electric vehicles (EVs) is widely viewed as essential to address climate
change and requires a compelling case for ownership worldwide. While the manufacturing costs and technical capabilities of EVs are similar across regions, customer needs and economic contexts vary widely. Assessments of the all-electric-range (AER) required to...
Shuwen Guo Xuan Zheng Xiao He- [...]
Ye Wu
The role of intermediate-volatility and semi-volatile organic compounds (I/SVOCs) in heavy-duty diesel vehicle (HDDV) exhaust remains a significant research gap in previous studies, with limited focus on cumulative mileage and ambient temperature effects. This study analyzed gaseous and particulate I/SVOCs from four in-use HDDVs using thermal desor...
Shuwen Guo Xuan Zheng Xiao He- [...]
Ye Wu
The role of intermediate- and semi-volatile organic compounds (I/SVOCs) in heavy-duty diesel vehicle (HDDV) exhaust remains a significant research gap across previous studies, with limited focus on cumulative mileage and ambient temperature effects. This study analyzed gaseous and particulate I/SVOCs from four in-use HDDVs using thermal desorption...
The adoption of zero-emission vehicles (ZEVs) offers multiple benefits for the climate, air quality, and public health by reducing tailpipe emissions. However, the environmental justice implications of the nonexhaust emissions from future ZEV fleets for near-roadway communities remain unclear. Here, we model the on-road fine particulate matter (PM2...
Traffic-related air pollutants (TRAPs) emitted from vehicle tailpipes disperse into nearby microenvironments, posing potential exposure risks. Thus, accurately identifying the emission hotspots of TRAPs is essential for assessing potential exposure risks. We investigated the relationship between turbulent kinetic energy (TKE) and pollutant dispersi...
Xiao He Xuan Zheng Shuwen Guo- [...]
Ye Wu
The advancement of analytical techniques, such as comprehensive two-dimensional gas chromatography coupled with mass spectrometry (GC×GC–MS), enables the efficient separation of complex organics. Developing innovative methods for data processing and analysis is crucial to unlock the full potential of GC×GC–MS in understanding intricate chemical mix...
Implementing temporary traffic control measures is a common strategy to prevent air pollution and alleviate traffic congestion during mega-events. Accurate assessment of event-time vehicular emissions is useful for local authorities to develop effective policies. However, many previous assessments were based on policy-based scenarios, which often f...
The in-depth investigation of the high black carbon (BC) emission scenarios of heavy-duty diesel vehicles (HDDVs) is a crucial step toward developing effective control strategies. Chassis dynamometer tests were conducted for three in-use HDDVs, namely, vehicle #1, #2, and #3, focusing on the instantaneous BC characterizations during multiple drivin...
Xiao He Xuan Zheng Shuwen Guo- [...]
Ye Wu
The advancement of analytical techniques, such as comprehensive two-dimensional gas chromatography coupled with mass spectrometry (GC×GC-MS), enables the efficient separation of complex organic matrix. Developing innovative methods for data processing and analysis is crucial to unlock the full potential of GC×GC-MS in understanding intricate chemic...
Nitrogen oxides (NOx) emissions from heavy-duty diesel vehicles (HDDVs) have adverse effects on human health and the environment. On-board monitoring (OBM), which can continuously collect the vehicle performance and NOx emissions throughout the operation lifespan, is recognized as the core technology for future vehicle in-use compliance, but its la...
Some in-use China IV and China V heavy-duty diesel vehicles (HDDVs) with selective catalytic reduction (SCR) systems probably fail to mitigate nitrogen oxide (NOX) emissions as expected. Meanwhile, these SCR-equipped HDDVs might emit excessive ammonia (NH3). To better understand the NOX and NH3 emissions from typical HDDVs in China, seventeen in-us...
China’s civil aviation market has rapidly expanded, becoming the world’s second-largest. However, the air quality and health impacts caused by its aircraft emissions have been inadequately assessed. Here, we leverage an updated emission inventory of air pollutants with improved temporal and spatial resolution based on hundreds of thousands of fligh...
Real-world heavy-duty diesel trucks (HDTs) were found to emit far more excess nitrogen oxides (NOx) and black carbon (BC) pollutants than regulation limits. It is essential to systematically evaluate on-road NOx and BC emission levels for mitigating HDTs emissions. This study launched 2109 plume chasing campaigns for NOx and BC emissions of HDTs ac...
Vehicle emissions in China have been decoupled from the rapid motorization owing to the comprehensive control strategies. China’s increasingly ambitious goals for better air quality are calling for deep emission mitigation, posing a need to develop an up-to-date emission inventory that can reflect the fast-developing policies on vehicle emission co...
On-road tailpipe ammonia (NH3) emissions contribute to urban secondary organic aerosol formation and have direct or indirect adverse impacts on the environment and human health. To understand the tailpipe NH3 emission characteristics, we performed comprehensive chassis dynamometer measurements of NH3 emission from two China 5 and two China 6 light-...
A widening gap between official and real-world fuel consumption of passenger cars has been reported worldwide. However, previous policy evaluation has not adequately incorporated real-world performance. To comprehensively evaluate China’s orporate Average Fuel Consumption (CAFC) policy, we update the fuel
consumption gap with millions of consumer-r...
China is facing the challenge of synergistic reduction of air pollutants and CO2 emissions. However, the studies on its historical progress and future priorities are insufficient. This study compiled China's emission inventory of air pollutants and CO2 from 2005 to 2021 (ABaCAS-EI v2.0 dataset) based on a unified emission-source framework by consid...
The synergetic benefit of air quality improvements together with greenhouse gas (GHG) mitigations from fleet electrification can be maximized if the power used for electric vehicles (EVs) is from renewables. The worth-noting mismatch between renewable power generation and EV fleet charging demand requires appropriate coordination strategy. Here, we...
China has made great progress in the electrification of passenger cars, and the sales of battery electric vehicles (BEVs) have exceeded 10%. We applied a life-cycle assessment (LCA) method to estimate the carbon dioxide (CO 2) emissions of the past (2015), present (2020), and future (2030) BEVs, incorporating China's carbon peaking and neutrality p...
On-road ammonia (NH3) emissions play a significant role in fine particulate matter (PM2.5) formation in urban areas, posing severe risks for human health. Limited studies have depicted the spatial and temporal variations of on-road NH3 emissions, in particular lacking detailed quantification of their contributions within densely populated areas. In...
An increasing divergence regarding fuel consumption (and/or CO2 emissions) between real-world and type-approval values for light-duty gasoline vehicles (LDGVs) has posed severe challenges to mitigating greenhouse gases (GHGs) and achieving carbon emissions peak and neutrality. To address this divergence issue, laboratory test cycles with more real-...
Ammonia (NH3) plays a vital role in the formation of fine particulate matter (PM2.5). Prior studies have primarily focused on the control of agricultural NH3 emissions, the dominant source of anthropogenic NH3 emissions. The air quality impact from vehicular NH3 emissions, which could be particularly important in urban areas, has not been adequatel...
China is facing the challenge of synergistic reducing air pollutants and CO2 emissions in the coming decades. The coupled emission inventory of air pollutants and CO2 is a prerequisite to designing the synergetic emission reduction strategy. This study compiled China’s emission inventory of air pollutants and CO2 during 2005–2021 (ABaCAS-EI v2.0 da...
On-road ammonia (NH3) emissions play a significant role in fine particulate matter (PM2.5) formation in urban areas, posing severer risks for human health. Limited studies have depicted the spatial and temporal variations of on-road NH3 emissions, in particular lacking detailed quantification of their contributions within densely-populated areas. I...
The rapidly growing vehicle population has become a crucial contributor to severe air-pollution and public health issues. In urban areas, vehicles have become one of the important sources of air pollutants such as nitrogen oxides and fine particulate matter (PM2.5). In particular, the on-road concentrations of traffic-related air pollutants (TRAPs)...
The distribution pattern of near-road air pollutants is important for addressing air pollution issues. In this study, size-segregated particle number concentration (PNC) and black carbon (BC) concentration were measured at different locations perpendicular to a major roadway in Shanghai, aiming to improve the understanding of distribution patterns...
Dong Ma Xiaomeng Wu Xin Sun- [...]
Ye Wu
Vehicle mileage is one of the key parameters for accurately evaluating vehicle emissions and energy consumption. With the support of the national annual vehicle emission inspection networked platform in China, this study used big data methods to analyze the activity level characteristics of the light-duty passenger vehicle fleet with the highest ow...
Tailpipe emissions from three heavy-duty diesel vehicles (HDDVs), complying with varying emission standards and installed with diverse aftertreatment technologies, are collected at a certified chassis dynamometer laboratory. The HDDV-emitted intermediate-volatility and semi-volatile organic compound (I/SVOC) emission and the gas–particle partitioni...
Efforts have been directed to pollution control of fine particles (PM2.5) since exposure to PM2.5 could result in adverse health effects. However, PM2.5 exposure disparities persisted even with largely declined concentrations. Here, we applied taxi-based measurements to characterize hyper-localized PM2.5 exposures (30-m resolution) in Xi'an in 2019...
Tailpipe emissions from three heavy-duty diesel vehicles (HDDVs), complying with varying emission standards and installed with diverse aftertreatment technologies, are collected at a certified chassis dynamometer laboratory. The HDDV-emitted intermediate-volatility and semi-volatile organic compound (I/SVOC) emission and the gas-particle partitioni...
Rooftop solar photovoltaics (RSPV) is critical for megacities to achieve low-carbon emissions. However, a knowledge gap exists in a supply-demand coupled analysis that considered simultaneously RSPV spatiotemporal patterns and city-accommodation capacities, a pivotal way to address solar PV intermittency issues. Here, we developed an aggregated mod...
Progressively stringent regulations regarding vehicle emissions and fuel economy have spurred technology diversification in light-duty passenger vehicles (LDPVs). To assess the real-world emissions and fuel economy performances of hybrid electric vehicles (HEVs) compared to conventional internal combustion engine (ICE) vehicles, on-road measurement...
Assessing the disparities of urban-rural air quality response to changes in emissions is essential for the development of effective air pollution mitigation strategies in megacities. However, meteorology and nonlinear atmospheric chemistry complicate the determination of emission-air quality responses. Here, we established a machine� learning (ML)-...
Accompanying with increases in vehicle population and gasoline consumption, gasoline evaporation accounted for an enlarged portion of total volatile organic compound (VOC) emissions in China, raising increasing environmental concerns especially in megacities. In this study, an intensive sampling campaign was performed in a gasoline service station,...
Ting Chen Xuan Zheng Xiao He- [...]
Ye Wu
Comprehensive characterization of diesel vehicle emitted polycyclic aromatic hydrocarbons (PAHs) emissions is yet to achieve due to the limitation of analytical methods. Therefore, we herein developed a two-dimensional gas chromatography time-of-flight mass spectrometry (GC × GC-ToF-MS) method and quantified the total PAHs from diesel vehicles base...
Xiao He Xuan Zheng Yan You- [...]
Ye Wu
Intermediate-volatility and semi-volatile organic compounds (I/SVOCs) are key precursors of secondary organic aerosol (SOA). However, the comprehensive characterization of I/SVOCs has long been an analytical challenge. Here, we develop a novel method of speciating and quantifying I/SVOCs using two-dimensional gas chromatography time-of-flight mass...
The spatial distribution of elevated particulate matter (PM) concentrations represents a public health concern due to its association with adverse health effects. In this study, a city-wide spatial variability of PM (PM10 and PM2.5) concentrations in Jinan, China is evaluated using a combination of measurements from 1700 fixed sites and taxi-based...
On-road vehicle emissions are a major contributor to significant atmospheric pollution in populous metropolitan areas. We developed an hourly link-level emissions inventory of vehicular pollutants using two land-use machine learning methods based on road traffic monitoring datasets in the Beijing–Tianjin–Hebei (BTH) region. The results indicate tha...
During the COVID-19 lockdown, the dramatic reduction of anthropogenic emissions provided a unique opportunity to investigate the effects of reduced anthropogenic activity and primary emissions on atmospheric chemical processes and the consequent formation of secondary pollutants. Here, we utilize comprehensive observations to examine the response o...
Plug-in electric vehicles (EVs) are expected to synergize with low or even zero-carbon electricity towards a deep mitigation of greenhouse gas (GHG) emission and ultimately carbon neutrality. These benefits are only obtainable when EV charging maximizes the consumption of electricity generated from renewable energy sources. However, the current mis...
Diesel vehicles have caused serious environmental problems in China. Hence, the Chinese government has launched serious actions against air pollution and imposed more stringent regulations on diesel vehicle emissions in the latest China VI standard. To fulfill this stringent legislation, two major technical routes, including the Exhaust Gas Recircu...
Significance
Solar photovoltaic power is gaining momentum as a solution to intertwined air pollution and climate challenges in China, driven by declining capital costs and increasing technical efficiencies. The dynamic spatial trajectory of cost-competitive and grid-compatible penetration potentials for solar power will be a critical determinant of...
The development of intelligent approaches to quantify and mitigate on-road emissions is essential for urban and transportation sustainability for global megacities. Here, we utilize high-density traffic monitoring data and land use data to train random forest models capable of accurately predicting dynamic, link-level vehicle emissions. A total of...
The plume-chasing method has been showing great advantages in measuring on-road emission factors (EFs) compared with regulatory methods like dynamometer and portable emission measurement systems (PEMS). In this study, a new on-board measurement system incorporating ultrasonic anemometers and solid-state Lidar was developed to investigate the uncert...
The Carbon Offsetting and Reduction Scheme for International Aviation (CORSIA) is the first programme to tackle carbon dioxide (CO2) emissions from a single industry at the global level, to realize the carbon-neutral growth of international flights from 2020 onwards. However, the COVID-19 pandemic has caused a drastic decline in the global aviation...
Significance
We capitalize on large variations of urban air quality during the COVID-19 pandemic and real-time observations of traffic, meteorology, and air pollution in Los Angeles to develop a machine-learning air pollution prediction model. Such a model can adequately account for the nonlinear relationships between emissions, atmospheric chemist...
The escalating concerns regarding air pollution problems surrounding port cities have attracted much research attention. The Port of Shenzhen is one of the busiest container ports worldwide, only third to Shanghai and Singapore globally. However, 70% of the freight transportation demand is satisfied via on-road trucks, leading to serious traffic co...
On-road vehicle emissions are a major contributor to significant atmospheric pollution in populous metropolitan areas. We developed an hourly-based, link-level emissions inventory of vehicular pollutants using two land-use machine learning methods based on the datasets of road traffic monitoring in the Beijing-Tianjin-Hebei (BTH) region. The result...
In roadside environments, commuters are exposed to a high level of traffic-related pollution. Despite vegetation is often used to mitigate air pollution in road environments, its air quality impacts are complex and could be both positive or negative depending on specific conditions. This study conducted field measurements to assess the air quality...
Black carbon (BC) is considered the second largest anthropogenic climate forcer, but the radiative effects of BC are highly correlated with its combustion sources. On-road vehicles are an important source of anthropogenic BC. However, there are major uncertainties in the estimates of the BC emissions from on-road light-duty passenger vehicles (LDPV...
Black carbon (BC) is the most potent light-absorbing component of particulate matter and can have a significant warming impact. On-road vehicles are a major source of BC and a significant contributor to global warming. This paper establishes an updated inventory to quantify the mitigation potential of efforts to control BC emissions from on-road tr...
Enhancing automobile fuel efficiency is crucial to decarbonizing the transport sector. Recent studies have revealed a gap between real-world fuel efficiency and results from laboratory tests, where “off-cycle” auxiliary devices, like air conditioning (AC) systems, are not turned on. AC consumes the most energy among all off-cycle devices; however,...
Start emissions from gasoline light-duty passenger vehicles (LDPVs) remain an important source of emissions modeling. This study measured start emissions of gaseous pollutants and solid particle number based on dynamometer tests for a fleet of 111 LDPVs in China, and selected a portion of samples to be tested under low temperature or shorter soak c...
Asia Pacific (AP) is the largest regional vehicle market and accounted for 48% of global sales in 2019. Air quality is a pressing issue in many AP countries and together with increased vehicle sales has led to intense scrutiny of vehicle emissions. The heterogeneity of socio-economic features and transportation patterns in AP countries has resulted...
China’s past economic growth has substantially relied on fossil fuels, causing serious air pollution issues. Decoupling economic growth and pollution has become the focus in developing ecological civilization in China. We have analyzed the three-decade progress of air pollution controls in China, highlighting a strategic transformation from emissio...
Many countries have adopted portable emissions measurement system (PEMS) testing in their latest regulations to measure real-world vehicular emissions. However, its fleetwide implementation is severely limited by the high equipment costs and lengthy setup procedures, posing a need to develop more cost-effective, efficient emission measurement metho...
The latest China VI emission standard has introduced a remote monitoring rule for regulating in-use emissions of heavy-duty diesel vehicles (HDDVs). Real-time data regarding engine and aftertreatment operating conditions and tailpipe nitrogen oxides (NOx) concentrations are required to be collected through electronic control unit and on-board NOx s...
An increasing discrepancy between real-world and type-approval fuel consumption for light-duty passenger vehicles (LDPVs) has been reported by several studies. Normally, real-world fuel consumption is measured primarily by a portable emission measurement system. The on-board diagnostic (OBD) approach, which is flexible and offers high-resolution da...
Energy security and climate change are critical concerns in the present era. The booming of the vehicle population has worsened the environment and has caused severe air pollution problems, especially in urban areas. The utilization of hydrogen-enriched compressed natural gas in internal combustion engines shows abundant prospects for improved perf...
Electric vehicles (EVs) play a crucial role in addressing climate change and urban air quality concerns. China has emerged as the global largest EV market with 1.2 million EVs sold in 2018. This study established a novel life cycle energy use and emission inventory collecting up-to-date data including the electricity generation mix, emission contro...
China's government has announced the mandatory, nationwide use of ethanol blended gasoline fuels (E10, namely, 10% ethanol blend) by 2020. It is necessary to assess the air quality and health impacts of E10 gasoline in China. This study compares two E10 gasoline fuels, ELA (lower content of aromatics) and ELO (lower content of olefins), assuming 10...
Emissions of major reactive nitrogen compounds, including nitric oxide (NO), nitrogen dioxide (NO2) and ammonia (NH3), from heavy-duty diesel vehicles (HDDVs) place substantial pressure on air quality for many large cities in China. To control nitrogen oxide (NOX) emissions from HDDVs, selective catalytic reduction (SCR) systems have been widely us...
Greenhouse gas (GHG) burdens of steel and aluminum production and life cycle benefits of vehicle lightweighting in China were evaluated. Production of advanced high-strength steel (AHSS) and wrought aluminum (Al) have average cradle-to-gate GHG emissions of 3.9 and 17.5 kg CO2eq/kg. Lightweighting benefits for eleven passenger car models over five...
The high populations of vehicles in global megacities have raised serious mobility and sustainability challenges, such as traffic congestion, air pollution deterioration and energy consumption issues. Detailed emission inventories at the link level are a prerequisite to accurately quantifying ambient pollution concentrations and identifying hotspot...