Richard M Lueptow

Northwestern University | NU · Department of Mechanical Engineering

The Discrete Element Method is widely employed for simulating granular flows, but conventional integration techniques may produce unphysical results for simulations with static friction when particle size ratios exceed $R \approx 3$. These inaccuracies arise because some variables in the velocity-Verlet algorithm are calculated at the half-timestep...

The origin of large and small particle axial bands in long rotating tumblers is a long-standing question. Using DEM simulations, we show that this axial segregation is due to a Rayleigh-Taylor instability which is characterized by the fact that the density of a granular medium increases with mixing and decreases with segregation. For initially mixe...

Predicting particle segregation has remained challenging due to the lack of a general model for the segregation velocity that is applicable across a range of granular flow geometries. Here, a segregation velocity model for dense granular flows is developed by exploiting momentum balance and recent advances in particle-scale modelling of the segrega...

Lift and drag forces on moving intruders in granular materials are of fundamental interest. While the drag force on an intruder in granular flow has been studied, the few studies characterizing the lift force explore a relatively limited range of parameters. Here we use discrete element method (DEM) simulations to measure the lift force, $F_\mathrm...

DOI:https://doi.org/10.1103/PhysRevE.110.039902

The origin of large and small particle axial bands in long rotating tumblers is a long-standing question. Using DEM simulations, we show that this axial segregation is due to a Rayleigh-Taylor instability which is characterized by the fact that the density of a granular medium increases with mixing and decreases with segregation. For initially mixe...

Membranes facilitate scalable and continuous lithium concentration from hypersaline salt lakes and battery leachates. Conventional nanofiltration (NF) membranes, however, exhibit poor monovalent selectivity in high‐salinity environments due to weakened exclusion mechanisms. This study examines polyamide NF membranes coated with polyelectrolytes enr...

Particle segregation in dense flowing size-disperse granular mixtures is driven by gravity and shear, but predicting the associated segregation force due to both effects has remained an unresolved challenge. Here, a model of the combined gravity- and kinematics-induced segregation force on a single intruder particle is integrated with a model of th...

Static granular packings play a central role in numerous industrial applications and natural settings. In these situations, fluid or fine particle flow through a bed of static particles is heavily influenced by the narrowest passage connecting the pores of the packing, commonly referred to as pore throats, or constrictions. Existing studies predomi...

Small particles fall through sheared beds of larger particles in settings ranging from geophysics to industry, but the study of large-to-small size ratios R , spanning the trapping threshold R t , has been neglected. In simulations of noncohesive spheres for R < R t , the small-sphere vertical velocity v p first increases with shear rate γ ̇ as tra...

Particle segregation in dense flowing size-disperse granular mixtures is driven by gravity and shear, but predicting the associated segregation force due to both effects has remained an unresolved challenge. Here, a model of the combined gravity-and kinematics-induced segregation force on a single intruder particle is integrated with a model of the...

In 1923, the Philosophical Transactions published G. I. Taylor’s seminal paper on the stability of what we now call Taylor–Couette flow. In the century since the paper was published, Taylor’s ground-breaking linear stability analysis of fluid flow between two rotating cylinders has had an enormous impact on the field of fluid mechanics. The paper’s...

In 1923, the Philosophical Transactions published G. I. Taylor’s seminal paper on the stability of what we now call Taylor–Couette flow. In the century since the paper was published, Taylor’s ground-breaking linear stability analysis of fluid flow between two rotating cylinders has had an enormous impact on the field of fluid mechanics. The paper’s...

We study the percolation of a fine spherical particle under gravity in static randomly packed large-particle beds with different packing densities ϕ and large to fine particle size ratios R ranging from 4 to 7.5 using discrete element method simulations. The particle size ratio at the geometrical trapping threshold, defined by three touching large...

In dense flowing bidisperse particle mixtures varying in size or density alone, smaller particles sink (percolation‐driven) and lighter particles rise (buoyancy‐driven). But when particle species differ from each other in both size and density, percolation and buoyancy can either enhance (large/light and small/heavy) or oppose (large/heavy and smal...

The drag force on a spherical intruder in dense granular shear flows is studied using discrete element method simulations. Three regimes of the intruder dynamics are observed depending on the magnitude of the drag force (or the corresponding intruder velocity) and the flow inertial number: a fluctuation-dominated regime for small drag forces, a vis...

In dense flowing bidisperse particle mixtures varying in size or density alone, smaller particles sink (driven by percolation) and lighter particles rise (driven by buoyancy). But when the particle species differ from each other in both size and density, percolation and buoyancy can either enhance (large/light and small/heavy) or oppose (large/heav...

Flow of size-bidisperse particle mixtures in a spherical tumbler rotating alternately about two perpendicular axes produces segregation patterns that track the location of nonmixing islands predicted by a dynamical systems approach. To better understand the paradoxical accumulation of large particles in regions defined by barriers to transport, we...

We present a continuum approach to model segregation of size-bidisperse granular materials in unsteady bounded heap flow as a prototype for modeling segregation in other time varying flows. In experiments, a periodically modulated feed rate produces stratified segregation like that which occurs due to intermittent avalanching, except with greater l...

Cut-and-shuffle mixing is an instructive candidate system with which to assess the potential of machine learning (ML) as an approach to solve difficult mixing problems. We focus on a specific subset of cut-and-shuffle systems, the one-dimensional interval exchange transform. This class of mixing operations is well studied, and a simple mixing metho...

Using simulations and a virtual-spring-based approach, we measure the segregation force, Fseg , in size-bidisperse sphere mixtures over a range of concentrations, particle-size ratios and shear rates to develop a semiempirical model for Fseg that extends its applicability from the well-studied non-interacting intruders regime to finite-concentratio...

Cut-and-shuffle mixing is an instructive candidate system with which to assess the potential of machine learning (ML) as an approach to solve difficult mixing problems. We focus on a specific subset of cut-and-shuffle systems, the one-dimensional interval exchange transform. This class of mixing operations is well studied, and a simple mixing metho...

Friction at the endwalls of partially filled horizontal rotating tumblers induces curvature and axial drift of particle trajectories in the surface flowing layer. Here we describe the results of a detailed discrete element method study of the dry granular flow of monodisperse particles in three-dimensional cylindrical tumblers with endwalls and cyl...

To better understand and optimize the capture of passive scalars (particles, pollutants, greenhouse gases, etc.) in complex geophysical flows, we study capture in the simpler, but still chaotic, time-dependent double-gyre flow model. For a range of model parameters, the domain of the double-gyre flow consists of a chaotic region, characterized by r...

Friction at the endwalls of partially-filled horizontal rotating tumblers induces curvature and axial drift of particle trajectories in the surface flowing layer. Here we describe the results of a detailed discrete element method study of the dry granular flow of monodisperse particles in threedimensional cylindrical tumblers with endwalls and cyli...

While polyamide-based reverse osmosis (RO) and nanofiltration (NF) membranes are widely used for desalination and water purification, the influence of membrane porosity and charge on water transport remains to be fully understood at a molecular level. Here we use molecular dynamics (MD) to build 56 distinct piperazine-based NF membranes models, whi...

Particle segregation is common in natural and industrial processes involving flowing granular materials. Complex, and seemingly contradictory, segregation phenomena have been observed for different boundary conditions and forcing. Using discrete element method simulations, we show that segregation of a single particle intruder can be described in a...

Using simulations and a virtual-spring-based approach, we measure the segregation force, Fseg, over a range of size-bidisperse mixture concentrations, particle size ratios, and shear rates to develop a model for Fseg that extends its applicability from the well-studied non-interacting intruders regime to finite-concentration mixtures where cooperat...

Flowing granular materials segregate due to differences in particle size (driven by percolation) and density (driven by buoyancy). Modelling the segregation of mixtures of large/heavy particles and small/light particles is challenging due to the opposing effects of the two segregation mechanisms. Using discrete element method (DEM) simulations of c...

Segregation, or demixing, of flowing mixtures of size-disperse noncohesive spherical particles is well understood. However, most particle systems in industry and geophysics involve nonspherical particles. Here, the segregation of bidisperse mixtures of millimeter-sized particles having various shapes is characterized using discrete element method s...

Particle segregation is common in natural and industrial processes involving flowing granular materials. Complex, and seemingly contradictory, segregation phenomena have been observed for different boundary conditions and forcing. Using discrete element method simulations, we show that segregation of a single particle intruder can be described in a...

In bidisperse particle mixtures varying in size or density alone, large particles rise (driven by percolation) and heavy particles sink (driven by buoyancy). When the two particle species differ from each other in both size and density, the two segregation mechanisms either enhance (large/light and small/heavy) or oppose (large/heavy and small/ligh...

Particle segregation in geophysical and industrial granular flows is typically driven by gravity and shear. While gravity-induced segregation is relatively well understood, shear-induced segregation is not. In particular, what controls segregation in the absence of gravity and the interplay between shear and gravity-driven segregation remain unclea...

In dense flowing bidisperse particle mixtures varying in size or density alone, large particles rise (driven by percolation) and heavy particles sink (driven by buoyancy). When the two particle species differ from each other in both size and density, the two segregation mechanisms either enhance (large/light and small/heavy) or oppose (large/heavy...

Flowing granular materials segregate due to differences in particle size (driven by percolation) and density (driven by buoyancy). Modelling the segregation of mixtures of large/heavy particles and small/light particles is challenging due to the opposing effects of the two segregation mechanisms. Using discrete element method (DEM) simulations of c...

We explore the segregation of two size-polydisperse particle species with overlapping size distributions using an experimentally validated continuum segregation model and discrete element method simulations. The continuum approach is extended to successfully model segregation for two species with overlapping size distributions. Nevertheless, the im...

Size-disperse mixtures of noncohesive particles segregate, or demix, during flow. For spherical particles, mixture segregation can be predicted based on the relative particle diameters. However, most particle systems in industry and geophysics involve nonspherical particles. Accounting for the immense range of particle shapes introduces additional...

We present a method to estimate the segregation parameter, $S,$ a key input in a continuum transport model of particulate flows. $S$ is determined by minimizing the difference between measured and model-predicted concentration profiles. To validate the approach, we conduct discrete element method simulations of size-bidisperse mixtures in quasi-2D...

Size segregation of polydisperse materials during hopper discharge is problematic in various industrial situations. However, due to the complexity of hopper discharge flow kinematics and limited prediction techniques for polydisperse segregation, accurate modeling of polydisperse segregation during hopper discharge has been challenging. We extend t...

We computationally determine the net bed force on single spherical intruder particles in dense granular flows as a function of particle size, particle density, shear rate, overburden pressure, and gravity. A simple buoyancy-like scaling law is recovered (analogous to that in fluids), but with a scale factor that depends on the particle size ratio d...

Free surface flows of granular materials in bounded axisymmetric geometries such as a cylindrical silo are poorly understood. In particular, a detailed description of the local three-dimensional velocity field and predictive models for segregation are lacking. Here, the details of the kinematics of flow in a rising conical heap formed by a centrall...

To apply an existing transport model to industrially relevant granular mixtures and flows, we demonstrate an approach to experimentally measure the segregation coefficient, S, and the flowing layer thickness, δ, using a modified quasi-2D bounded heap. During heap formation, the flowing layer velocity is characterized using particle image velocimetr...

Individual constituent balance equations are often used to derive expressions for species-specific segregation velocities in flows of dense granular mixtures. We propose a semiempirical expression for the interspecies momentum exchange in density-bidisperse granular flows as an extension of ideas from kinetic theory and compare it to a previous vis...

We present a method to estimate the segregation parameter, S, a key input in a continuum transport model of particulate flows. S is determined by minimizing the difference between measured and model-predicted concentration profiles. To validate the approach, we conduct discrete element method simulations of size-bidisperse mixtures in quasi-2D boun...

Individual constituent balance equations are often used to derive expressions for species specific segregation velocities in flows of dense granular mixtures. We propose a semi-empirical expression for the interspecies momentum exchange in density bidisperse granular flows as an extension of ideas from kinetic theory and compare it to a previous vi...

Free surface granular flows in bounded axisymmetric geometries are poorly understood. Here, we consider the kinematics and segregation of size‐bidisperse flow in a rising conical heap by characterizing the flow of particles in a wedge‐shaped silo with frictional sidewalls using experiments and discrete‐element‐method simulations. We find that the s...

Mixing by cutting and shuffling can be mathematically described by the dynamics of piecewise isometries (PWIs), higher dimensional analogs of one-dimensional interval exchange transformations. In a two-dimensional domain under a PWI, the exceptional set, E¯, which is created by the accumulation of cutting lines (the union of all iterates of cutting...

Size-driven particle segregation can occur when an object such as a blade moves through an otherwise static bed of granular material. Here we use discrete element method (DEM) simulations to study segregation resulting from a subsurface blade moving through a bed of size-bidisperse spherical particles. Segregation increases with each pass of the bl...

A discrete element model based on super-ellipsoids was used to simulate cylindrical particle flow. The model can describe a cylindrical particle accurately provided the shape indices of the super-ellipsoids are set to appropriate values. To achieve more rapid calculations, we implemented an “oriented bounding box algorithm” (OBBA) for the initial c...

Segregation patterns of size-bidisperse particle mixtures in a fully three-dimensional flow produced by alternately rotating a spherical tumbler about two perpendicular axes are studied over a range of particle sizes and volume ratios using both experiments and a continuum model. Pattern formation results from the interaction of size segregation wi...

Accurate continuum models of flow and segregation of dense granular flows are now possible. This is the result of extensive comparisons, over the last several years, of computer simulations of increasing accuracy and scale, experiments, and continuum models, in a variety of flows and for a variety of mixtures. Computer simulations—discrete element...

We computationally determine the force on single spherical intruder particles in sheared granular flows as a function of particle size, particle density, shear rate, overburden pressure, and gravitational acceleration. The force scales similarly to, but deviates from, the buoyancy force predicted by Archimedes' principle. The deviation depends only...

Mixing by cutting-and-shuffling can be mathematically described by the dynamics of piecewise isometries (PWIs), higher dimensional representations of one-dimensional interval exchange transformations. In a two-dimensional domain under a PWI, the exceptional set, $\bar{E}$, which is created by the accumulation of cutting lines (the union of all iter...

We examine the dynamics of cutting-and-shuffling a hemispherical shell driven by alternate rotation about two horizontal axes using the framework of piecewise isometry (PWI) theory. Previous restrictions on how the domain is cut-and-shuffled are relaxed to allow for nonorthogonal rotation axes, adding a new degree of freedom to the PWI. A new compu...

Cutting and shuffling is emerging as an alternative mixing mechanism for fluids and granular matter beyond the well established stretching and folding. Dynamical systems and chaos theory provided a foundation for stretching and folding which has led to applications ranging from microfluidic devices and physiological scales to many engineering and E...

Segregation patterns of size-bidisperse particle mixtures in a fully-three-dimensional flow produced by alternately rotating a spherical tumbler about two perpendicular axes are studied over a range of particle sizes and volume ratios using both experiments and a continuum model. Pattern formation results from the interaction of size segregation wi...

Predicting segregation and mixing of polydisperse granular materials in industrial processes remains a challenging problem. Here, we extend the application of a general predictive continuum model that captures the effects of segregation, diffusion, and advection in two ways. First, we consider polydisperse segregating flow in developing steady segr...

Discrete element method simulations of confined bidisperse granular shear flows elucidate the balance between diffusion and segregation that can lead to either mixed or segregated states, depending on confining pressure. Results indicate that the collisional diffusion is essentially independent of overburden pressure. Because the rate of segregatio...

We examine the dynamics of cutting-and-shuffling a hemispherical shell driven by alternate rotation about two horizontal axes using the framework of piecewise isometry (PWI) theory. Previous restrictions on how the domain is cut-and-shuffled are relaxed to allow for non-orthogonal rotation axes, adding a new degree of freedom to the PWI. A new comp...

We experimentally study the transition from steady flow to unsteady flow in a quasi-two-dimensional granular heap when small amounts of water are added to monodisperse glass spheres. Particles flow uniformly down both sides of the heap for low water content, but unsteady flow occurs as the water content increases. The unsteady flow mode consists of...

Discrete element method simulations of confined bidisperse granular shear flows elucidate the balance between diffusion and segregation that can lead to either mixed or segregated states, depending on confining pressure. Results indicate that the collisional diffusion is essentially independent of overburden pressure. Because the rate of segregatio...

We characterize the local concentration dependence of segregation velocity and segregation flux in both size and density bidisperse gravity-driven free-surface granular flows as a function of the particle size ratio and density ratio, respectively, using discrete element method simulations. For a range of particle size ratios and inlet volume flow...

Modeling segregation of size disperse granular materials during hopper discharge is important as hoppers are widely used in various industries. However, due to the complexity of segregation and hopper discharge flows, accurately modeling this process has been challenging. In this study, we apply a continuum transport model to predict segregation of...

Mixing of fluids and mixing of solids are both relatively mature fields. In contrast, mixing in systems where flowing and non-flowing regions coexist remains largely unexplored and little understood. Here we report remarkably persistent mixing and non-mixing regions in a three-dimensional dynamical system where randomness is expected. A spherical s...

The effect of confining pressure (overburden) on segregation of granular material is studied in discrete element method (DEM) simulations of horizontal planar shear flow. To mitigate changes to the shear rate due to the changing overburden, a linear with depth variation in the streamwise velocity component is imposed using a simple feedback scheme....