Marko Loncar

• Harvard University

Recent advancements in thin-film lithium niobate (TFLN) photonics have led to a new generation of high-performance electro-optic devices, including modulators, frequency combs, and microwave-to-optical transducers. However, the broader adoption of TFLN-based devices that rely on all-optical nonlinearities have been limited by the sensitivity of qua...

Quantum communications technologies require a network of quantum processors connected with low-loss and low-noise communication channels capable of distributing entangled states. Superconducting microwave qubits operating in cryogenic environments have emerged as promising candidates for quantum processor nodes. However, scaling these systems is ch...

The radiative properties of atoms are inherently linked to their surrounding environment. Placing an electromagnetic resonator around atoms can enhance spontaneous emission, as shown by Purcell in the 1940s. This approach is now routinely used in quantum computing and communication to channel photons emitted by atoms into well-defined modes and con...

Quantum memories based on emitters with optically addressable spins rely on efficient photonic interfaces, often implemented as nanophotonic cavities with ideally narrow spectral linewidths and small mode volumes. However, these approaches require nearly perfect spectral and spatial overlap between the cavity mode and quantum emitter, which can be...

We demonstrate a low half-wave voltage (0.7 V), high-bandwidth modulator in thin-film lithium niobate operating at near-infrared wavelengths (850 nm) and show the ability to transmit 60 GBd signals with direct electrical driving (400 mVpp). This paves the way for high-bandwidth, low-power, and compact optical engines for short-range optical communi...

Soliton microcombs are a cornerstone of integrated frequency comb technologies, with applications spanning photonic computing, ranging, microwave synthesis, optical communications, and quantum light generation. In nearly all such applications, electro-optic (EO) components play a critical role in generating, monitoring, stabilizing, and modulating...

Thin-film lithium niobate (TFLN) has emerged as a promising platform for the realization of high-performance chip-scale optical systems, spanning a range of applications from optical communications to microwave photonics. Such applications rely on the integration of multiple components onto a single platform. However, while many of these components...

In certain materials, the linear electro-optic (Pockels) effect allows direct control of the refractive index with an applied electric field. In practice, material inhomogeneities and defects cause the field inside the material to drift over macroscopic time scales. Such phenomena degrade the reliability and stability of integrated electro-optic de...

The ability to control phonons in solids is key in many fields of quantum science, ranging from quantum information processing to sensing. Phonons often act as a source of noise and decoherence when solid-state quantum systems interact with the phonon bath of their host matrix. In this study, we demonstrate the ability to control the phononic local...

Blind quantum computing (BQC) is a promising application of distributed quantum systems, where a client can perform computations on a remote server without revealing any details of the applied circuit. While the most promising realizations of quantum computers are based on various matter qubit platforms, implementing BQC on matter qubits remains an...

Practical quantum networks will require multi-qubit quantum nodes. This in turn will increase the complexity of the photonic circuits needed to control each qubit and require strategies to multiplex memories. Integrated photonics operating at visible to near-infrared (VNIR) wavelength range can provide solutions to these needs. In this work, we rea...

We demonstrate telecommunication-wavelength Pockels electro-optic modulators in thin-film lithium tantalate (TFLT) with superior DC stability compared to equivalent thin-film lithium niobate (TFLN) modulators. Less than 1 dB output power fluctuation for quadrature-biased TFLT is measured compared to 5 dB with TFLN over 46 hours with 12.1 dBm input...

The rapid growth in artificial intelligence and modern communication systems demands innovative solutions for increased computational power and advanced signaling capabilities. Integrated photonics, leveraging the analog nature of electromagnetic waves at the chip scale, offers a promising complement to approaches based on digital electronics. To f...

Here we show a photonic computing accelerator utilizing a system-level thin-film lithium niobate circuit which overcomes this limitation. Leveraging the strong electro-optic (Pockels) effect and the scalability of this platform, we demonstrate photonic computation at speeds up to 1.36 TOPS while consuming 0.057 pJ/OP. Our system features more than...

Deployment of terahertz communication and spectroscopy systems relies on the availability of low-noise and fast detectors, with plug-and-play capabilities. However, most currently available technologies are stand-alone, discrete components, either slow or susceptible to temperature drifts. Moreover, phase-sensitive schemes are mainly based on bulk...

Dissipative Kerr solitons from optical microresonators, commonly referred to as soliton microcombs, have been developed for a broad range of applications, including precision measurement, optical frequency synthesis, and ultra-stable microwave and millimeter wave generation, all on a chip. An important goal for microcombs is self-referencing, which...

Quantum information technology offers the potential to realize unprecedented computational resources via secure channels distributing entanglement between quantum computers. Diamond, as a host to optically-accessible spin qubits, is a leading platform to realize quantum memory nodes needed to extend such quantum links. Photonic crystal (PhC) caviti...

The field of integrated photonics has significantly impacted numerous fields including communication, sensing, and quantum physics owing to the efficiency, speed, and compactness of its devices. However, the reliance on off‐chip bulk lasers compromises the compact nature of these systems. While silicon photonics and III‐V platforms have established...

Thin-film lithium niobate (TFLN) has emerged as a promising platform for the realization of high-performance chip-scale optical systems, spanning a range of applications from optical communications to microwave photonics. Such applications rely on the integration of multiple components onto a single platform. However, while many of these components...

Modern communication and sensing technologies rely on connecting the optical domain with the microwave domain. Terahertz technologies, spanning increased frequencies from 100 GHz to 10 THz, are critical for providing larger bandwidths and faster switching capabilities. Despite progress in high-frequency electronic sources and detectors, these techn...

Stable pulse and flat-top frequency comb generation are an indispensable component of many photonic applications, from ranging to communications. Lithium niobate on insulator is an excellent electro-optic (EO) platform, exhibiting high modulation efficiency and low optical loss, making it a fitting candidate for pulse generation through electro-opt...

The recent emergence of thin-film lithium niobate (TFLN) has extended the landscape of integrated photonics. This has been enabled by the commercialization of TFLN wafers and advanced nanofabrication of TFLN such as high-quality dry etching. However, fabrication imperfections still limit the propagation loss to a few dB/m, restricting the impact of...

Resonator-based optical frequency comb generation is an enabling technology for a myriad of applications ranging from communications to precision spectroscopy. These frequency combs can be generated in nonlinear resonators driven using either continuous-wave (CW) light, which requires alignment of the pump frequency with the cavity resonance, or pu...

Ultra-small mode volume nanophotonic crystal cavities have been proposed as powerful tools for increasing coupling rates in cavity quantum electrodynamics systems. However, their adoption in quantum information applications remains elusive. In this work, we investigate possible reasons why, and analyze the impact of different low mode volume resona...

Recent advancements in thin-film lithium niobate (TFLN) photonics have led to a new generation of high-performance electro-optic devices, including modulators, frequency combs, and microwave-to-optical transducers. However, the broader adoption of TFLN-based devices that rely on all-optical nonlinearities have been limited by the sensitivity of qua...

Silicon vacancy centers (SiVs) in diamond have emerged as a promising platform for quantum sciences due to their excellent photostability, minimal spectral diffusion, and substantial zero-phonon line emission. However, enhancing their slow nanosecond excited-state lifetime by coupling to optical cavities remains an outstanding challenge, as current...

Solving large-scale computationally hard optimization problems using existing computers has hit a bottleneck. A promising alternative approach uses physics-based phenomena to naturally solve optimization problems, wherein the physical phenomena evolve to their minimum energy. In this regard, photonics devices have shown promise as alternative optim...

Thin-film lithium niobate (TFLN) is a promising electro-optic (EO) photonics platform with high modulation bandwidth, low drive voltage, and low optical loss. However, EO modulation in TFLN is known to relax on long timescales. Instead, thermo-optic heaters are often used for stable biasing, but heaters incur challenges with cross-talk, high power,...

Efficient generation, guiding, and detection of phonons, or mechanical vibrations, are of interest in various fields, including radio-frequency communication, sensing, and quantum information. Diamond is a useful platform for phononics because of the presence of strain-sensitive spin qubits, and its high Young’s modulus, which allows for low-loss g...

Distributing quantum information between remote systems will necessitate the integration of emerging quantum components with existing communication infrastructure. This requires understanding the channel-induced degradations of the transmitted quantum signals, beyond the typical characterization methods for classical communication systems. Here we...

Practical quantum networks require interfacing quantum memories with existing channels and systems that operate in the telecom band. Here we demonstrate low-noise, bidirectional quantum frequency conversion that enables a solid-state quantum memory to directly interface with telecom-band systems. In particular, we demonstrate conversion of visible-...

We demonstrate state-of-the-art ultra-low voltage (0.7V), high-bandwidth modulators in thin-film lithium niobate operating at near-infrared wavelengths (850nm) and show the ability to transmit 60 GBd signals with direct electrical driving (400 mV pp ).

We show progress towards the experimental demonstration of distributed blind quantum computing using a two node quantum network of Silicon-Vacancy (SiV) centres in diamond nanocavities.

We present an octave-spanning soliton microcomb in thin-film lithium niobate. The comb is connected between 126 and 252 THz, with repetition rate 491 . 85 GHz. Engineered coupling suppresses Raman lasing and enhances comb extraction.

We present emission up to 3 THz from a phase-matched terahertz-optical photonic circuit, featuring a co-planar metallic cavity traversed by an optical rib waveguide and a dipolar antenna for efficient out-coupling of terahertz waves.

We present an optically packaged thin film lithium niobate device. We show that this packaged device is capable of cryogenic operation and is resistant to extreme thermal shock.

We present a new class of thin-film lithium niobate integrated detectors, featuring a millimeter-long sensitive area and capable of performing the off-focus field-resolved reconstruction of sub-terahertz transients.

We engineer the interaction between phonons and single silicon-vacancy centers using phononic crystals with a complete bandgap spanning 50-70 GHz. We observe a 18-fold extension of single color center's orbital lifetime in the phononic bandgap.

We describe coherent optical control of a superconducting qubit with an electro-optic transducer as a step towards enabling optical interconnects between superconducting processor nodes.

We present the first experimental demonstration of backward stimulated Brillouin scattering in lithium niobate on insulator waveguides. We observed both intra- and intermodal scattering, showcasing gains up to G B = 10 m –1 W –1 .

We report on the controlled generation and annihilation of defects in photonic platforms using low-energy electron beams. We show how these defects impact propagation losses and EO-stability in LNOI, and how they can be rectified.

We report on near-infrared thin-film lithium niobate devices for scaling up quantum nodes. We demonstrate integrated low-insertion loss couplers, frequency shifters, laser pulse generators, switches, and more.

We discuss recent progress in miniaturizing terahertz devices, facilitated by integrated photonic circuits. We show these provide ways to engineer dispersion, achieve field enhancement and realise complex functionalities on a single chip.

We report photonic crystal cavities fabricated in a thin film diamond, featuring quality factors as high as ~2 x10 ⁵ in visible wavelengths, and we demonstrate coupling between the cavity mode and a single silicon-vacancy center.

The ferroelectric domains of thin-film lithium niobate are structured for multi-wavelength nonlinear optical frequency conversion. We target frequency-multiplexed photon-pair generation, in which we show conditions for five pair sources (purity > 90%) in a single waveguide.

We report progress on a process flow for fabricating wavelength-accurate quasi-phasematched frequency conversion devices in thin-film lithium niobate. Of 156 sampled devices, ~48% are phasematched within ±5 nm of a target second-harmonic generation process.

We demonstrate an integrated electro-optic Mach-Zehnder modulator in thin-film lithium tantalate at 737 nm with record low V π L of 0.65 Vcm. An extinction ratio of 30 dB and a detector-limited operating bandwidth of 20 GHz was measured.

Integrated photonic circuits from thin film lithium niobate are emerging as a promising platform to address the lack of miniaturized terahertz emitters and detectors within one single chip. In this talk, we will discover how terahertz transmission lines co-integrated with photonics fulfill the essential requirements for efficient terahertz-optical...

We propose a new approach to supercontinuum generation and carrier-envelope-offset detection based on saturated second-order nonlinear interactions in dispersion-engineered nanowaveguides. The technique developed here broadens the interacting harmonics by forming stable bifurcations of the pulse envelopes due to an interplay between phase-mismatch...

Robust, low-loss photonic packaging of on-chip nanophotonic circuits is a key enabling technology for the deployment of integrated photonics in a variety of classical and quantum technologies including optical communications and quantum communications, sensing, and transduction. To date, no process has been established that enables permanent, broad...

Distributing quantum information between remote systems will necessitate the integration of emerging quantum components with existing communication infrastructure. This requires understanding the channel-induced degradations of the transmitted quantum signals, beyond the typical characterization methods for classical communication systems. Here we...

Practical quantum networks require interfacing quantum memories with existing channels and systems that operate in the telecom band. Here we demonstrate low-noise, bidirectional quantum frequency conversion that enables a solid-state quantum memory to directly interface with telecom-band systems. In particular, we demonstrate conversion of visible-...

Optical isolators are indispensable components of almost any optical system and are used to protect a laser from unwanted reflections for phase-stable coherent operation. The emergence of chip-scale optical systems, powered by semiconductor lasers that are integrated on the same chip, has generated a demand for a fully integrated optical isolator....

Robust, low-loss photonic packaging of on-chip nanophotonic circuits is a key enabling technology for the deployment of integrated photonics in a variety of classical and quantum technologies including optical communications and quantum communications, sensing, and transduction. To date, no process has been established that enables permanent, broad...

Photonic integrated circuit based optical phased arrays (PIC-OPAs) are emerging as promising programmable processors and spatial light modulators, combining the best of planar and free-space optics. Their implementation on silicon photonic platforms has been especially fruitful. Despite much progress in this field, demonstrating steerable two-dimen...

Optical parametric oscillation (OPO) has widely been utilized as a means of generating light with wide spectral coverage from a single pump laser. These oscillators can be driven using either continuous-wave (CW) light, which only requires lining up of the pump frequency with OPO resonance, or pulsed light, which also mandates that the repetition r...

Integrated electro-optic (EO) modulators are fundamental photonics components with utility in domains ranging from digital communications to quantum information processing. At telecommunication wavelengths, thin-film lithium niobate modulators exhibit state-of-the-art performance in voltage-length product (VπL), optical loss, and EO bandwidth. Howe...

Correlated quantum phenomena in one-dimensional (1D) systems that exhibit competing electronic and magnetic order are of strong interest for the study of fundamental interactions and excitations, such as Tomonaga-Luttinger liquids and topological orders and defects with properties completely different from the quasiparticles expected in their highe...

Photonic integrated circuit based optical phased arrays (PIC-OPA) are emerging as promising programmable processors and spatial light modulators, combining the best of planar and free-space optics. Their implementation in silicon photonic platforms has been especially fruitful. Despite much progress in this field, demonstrating steerable two-dimens...

Lithium niobate (LN), first synthesized 70 years ago, has been widely used in diverse applications ranging from communications to quantum optics. These high-volume commercial applications have provided the economic means to establish a mature manufacturing and processing industry for high-quality LN crystals and wafers. Breakthrough science demonst...

Bridging the “terahertz gap“ relies upon synthesizing arbitrary waveforms in the terahertz domain enabling applications that require both narrow band sources for sensing and few-cycle drives for classical and quantum objects. However, realization of custom-tailored waveforms needed for these applications is currently hindered due to limited flexibi...

We realize a temporal magnifying and 2f system using a lithium-niobate-chip-based electro-optic time lens. We achieve a temporal magnification factor up to 7.25 and Fourier transform operation of the input pulses with sub-picosecond resolution.

We demonstrate visible sub-1 V amplitude and phase modulators in thin-film lithium niobate. We use these devices to demonstrate EO frequency shifting of pulsed light over 7 times the intrinsic pulse bandwidth.

We demonstrate a technique allowing scalable integration of III-V lasers on thin-film lithium niobate platform. Our method relies on an unconventional growth of the III-V epitaxial layer such that the n-layer ends on the top.

We perform low noise conversion of single photons from a diamond silicon vacancy color center to the telecom O-band. We demonstrate preservation of the photonic quantum properties, enabling their usage in deployed quantum networking applications.

We present an electro-optically modulated dissipative Kerr soliton with microwave-rate spacing over a 20 THz span, using thin-film lithium niobate. In this experiment, we first operate lithium niobate solitons with a laser power of 40 mW on chip. Electro-optic phase modulation of these solitons then generate a total of 570 frequency comb lines with...

Atomic-level defects in van der Waals (vdW) materials are essential building blocks for quantum technologies and quantum sensing applications. The layered magnetic semiconductor CrSBr is an outstanding candidate for exploring optically active defects because of a direct gap, in addition to a rich magnetic phase diagram, including a recently hypothe...

Optical isolator is an indispensable component of almost any optical system and is used to protect a laser from unwanted reflections for phase-stable coherent operation. The development of chip-scale optical systems, powered by semiconductor lasers integrated on the same chip, has resulted in a need for a fully integrated optical isolator. However,...

Surface-acoustic-wave (SAW) devices have a wide range of applications in microwave signal processing. Microwave SAW components benefit from higher quality factors and much smaller crosstalk when compared to their electromagnetic counterparts. Efficient routing and modulation of SAWs are essential for building large-scale and versatile acoustic wave...

Integrated femtosecond pulse and frequency comb sources are critical components for a wide range of applications, including optical atomic clocks1, microwave photonics2, spectroscopy3, optical wave synthesis4, frequency conversion5, communications6, lidar7, optical computing8 and astronomy9. The leading approaches for on-chip pulse generation rely...

Long-distance quantum communication and networking require quantum memory nodes with efficient optical interfaces and long memory times. We report the realization of an integrated two-qubit network node based on silicon-vacancy centers (SiVs) in diamond nanophotonic cavities. Our qubit register consists of the SiV electron spin acting as a communic...

Manipulating the frequency and bandwidth of nonclassical light is essential for implementing frequency-encoded/multiplexed quantum computation, communication, and networking protocols, and for bridging spectral mismatch among various quantum systems. However, quantum spectral control requires a strong nonlinearity mediated by light, microwave, or a...

A Project Scoping Workshop reports that the quantum information science and technology (QIST) community is ready to stand up five to ten large-scale National Science Foundation-supported Quantum Technology Demonstration Projects (QTDPs) - large-scale public-private partnerships - that have a high probability for translation from laboratory to pract...

Integrated electro-optic (EO) modulators are fundamental photonics components with utility in domains ranging from digital communications to quantum information processing. At telecommunication wavelengths, thin-film lithium niobate modulators exhibit state-of-the-art performance in voltage-length product ($V_\pi$L), optical loss, and EO bandwidth....

Mirrors are ubiquitous in optics and are used to control the propagation of optical signals in space. Here we propose and demonstrate frequency domain mirrors that provide reflections of the optical energy in a frequency synthetic dimension, using electro-optic modulation. First, we theoretically explore the concept of frequency mirrors with the in...

We measure the photothermal nonlinear response in suspended cubic silicon carbide (3C-SiC) and 3C-SiC-on-insulator (SiCOI) microring resonators. Bi-stability and thermo-optic hysteresis is observed in both types of resonators, with the suspended resonators showing a stronger response. A photothermal nonlinear index of 4.02×10⁻¹⁵ m²/W is determined...