Marcus Huber

University of Bristol | UB · School of Mathematics

The second law of thermodynamics states that the entropy of an isolated system can only increase over time. This appears to conflict with the reversible evolution of isolated quantum systems under the Schrödinger equation, which preserves the von Neumann entropy. Nonetheless, one finds that with respect to many observables, expectation values appro...

High-dimensional entangled states offer higher information capacity and stronger resilience to noise compared with two-dimensional systems. However, the large number of modes and sensitivity to random rotations complicate experimental entanglement certification. Here, we experimentally certify three-dimensional entanglement in a five-dimensional tw...

Controlled quantum machines have matured significantly. A natural next step is to increasingly grant them autonomy, freeing them from time-dependent external control. For example, autonomy could pare down the classical control wires that heat and decohere quantum circuits; and an autonomous quantum refrigerator recently reset a superconducting qubi...

High-dimensional encoding of quantum information holds the potential to greatly increase the computational power of existing devices by enlarging the accessible state space for fixed register size and by reducing the number of required entangling gates. However, qudit-based quantum computation remains far less developed than conventional qubit-base...

Physical devices operating out of equilibrium are inherently affected by thermal fluctuations, limiting their operational precision. This issue is pronounced at microscopic and especially quantum scales and can only be mitigated by incurring additional entropy dissipation. Understanding this constraint is crucial for both fundamental physics and te...

The second law of thermodynamics states that the entropy of an isolated system can only increase over time. This appears to conflict with the reversible evolution of isolated quantum systems under the Schr\"odinger equation, which preserves the von Neumann entropy. Nonetheless, one finds that with respect to many observables, expectation values app...

Quantum technologies have matured to the point that we can test fundamental quantum phenomena under extreme conditions. Specifically, entanglement, a cornerstone of modern quantum information theory, can be robustly produced and verified in various adverse environments. We take these tests further and implement a high-quality Bell experiment during...

High-dimensional entanglement has been identified as an important resource in quantum information processing, and also as a main obstacle for simulating quantum systems. Its certification is often difficult, and most widely used methods for experiments are based on fidelity measurements with respect to highly entangled states. Here, instead, we con...

We present an inequality on the purity of a bipartite state depending solely on the length difference of the local Bloch vectors. For two qubits this inequality is tight for all marginal states and so extends the previously known solution for the two-qubit marginal problem. With this inequality we construct a three-dimensional Bloch model of the tw...

We introduce two families of criteria for detecting and quantifying the entanglement of a bipartite quantum state of arbitrary local dimension. The first is based on measurements in mutually unbiased bases and the second is based on equiangular measurements. Both criteria give a qualitative result in terms of the state’s entanglement dimension and...

In order to unitarily evolve a quantum system, an agent requires knowledge of time, a parameter that no physical clock can ever perfectly characterize. In this Letter, we study how limitations on acquiring knowledge of time impact controlled quantum operations in different paradigms. We show that the quality of timekeeping an agent has access to li...

Gate-based universal quantum computation is formulated in terms of two types of operations: local single-qubit gates, which are typically easily implementable, and two-qubit entangling gates, whose faithful implementation remains one of the major experimental challenges since it requires controlled interactions between individual systems. To make t...

High‐dimensional photonic entanglement is a promising candidate for error‐protected quantum information processing with improved capacity. Encoding high‐dimensional qudits in the carrier frequency of photons combines ease of generation, universal single‐photon gates, and compatibility with fiber transmission for high‐capacity quantum communication....

Our study investigates the presence of high-dimensional entanglement in a recent demonstration of a noise-resistant quantum key distribution (QKD) protocol presented in [Phys. Rev. X 13, 021001 (2023)]. We determined that it is possible to certify the dimensionality of the distributed entangled states to be at least three. To demonstrate this, we d...

Computing the key rate in quantum key distribution (QKD) protocols is a long standing challenge. Analytical methods are limited to a handful of protocols with highly symmetric measurement bases. Numerical methods can handle arbitrary measurement bases, but either use the min-entropy, which gives a loose lower bound to the von Neumann entropy, or re...

We consider the problem of detecting the dimensionality of entanglement with the use of correlations between measurements in randomized directions. First, exploiting the recently derived covariance matrix criterion for the entanglement dimensionality [S. Liu et al., arXiv:2208.04909], we derive an inequality that resembles well-known entanglement c...

Entanglement distribution is at the heart of most quantum communication protocols. Inevitable loss of photons along quantum channels is a major obstacle for distributing entangled photons over long distances, as the no-cloning theorem forbids the information to simply be amplified along the way as is done in classical communication. It is therefore...

We introduce two families of criteria for detecting and quantifying the entanglement of a bipartite quantum state of arbitrary local dimension. The first is based on measurements in mutually unbiased bases and the second is based on equiangular measurements. Both criteria give a qualitative result in terms of the state's entanglement dimension and...

Entanglement distribution via photons over long distances enables many applications, including quantum key distribution, which provides unprecedented privacy. The inevitable degradation of entanglement through noise accumulated over long distances remains one of the key challenges in this area. Exploiting the potential of higher-dimensional entangl...

Thermodynamics connects our knowledge of the world to our capability to manipulate and thus to control it. This crucial role of control is exemplified by the third law of thermodynamics, Nernst’s unattainability principle, which states that infinite resources are required to cool a system to absolute zero temperature. But what are these resources a...

We present a novel inequality on the purity of a bipartite state depending solely on the difference of the local Bloch vector lengths. For two qubits this inequality is tight for all marginal states and so extends the previously known solution for the 2-qubit marginal problem and opens a new research avenue. We further use this inequality to constr...

Textbook quantum physics features two types of dynamics, reversible unitary dynamics and irreversible measurements. The latter stands in conflict with the laws of thermodynamics and has evoked debate on what actually constitutes a measurement. With the help of modern quantum statistical mechanics, we take the first step in formalising the hypothesi...

In order to unitarily evolve a quantum system, an agent requires knowledge of time, a parameter which no physical clock can ever perfectly characterise. In this letter, we study how limitations on acquiring knowledge of time impact controlled quantum operations in different paradigms. We show that the quality of timekeeping an agent has access to l...

In a recent quantum key distribution experiment, high-dimensional protocols were used to show an improved noise resistance over a 10.2 km free-space channel. One of the unresolved questions in this context is whether the communicating parties actually shared genuine high-dimensional entanglement. In this letter we introduce an improved discretisati...

From a thermodynamic point of view, all clocks are driven by irreversible processes. Additionally, one can use oscillatory systems to temporally modulate the thermodynamic flux towards equilibrium. Focusing on the most elementary thermalization events, this modulation can be thought of as a temporal probability concentration for these events. There...

We consider the problem of detecting the dimensionality of entanglement with the use of correlations between measurements in randomized directions. First, exploiting the recently derived covariance matrix criterion for the entanglement dimensionality [S. Liu \textit{et al.}, arXiv:2208.04909], we derive an inequality that resembles well-known entan...

Entanglement distribution is at the heart of most quantum communication protocols. Inevitable loss of photons along quantum channels is a major obstacle for distributing entangled photons over long distances, as the no-cloning theorem forbids the information to simply be amplified along the way as is done in classical communication. It is therefore...

Entanglement distribution is at the heart of most quantum communication protocols. Inevitable loss of photons along quantum channels is a major obstacle for distributing entangled photons over long distances, as the no-cloning theorem forbids the information to simply be amplified along the way as is done in classical communication. It is therefore...

High-dimensional entanglement has been identified as an important resource in quantum information processing, and also as a main obstacle for simulating quantum systems. Its certification is often difficult, especially because complicated fidelity measurements are needed for the most widely used methods. Here, we consider covariances of collective...

We investigate entanglement detection when the local measurements only nearly correspond to those intended. This corresponds to a scenario in which measurement devices are not perfectly controlled, but nevertheless operate with bounded inaccuracy. We formalize this through an operational notion of inaccuracy that can be estimated directly in the la...

We introduce finite-function-encoding (FFE) states which encode arbitrary d -valued logic functions, i.e., multivariate functions over the ring of integers modulo d , and investigate some of their structural properties. We also point out some differences between polynomial and non-polynomial function encoding states: The former can be associated to...

Entanglement shared among multiple parties presents complex challenges for the characterisation of different types of entanglement. One of the most fundamental insights is the fact that some mixed states can feature entanglement across every possible cut of a multipartite system yet can be produced via a mixture of states separable with respect to...

We investigate entanglement detection when the local measurements only nearly correspond to those intended. This corresponds to a scenario in which measurement devices are not perfectly controlled, but nevertheless operate with bounded inaccuracy. We formalise this through an operational notion of inaccuracy that can be estimated directly in the la...

We experimentally realize an entanglement distillation protocol which, against conventional wisdom, operates on a single photon pair entangled in two properties. This enables practical entanglement distillation which is orders of magnitude more efficient over long distances.

High-dimensional quantum entanglement is currently one of the most prolific fields in quantum information processing due to its high information capacity and error resilience. A versatile method for harnessing high-dimensional entanglement has long been hailed as an absolute necessity in the exploration of quantum science and technologies. Here we...

In general, generation of entangled photon pairs and also the random choice of measurement basis can be implemented with passive optical devices in entanglement based quantum key distribution (QKD) system. However, auxiliary random numbers are still mandatory for conducting the privacy amplification procedure. In this paper, we propose a fully pass...

Entanglement-based quantum communication offers an increased level of security in practical secret shared key distribution. One of the fundamental principles enabling this security—the fact that interfering with one photon will destroy entanglement and thus be detectable—is also the greatest obstacle. Random encounters of traveling photons, losses,...

The phenomenon of entanglement marks one of the furthest departures from classical physics and is indispensable for quantum information processing. Despite its fundamental importance, the distribution of entanglement over long distances through photons is unfortunately hindered by unavoidable decoherence effects. Entanglement distillation is a mean...

Geometric intuition is a crucial tool to obtain deeper insight into many concepts of physics. A paradigmatic example of its power is the Bloch ball, the geometrical representation for the state space of the simplest possible quantum system, a two-level system (or qubit). However, already for a three-level system (qutrit) the state space has eight d...

Entanglement measures quantify nonclassical correlations present in a quantum system, but can be extremely difficult to calculate, even more so, when information on its state is limited. Here, we consider broad families of entanglement criteria that are based on variances of arbitrary operators and analytically derive the lower bounds these criteri...

Beyond future applications, quantum networks open interesting fundamental perspectives, notably novel forms of quantum correlations. In this Letter we discuss quantum correlations in networks from the perspective of the underlying quantum states and their entanglement. We address the questions of which states can be prepared in the so-called triang...

Thermodynamics connects our knowledge of the world to our capability to manipulate and thus to control it. This crucial role of control is exemplified by the third law of thermodynamics, Nernst's unattainability principle, stating that infinite resources are required to cool a system to absolute zero temperature. But what are these resources? And h...

Entanglement shared among multiple parties presents complex challenges for the characterisation of different types of entanglement. One of the most basic insights is the fact that some mixed states can feature entanglement across every possible cut of a multipartite system, yet can be produced via a mixture of partially separable states. To disting...

Entanglement measures quantify nonclassical correlations present in a quantum system, but can be extremely difficult to calculate, even more so, when information on its state is limited. Here, we consider broad families of entanglement criteria that are based on variances of arbitrary operators and analytically derive the lower bounds these criteri...

According to thermodynamics, the inevitable increase of entropy allows the past to be distinguished from the future. From this perspective, any clock must incorporate an irreversible process that allows this flow of entropy to be tracked. In addition, an integral part of a clock is a clockwork, that is, a system whose purpose is to temporally conce...

The phenomenon of quantum entanglement marks one of the furthest departures from classical physics and is indispensable for quantum information processing. Despite its fundamental importance, the distribution of entanglement over long distances trough photons is unfortunately hindered by unavoidable decoherence effects. Entanglement distillation is...

Photons offer the potential to carry large amounts of information in their spectral, spatial, and polarisation degrees of freedom. While state-of-the-art classical communication systems routinely aim to maximize this information-carrying capacity via wavelength and spatial-mode division multiplexing, quantum systems based on multi-mode entanglement...

Quantum entanglement is one of the most important resources in quantum information. In recent years, the research of quantum entanglement mainly focused on the increase in the number of entangled qubits or the high-dimensional entanglement of two particles. Compared with qubit states, multipartite high-dimensional entangled states have beneficial p...

We investigate the encoding of higher-dimensional logic into quantum states. To that end we introduce finite-function-encoding (FFE) states which encode arbitrary $d$-valued logic functions and investigate their structure as an algebra over the ring of integers modulo $d$. We point out that the polynomiality of the function is the deciding property...

Geometric intuition is a crucial tool to obtain deeper insight into many concepts of physics. A paradigmatic example of its power is the Bloch ball, the geometrical representation for the state space of the simplest possible quantum system, a two-level system (or qubit). However, already for a three-level system (qutrit) the state space has eight d...

Entanglement based quantum communication offers an increased level of security in practical secret shared key distribution. One of the fundamental principles enabling this security -- the fact that interfering with one photon will destroy entanglement and thus be detectable -- is also the greatest obstacle. Random encounters of traveling photons, l...

High-dimensional quantum entanglement is currently one of the most prolific fields in quantum information processing due to its high information capacity and error resilience. A versatile method for harnessing high-dimensional entanglement has long been hailed as an absolute necessity in the exploration of quantum science and technologies. Here we...

According to thermodynamics, the inevitable increase of entropy allows the past to be distinguished from the future. From this perspective, any clock must incorporate an irreversible process that allows this flow of entropy to be tracked. In addition, an integral part of a clock is a clockwork, that is, a system whose purpose is to temporally conce...

High-dimensional entanglement promises to increase the information capacity of photons and is now routinely generated exploiting spatio-temporal degrees of freedom of single photons. A curious feature of these systems is the possibility to certify entanglement despite strong noise in the data. We show that it is also possible to exploit this noisy...

Photons offer the potential to carry large amounts of information in their spectral, spatial, and polarisation degrees of freedom. While state-of-the-art classical communication systems routinely aim to maximize this information-carrying capacity via wavelength and spatial-mode division multiplexing, quantum systems based on multi-mode entanglement...

Practical implementations of quantum technologies require one to prepare physical states with a high degree of purity---or, in thermodynamic terms, very low temperatures. The ability to do so is restricted by the Third Law of thermodynamics, which prohibits the attainability of perfect cooling given finite resources. For a finite dimensional system...

Entanglement and quantum interference are key ingredients in a variety of quantum information processing tasks. Harnessing the generation and characterization of entanglement in high-dimensional state spaces is a necessary prerequisite towards practical quantum protocols. Here, we use quantum interference on a beam splitter to engineer hyperentangl...

Beyond future applications, quantum networks open interesting fundamental perspectives, notably novel forms of quantum correlations. In this work we discuss quantum correlations in networks from the perspective of the underlying quantum states and their entanglement. We address the questions of which states can be prepared in the so-called triangle...

Unitary transformations are the fundamental building blocks of gates and operations in quantum information processing, allowing the complete manipulation of quantum systems in a coherent manner. In the case of photons, optical elements that can perform unitary transformations are readily available only for some degrees of freedom, e.g., wave plates...

We show that it is impossible to perform ideal projective measurements on quantum systems using finite resources. We identify three fundamental features of ideal projective measurements and show that when limited by finite resources only one of these features can be salvaged. Our framework is general enough to accommodate any system and measuring d...

Noise can be considered the natural enemy of quantum information. An often implied benefit of high-dimensional entanglement is its increased resilience to noise. However, manifesting this potential in an experimentally meaningful fashion is challenging and has never been done before. In infinite dimensional spaces, discretization is inevitable and...

From the perspective of quantum thermodynamics, realisable measurements cost work and result in measurement devices that are not perfectly correlated with the measured systems. We investigate the consequences for the estimation of work in non-equilibrium processes and for the fundamental structure of the work fluctuations when one assumes that the...

Cooling quantum systems is arguably one of the most important thermodynamic tasks connected to modern quantum technologies and an interesting question from a foundational perspective. It is thus of no surprise that many different theoretical cooling schemes have been proposed, differing in the assumed control paradigm and complexity, and operating...

In classical thermodynamics the work cost of control can typically be neglected. On the contrary, in quantum thermodynamics the cost of control constitutes a fundamental contribution to the total work cost. Here, focusing on quantum refrigeration, we investigate how the level of control determines the fundamental limits to cooling and how much work...

Correlations lie at the heart of almost all scientific predictions. It is therefore of interest to ask whether there exist general limitations to the amount of correlations that can be created at a finite amount of invested energy. Within quantum thermodynamics such limitations can be derived from first principles. In particular, it can be shown th...

Entanglement and quantum interference are key ingredients in a variety of quantum information processing tasks. Harnessing the generation and characterization of entanglement in high-dimensional state spaces is a necessary prerequisite towards practical quantum protocols. Here, we use quantum interference on a beam splitter to engineer hyperentangl...

We derive an inequality for the linear entropy, that gives sharp bounds for all finite dimensional systems. The derivation is based on generalised Bloch decompositions and provides a strict improvement for the possible distribution of purities for all finite dimensional quantum states. It thus extends the widely used concept of entropy inequalities...

Unitary transformations are the fundamental building blocks of gates and operations in quantum information processing allowing the complete manipulation of quantum systems while preserving crucial physical properties such as energy, orthogonality and entanglement. In the case of photons, optical elements that can perform unitary transformations are...

Entanglement is an important resource that allows quantum technologies to go beyond the classically possible. There are many ways quantum systems can be entangled, ranging from the archetypal two-qubit case to more exotic scenarios of entanglement in high dimensions or between many parties. Consequently, a plethora of entanglement quantifiers and c...

DOI:https://doi.org/10.1103/PhysRevLett.122.169901

Correlations lie at the heart of almost all scientific predictions. It is therefore of interest to ask whether there exist general limitations to the amount of correlations that can be created at a finite amount of invested energy. Within quantum thermodynamics such limitations can be derived from first principles. In particular, it can be shown th...

Noise can be considered the natural enemy of quantum information. An often implied benefit of high-dimensional entanglement is its increased resilience to noise. However, manifesting this potential in an experimentally meaningful fashion is challenging and has never been done before. In infinite dimensional spaces, discretisation is inevitable and...

We derive an inequality for the linear entropy, that gives sharp bounds for all finite dimensional systems. The derivation is based on generalised Bloch decompositions and provides a strict improvement for the possible distribution of purities for all finite dimensional quantum states. It thus extends the widely used concept of entropy inequalities...

In classical thermodynamics the work cost of control can typically be neglected. On the contrary , in quantum thermodynamics the cost of control constitutes a fundamental contribution to the total work cost. Here, focusing on quantum refrigeration, we investigate how the level of control determines the fundamental limits to cooling and how much wor...