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Introduction
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Polyoxometalates (POMs) are metal-oxo clusters formed by early transition metals in their highest oxidation state. More particularly, they exhibit adjustable redox properties, i.e. they can be reduced successively and reversibly to one or several electrons, such that they find their applications as redox mediators or electron reservoirs for electro...
![Figure 1. (left) cyclic voltammogram of K W Sn[COOH] in acetonitrile...](profile/Dominique-Vuillaume-2/publication/346014208/figure/fig1/AS:959569756954625@1605790666401/left-cyclic-voltammogram-of-K-W-SnCOOH-in-acetonitrile-with-TBAPF6-01-M-at-various_Q320.jpg)
![Figure 2. UV visible spectra of K W Si[COOH] (black), K W Sn[COOH]...](profile/Dominique-Vuillaume-2/publication/346014208/figure/fig2/AS:959569756958726@1605790666431/UV-visible-spectra-of-K-W-SiCOOH-black-K-W-SnCOOH-orange-and-K-W-SnH-green_Q320.jpg)
![Figure 5. Theoretical UV-visible spectra for K W Sn[H] and K W...](profile/Dominique-Vuillaume-2/publication/346014208/figure/fig3/AS:959569756975104@1605790666457/Theoretical-UV-visible-spectra-for-K-W-SnH-and-K-W-SiCOOH-calculated-at-the_Q320.jpg)
![Figure 6. (a) Scheme of the extreme orientations of the K W Sn[COOH]...](profile/Dominique-Vuillaume-2/publication/346014208/figure/fig4/AS:959569756946435@1605790666613/a-Scheme-of-the-extreme-orientations-of-the-K-W-SnCOOH-layer-on-Si-SiO2-b-11-mm_Q320.jpg)
Immobilization of polyoxometalates (POMs) onto oxides is relevant to many applications in the fields of catalysis, energy conversion/storage or molecular electronics. Optimization and understanding the molecule/oxide interface is crucial to rationally improve the performance of the final molecular materials. We herein describe the synthesis and cov...
![Figure 1. (Left) Cyclic voltammogram of K W Sn [COOH] in acetonitrile...](profile/Florence-Volatron/publication/344424340/figure/fig1/AS:1129536372654081@1646313865496/Left-Cyclic-voltammogram-of-K-W-Sn-COOH-in-acetonitrile-with-TBAPF-6-01-M-at-various_Q320.jpg)
![Figure 2. UV visible spectra of K W Si [COOH] (black), K W Sn [COOH]...](profile/Florence-Volatron/publication/344424340/figure/fig2/AS:1129536372649988@1646313865516/UV-visible-spectra-of-K-W-Si-COOH-black-K-W-Sn-COOH-orange-and-K-W-Sn-H_Q320.jpg)
![Figure 3. Frontier molecular orbitals for K W Si [COOH], calculated at...](profile/Florence-Volatron/publication/344424340/figure/fig3/AS:1129536372637696@1646313865526/Frontier-molecular-orbitals-for-K-W-Si-COOH-calculated-at-the-B3LYP-D3-def2-SVP_Q320.jpg)
![Figure 4. Frontier molecular orbitals for K W Sn [H], calculated at the...](profile/Florence-Volatron/publication/344424340/figure/fig4/AS:1129536372654082@1646313865561/Frontier-molecular-orbitals-for-K-W-Sn-H-calculated-at-the-B3LYP-D3-def2-SVP-Color_Q320.jpg)
![Figure 5. Theoretical UV−visible spectra for K W Sn [H] and K W Si...](profile/Florence-Volatron/publication/344424340/figure/fig5/AS:1129536372649989@1646313865602/Theoretical-UV-visible-spectra-for-K-W-Sn-H-and-K-W-Si-COOH-calculated-at-the_Q320.jpg)
Immobilization of polyoxometalates (POMs) onto oxides is relevant to many applications in the fields of catalysis, energy conversion/storage or molecular electronics. Optimization and understanding the molecule/oxide interface is crucial to rationally improve the performance of the final molecular materials. We herein describe the synthesis and cov...
