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Publications (303)
Pushing the sensitivity of nuclear magnetic resonance spectroscopy to the single spin level would have a major impact in chemistry and biology and is the goal of intense research efforts. Individual nuclear spins have been detected via their hyperfine coupling to an individual electronic paramagnetic system, itself measured by optical or electrical...
Single-photon detection played an important role in the development of quantum optics. Its implementation in the microwave domain is challenging because the photon energy is five orders of magnitude smaller. In recent years, significant progress has been made in developing single microwave photon detectors (SMPDs) based on superconducting quantum b...
Counting the microwave photons emitted by an ensemble of electron spins when they relax radiatively has recently been proposed as a sensitive method for electron paramagnetic resonance spectroscopy, enabled by the development of operational single microwave photon detectors at millikelvin temperature. Here, we report the detection of spin echoes in...
Electron spin resonance spectroscopy is the method of choice for characterizing paramagnetic impurities, with applications ranging from chemistry to quantum computing1,2, but it gives access only to ensemble-averaged quantities owing to its limited signal-to-noise ratio. Single-electron spin sensitivity has, however, been reached using spin-depende...
Single photon detection played an important role in the development of quantum optics. Its implementation in the microwave domain is challenging because the photon energy is 5 orders of magnitude smaller. In recent years, significant progress has been made in developing single microwave photon detectors (SMPDs) based on superconducting quantum bits...
Electron spin resonance (ESR) spectroscopy is the method of choice for characterizing paramagnetic impurities, with applications ranging from chemistry to quantum computing, but it gives access only to ensemble-averaged quantities due to its limited signal-to-noise ratio. Single-electron-spin sensitivity has however been reached using spin-dependen...
Erbium doped crystals offer a versatile platform for hybrid quantum devices because they combine magnetically sensitive electron-spin transitions with telecom-wavelength optical transitions. At the high doping concentrations necessary for many quantum applications, however, strong magnetic interactions of the electron-spin bath lead to excess spect...
Counting the microwave photons emitted by an ensemble of electron spins when they relax radiatively has recently been proposed as a sensitive method for electron paramagnetic resonance (EPR) spectroscopy, enabled by the development of operational Single Microwave Photon Detectors (SMPD) at millikelvin temperature. Here, we report the detection of s...
We observe the emission of bunches of k≥1 photons by a circuit made of a microwave resonator in series with a voltage-biased tunable Josephson junction. The bunches are emitted at specific values V_k of the bias voltage, for which each Cooper pair tunneling across the junction creates exactly k photons in the resonator. The latter is a microfabrica...
Erbium-doped crystals offer a versatile platform for hybrid quantum devices because they combine magnetically-sensitive electron-spin transitions with telecom-wavelength optical transitions. At the high doping concentrations necessary for many quantum applications, however, strong magnetic interactions of the electron-spin bath lead to excess spect...
Erbium ions embedded in crystals have unique properties for quantum information processing, because of their optical transition at 1.5 μm and of the large magnetic moment of their effective spin-1/2 electronic ground state. Most applications of erbium require, however, long electron spin coherence times, and this has so far been missing. Here, by s...
Quantum emitters respond to resonant illumination by radiating part of the absorbed energy. A component of this radiation field is phase coherent with the driving tone, whereas another component is incoherent and consists of spontaneously emitted photons, forming the fluorescence signal¹. Atoms, molecules and colour centres are routinely detected b...
We observe the emission of bunches of $k \geqslant 1$ photons by a circuit made of a microwave resonator in series with a voltage-biased tunable Josephson junction. The bunches are emitted at specific values $V_k$ of the bias voltage, for which each Cooper pair tunneling across the junction creates exactly k photons in the resonator. The latter is...
Electron spins are amongst the most coherent solid-state systems known. However, to be used in devices for quantum sensing and information processing applications, they must typically be placed near interfaces. Understanding and mitigating the impacts of such interfaces on the coherence and spectral properties of electron spins is critical to reali...
We show experimentally that a dc-biased Josephson junction in series with two microwave resonators emits entangled beams of microwaves leaking out of the resonators. In the absence of a stationary phase reference for characterizing the entanglement of the outgoing beams, we measure second-order coherence functions to prove the entanglement. The exp...
Erbium ions doped into crystals have unique properties for quantum information processing, because of their optical transition at 1.5 $\mu$m and of the large magnetic moment of their effective spin-1/2 electronic ground state. Most applications of erbium require however long electron spin coherence times, and this has so far been missing. Here, by...
The nanoscale localization of individual paramagnetic defects near an electrical circuit is an important step for realizing hybrid quantum devices with strong spin-microwave photon coupling. Here, we fabricate an array of individual nitrogen vacancy (NV) centers in diamond near a metallic nanowire deposited on top of the substrate. We determine the...
In their Comment [P. Hakonen and E. B. Sonin, preceding comment, Phys. Rev. X 11, 018001 (2021)], Hakonen and Sonin (HS) object to our conclusion on the absence of a dissipation-induced superconducting-to-insulating quantum phase transition (DQPT) in resistively shunted Josephson junctions (RSJJs) originally predicted by Schmid and Bulgadaev (SB)....
Quantum emitters respond to resonant illumination by radiating electromagnetic fields. A component of these fields is phase-coherent with the driving tone, while another one is incoherent, consisting of spontaneously emitted photons and forming the fluorescence signal. Atoms and molecules are routinely detected by their fluorescence at optical freq...
Electron spins are amongst the most coherent solid-state systems known, however, to be used in devices for quantum sensing and information processing applications, they must be typically placed near interfaces. Understanding and mitigating the impacts of such interfaces on the coherence and spectral properties of electron spins is critical to reali...
We report measurements of electron-spin-echo envelope modulation (ESEEM) performed at millikelvin temperatures in a custom-built high-sensitivity spectrometer based on superconducting micro-resonators. The high quality factor and small mode volume (down to 0.2 pL) of the resonator allow us to probe a small number of spins, down to 5×102. We measure...
We report long coherence times (up to 300 ms) for near-surface bismuth donor electron spins in silicon coupled to a superconducting microresonator, biased at a clock transition. This enables us to demonstrate the partial absorption of a train of weak microwave fields in the spin ensemble, their storage for 100 ms, and their retrieval, using a Hahn-...
The nanoscale localization of individual paramagnetic defects near an electrical circuit is an important step for realizing hybrid quantum devices with strong spin-microwave photon coupling. Here, we demonstrate the fabrication of an array of individual NV centers in diamond near a metallic nanowire deposited on top of the substrate. We determine t...
We show experimentally that a dc-biased Josephson junction in series with two microwave resonators emits entangled beams of microwaves leaking out of the resonators. In the absence of a stationary phase reference for characterizing the entanglement of the outgoing beams, we measure second-order coherence functions for proving entanglement up to an...
We report measurements of electron spin echo envelope modulation (ESEEM) performed at millikelvin temperatures in a custom-built high-sensitivity spectrometer based on superconducting micro-resonators. The high quality factor and small mode volume (down to 0.2 pL) of the resonator allow to probe a small number of spins, down to 5 ⋅ 102. We measure...
Physical systems reach thermal equilibrium through energy exchange with their environment, and for spins in solids the relevant environment is almost always their host lattice. However, recent studies1 motivated by observations by Purcell2 have shown how radiative emission into a microwave cavity can become the dominant relaxation path for spins if...
A long-lived multi-mode qubit register is an enabling technology for modular quantum computing architectures. For interfacing with superconducting qubits, such a quantum memory should be able to store incoming quantum microwave fields at the single-photon level for long periods of time, and retrieve them on-demand. Here, we demonstrate the partial...
We report electron spin resonance measurements of donors in silicon at millikelvin temperatures using a superconducting LC planar micro-resonator and a Josephson parametric amplifier. The resonator includes a nanowire inductor, defining a femtoliter detection volume. Due to strain in the substrate, the donor resonance lines are heavily broadened. S...
Half a century after its discovery, the Josephson junction has become the most important nonlinear quantum electronic component at our disposal. It has helped reshape the International System of Units around quantum effects and is used in scores of quantum devices. By itself, the use of Josephson junctions in volt metrology seems to imply an exquis...
We report electron spin resonance measurements of donors in silicon at millikelvin temperatures using a superconducting $LC$ planar micro-resonator and a Josephson Parametric Amplifier. The resonator includes a nanowire inductor, defining a femtoliter detection volume. Due to strain in the substrate, the donor resonance lines are heavily broadened....
We report measurements of electron spin echo envelope modulation (ESEEM) performed at millikelvin temperatures in a custom-built high-sensitivity spectrometer based on superconducting micro-resonators. The high quality factor and small mode volume (down to 0.2pL) of the resonator allow to probe a small number of spins, down to $5\cdot 10^2$. We mea...
Physical systems reach thermal equilibrium through energy exchange with their environment, and for spins in solids the relevant environment is almost always the host lattice in which they sit. However, recent studies motivated by observations from Purcell showed how coupling to a cavity can become the dominant form of relaxation for spins, given su...
When spin relaxation is governed by spontaneous emission of a photon into the resonator used for signal detection (the Purcell effect), the relaxation time $T_1$ depends on the spin-resonator frequency detuning $\delta$ and coupling constant $g$. We analyze the consequences of this unusual dependence for the amplitude and temporal shape of a spin-e...
Half a century after its discovery, the Josephson junction has become the most important nonlinear quantum electronic component at our disposal. It has helped reshaping the SI system around quantum effects and is used in scores of quantum devices. By itself, the use of Josephson junctions in the Volt metrology seems to imply an exquisite understand...
In high sensitivity inductive electron spin resonance spectroscopy, superconducting microwave resonators with large quality factors are employed. While they enhance the sensitivity, they also distort considerably the shape of the applied rectangular microwave control pulses, which limits the degree of control over the spin ensemble. Here, we employ...
We show experimentally that a dc biased Josephson junction in series with a high-enough impedance microwave resonator emits antibunched photons. Our resonator is made of a simple micro-fabricated spiral coil that resonates at 4.4 GHz and reaches a 1.97 k$\Omega$ characteristic impedance. The second order correlation function of the power leaking ou...
Within the last two decades, quantum technologies (QT) have made tremendous progress, moving from Nobel Prize award-winning experiments on quantum physics (1997: Chu, Cohen-Tanoudji, Phillips; 2001: Cornell, Ketterle, Wieman; 2005: Hall, Hänsch-, Glauber; 2012: Haroche, Wineland) into a cross-disciplinary field of applied research. Technologies are...
Nature sets fundamental limits regarding how accurate the amplification of analog signals may be. For instance, a linear amplifier unavoidably adds some noise which amounts to half a photon at best. While for most applications much higher noise levels are acceptable, the readout of microwave quantum systems, such as spin or superconducting qubits r...
DOI:https://doi.org/10.1103/PhysRevLett.120.049901
Within the last two decades, Quantum Technologies (QT) have made tremendous progress, moving from Noble Prize award-winning experiments on quantum physics into a cross-disciplinary field of applied research. Technologies are being developed now that explicitly address individual quantum states and make use of the 'strange' quantum properties, such...
We show that a properly dc-biased Josephson junction in series with two microwave resonators of different frequencies emits photon pairs in the resonators. By measuring auto- and inter-correlations of the power leaking out of the resonators, we demonstrate two-mode amplitude squeezing below the classical limit. This non-classical microwave light em...
We report electron spin resonance spectroscopy measurements performed at millikelvin temperatures in a custom-built spectrometer comprising a superconducting micro-resonator at $7$ GHz and a Josephson parametric amplifier. Owing to the small ${\sim}10^{-12}\lambda^3$ magnetic resonator mode volume and to the low noise of the parametric amplifier, t...
Although vacuum fluctuations appear to represent a fundamental limit to the sensitivity of electromagnetic field measurements, it is possible to overcome them by using so-called squeezed states. In such states, the noise in one field quadrature is reduced below the vacuum level while the other quadrature becomes correspondingly more noisy, as requi...
We present a new scheme for controlling the quantum state of a harmonic oscillator by coupling it to an anharmonic multilevel system (MLS) with first to second excited state transition frequency on-resonance with the oscillator. In this scheme that we call "ef-resonant", the spurious oscillator Kerr non-linearity inherited from the MLS is very smal...
Coherent control of quantum states has been demonstrated in a variety of superconducting devices. In all of these devices,
the variables that are manipulated are collective electromagnetic degrees of freedom: charge, superconducting phase, or flux.
Here we demonstrate the coherent manipulation of a quantum system based on Andreev bound states, whic...
Spontaneous emission of radiation is one of the fundamental mechanisms by
which an excited quantum system returns to equilibrium. For spins, however,
spontaneous emission is generally negligible compared to other non-radiative
relaxation processes because of the weak coupling between the magnetic dipole
and the electromagnetic field. In 1946, Purce...
We report the storage of microwave pulses at the single-photon level in a
spin-ensemble memory consisting of $10^{10}$ NV centers in a diamond crystal
coupled to a superconducting LC resonator. The energy of the signal, retrieved
$100\, \mu \mathrm{s}$ later by spin-echo techniques, reaches $0.3\%$ of the
energy absorbed by the spins, and this stor...
We report pulsed electron-spin resonance (ESR) measurements on an ensemble of
Bismuth donors in Silicon cooled at 10mK in a dilution refrigerator. Using a
Josephson parametric microwave amplifier combined with high-quality factor
superconducting micro-resonators cooled at millikelvin temperatures, we improve
the state-of-the-art sensitivity of indu...
We present preliminary measurements of the time resolved g2 function of the photons emitted by a dc biased Josephson junction embedded in a microwave resonator: the quantum fluctuations of the current through the junction couples to the resonator, so that a dc current flows through the junction when the transfer of a Cooper pair corresponds to the...
We derive fluctuation-dissipation relations for a tunnel junction driven by a
high impedance microwave resonator, displaying strong quantum fluctuations. We
find that the fluctuation-dissipation relations derived for classical forces
hold, provided the effect of the circuit's quantum fluctuations is incorporated
into a modified non-linear $I(V)$ cu...
We have developed and measured a high-gain quantum-limited microwave
parametric amplifier based on a superconducting lumped LC resonator with the
inductor L including an array of 8 superconducting quantum interference devices
(SQUIDs). This amplifier is parametrically pumped by modulating the flux
threading the SQUIDs at twice the resonator frequen...
Achieving individual qubit readout is a major challenge in the development of
scalable superconducting quantum processors. We have implemented the
multiplexed readout of a four transmon qubit circuit using non-linear
resonators operated as Josephson bifurcation amplifiers. We demonstrate the
simultaneous measurement of Rabi oscillations of the four...
We present measurements of superconducting flux qubits embedded in a three dimensional copper cavity. The qubits are fabricated on a sapphire substrate and are measured by coupling them inductively to an on-chip superconducting resonator located in the middle of the cavity. At their flux-insensitive point, all measured qubits reach an intrinsic ene...
We present a microscopic theory for the current through a tunnel Josephson
junction coupled to a non-linear environment, which consists of an Andreev
two-level system coupled to a harmonic oscillator. It models a recent
experiment (Nature 499, 312 (2013)) on photon spectroscopy of Andreev bound
states in a superconducting atomic-size contact. We fi...
This book gathers the lecture notes of courses given at the 2011 Les Houches Summer School in Theoretical Physics, Session XCVI. What is a quantum machine? Can we say that lasers and transistors are quantum machines? After all, physicists advertise these devices as the two main spin-offs of the understanding of quantum physics. However, while quant...
We observe the suppression of the finite frequency shot-noise produced by a
voltage biased tunnel junction due to its interaction with a single
electromagnetic mode of high impedance. The tunnel junction is embedded in a
quarter wavelength resonator containing a dense SQUID array providing it with a
characteristic impedance in the kOhms range and a...
In this work, we report the first measurements of flux qubits in 3D cavity and show that they can reach long and apparently more reproducible T1.
In this work, we present measurements of superconducting flux qubits embedded
in a three dimensional copper cavity. The qubits were fabricated on a sapphire
substrate and were measured by coupling them inductively to an on-chip
superconducting resonator located in the middle of the cavity. At their
flux-insensitive point, all measured qubits reach...
In addition to their central role in quantum information processing, qubits have proven to be useful tools in a range of other applications such as enhanced quantum sensing and as spectrometers of quantum noise. Here we show that a superconducting qubit strongly coupled to a nonlinear resonator can act as a probe of quantum fluctuations of the intr...
A quantum memory at microwave frequencies, able to store the state of
multiple superconducting qubits for long times, is a key element for quantum
information processing. Electronic and nuclear spins are natural candidates for
the storage medium as their coherence time can be well above one second.
Benefiting from these long coherence times require...
We report the efficient coupling of a 50 Ω microwave circuit to a high impedance conductor. We use an impedance transformer consisting of a λ/4 co-planar resonator whose inner conductor contains an array of superconducting quantum interference devices (SQUIDs), providing it with a tunable lineic inductance L∼80 μ0, resulting in a characteristic imp...
We measure the excitation spectrum of a superconducting atomic contact. In
addition to the usual continuum above the superconducting gap, the single
particle excitation spectrum contains discrete, spin-degenerate Andreev levels
inside the gap. Quasiparticle excitations are induced by a broadband on-chip
microwave source and detected by measuring ch...
In addition to their central role in quantum information processing, qubits
have proven to be useful tools in a range of other applications such as
enhanced quantum sensing and as spectrometers of quantum noise. Here we show
that a superconducting qubit strongly coupled to a nonlinear resonator can act
as a probe of quantum fluctuations of the intr...
The Josephson effect describes the flow of supercurrent in a weak link-such as a tunnel junction, nanowire or molecule-between two superconductors. It is the basis for a variety of circuits and devices, with applications ranging from medicine to quantum information. Experiments using Josephson circuits that behave like artificial atoms are now revo...
The Josephson effect describes how phase coherence is established
between two weakly coupled superconductors. Microscopically, the
Josephson current is carried by Cooper pairs, occupying Andreev Bound
States, localized at the weak link. Andreev Bound States, which come in
particle-hole symmetric pairs, consitute a spin-like degree of freedom.
In ou...