Baptiste Vignolle

• French National Centre for Scientific Research

Multilayered cuprates possess not only the highest superconducting temperature transition but also offer a unique platform to study disorder-free CuO2 planes and the interplay between competing orders with superconductivity. Here, we study the underdoped trilayer cuprate HgBa2Ca2Cu3O8+δ and we report quantum oscillation and Hall effect measurements...

Multilayered cuprates possess not only the highest superconducting temperature transition but also offer a unique platform to study disorder-free CuO$_2$ planes and the interplay between competing orders with superconductivity. Here, we study the underdoped trilayer cuprate HgBa$_2$Ca$_2$Cu$_3$O$_{8+ \delta}$ and we report the first quantum oscilla...

Despite immense efforts, the cuprate Fermi surface (FS) has been unambiguously determined in only two distinct, low-temperature regions of the phase diagram: a large hole-like FS at high doping, and a small electron-like pocket associated with charge-density-wave driven FS reconstruction at moderate doping. Moreover, there exists incomplete underst...

High-Tc cuprate superconductors host spin, charge, and lattice instabilities. In particular, in the antiferromagnetic glass phase, over a large doping range, lanthanum-based cuprates display a glass-like spin freezing with antiferromagnetic correlations. Previously, sound velocity anomalies in La2−xSrxCuO4 (LSCO) for hole doping p=x≥0.145 were repo...

High-Tc cuprate superconductors host spin, charge, and lattice instabilities. In particular, in the antiferromagnetic glass phase, over a large doping range, lanthanum-based cuprates display a glass-like spin freezing with antiferromagnetic correlations. Previously, sound velocity anomalies in La2−xSrxCuO4 (LSCO) for hole doping p=x≥0.145 were repo...

High-$T_{\rm{c}}$ cuprate superconductors host spin, charge and lattice instabilities. In particular, in the antiferromagnetic glass phase, over a large doping range, lanthanum based cuprates display a glass-like spin freezing with antiferromagnetic correlations. Previously, sound velocity anomalies in La$_{2-x}$Sr$_{x}$CuO$_4$ (LSCO) for hole dopi...

Solid $^4$He may acquire superfluid characteristics due to the frustration of the solid phase at grain boundaries. Here, we show that an analogous effect occurs in systems with competition among charge-density-waves (CDWs) and superconductivity in the presence of disorder, as cuprate or dichalcogenide superconductors. The CDWs breaks apart in domai...

Strong magnetic field induces at least two phase transitions in graphite beyond the quantum limit where many-body effects are expected. We report on a study using a state-of-the-art nondestructive magnet allowing us to attain 90.5 T at 1.4 K, which reveals a new field-induced phase and evidence that the insulating state destroyed at 75 T is an exci...

The perfectly linear temperature dependence of the electrical resistivity observed as T → 0 in a variety of metals close to a quantum critical point1–4 is a major puzzle of condensed-matter physics⁵. Here we show that T-linear resistivity as T → 0 is a generic property of cuprates, associated with a universal scattering rate. We measured the low-te...

The perfectly linear temperature dependence of the electrical resistivity observed as $T \rightarrow$ 0 in a variety of metals close to a quantum critical point is a major puzzle of condensed matter physics . Here we show that $T$-linear resistivity as $T \rightarrow$ 0 is a generic property of cuprates, associated with a universal scattering rate....

We present a detailed synchrotron x-ray scattering study of the charge-density-wave (CDW) order in simple tetragonal HgBa2CuO4+δ (Hg1201). Resonant soft x-ray scattering measurements reveal that short-range order appears at a temperature that is distinctly lower than the pseudogap temperature and in excellent agreement with a prior transient reflec...

We present an X-ray scattering study of charge-density-wave (CDW) order in simple tetragonal HgBa$_2$CuO$_{4+\delta}$ (Hg1201). Short-range order appears at a temperature that is distinctly lower than the pseudogap temperature and in excellent agreement with a prior transient reflectivity result. Despite considerable structural differences between...

The exciton dynamics in monolayer black phosphorus is investigated over a very wide range of photoexcited exciton densities using time resolved photoluminescence. At low excitation densities, the exciton dynamics is successfully described in terms of a double exponential decay. With increasing exciton population, a fast, non-exponential component d...

Superconductivity in cuprates peaks in the doping regime between a metal at high p and an insulator at low p. Understanding how the material evolves from metal to insulator is a fundamental and open question. Early studies in high magnetic fields revealed that below some critical doping an insulator-like upturn appears in the resistivity of cuprate...

The exciton dynamics in monolayer black phosphorus is investigated over a very wide range of photoexcited exciton densities using time resolved photoluminescence. At low excitation densities, the exciton dynamics is successfully described in terms of a double exponential decay. With increasing exciton population, a fast, non-exponential component d...

We present two methods to determine whether the interactions in a Tomonaga-Luttinger liquid (TLL) state of a spin-$1/2$ Heisenberg antiferromagnetic ladder are attractive or repulsive. The first method combines two bulk measurements, of magnetization and specific heat, to deduce the TLL parameter that distinguishes between the attraction and repuls...

Close to a zero temperature transition between ordered and disordered electronic phases, quantum fluctuations can lead to a strong enhancement of the electron mass and to the emergence of competing phases such as superconductivity. A correlation between the existence of such a quantum phase transition and superconductivity is quite well established...

Close to a zero-temperature transition between ordered and disordered electronic phases, quantum fluctuations can lead to a strong enhancement of electron mass and to the emergence of competing phases such as superconductivity. A correlation between the existence of such a quantum phase transition and superconductivity is quite well established in...

The pseudogap is a central puzzle of cuprate superconductors. Its connection to the Mott insulator at low doping $p$ remains ambiguous and its relation to the charge order that reconstructs the Fermi surface at intermediate $p$ is still unclear. Here we use measurements of the Hall coefficient in magnetic fields up to 88 T to show that Fermi-surfac...

arxiv paper, 29 pages 9 figures

The microscopic nature of an insulating state in the vicinity of a superconducting state, in the presence of disorder, is a hotly debated question. While the simplest scenario proposes that Coulomb interactions destroy the Cooper pairs at the transition, leading to localization of single electrons, an alternate possibility supported by experimental...

Our knowledge of the ground state of underdoped hole-doped cuprates has evolved considerably over the last few years. There is now compelling evidence that inside the pseudogap phase, charge order breaks translational symmetry leading to a reconstructed Fermi surface made of small pockets. Quantum oscillations, optical conductivity and the validity...

The Fermi surface of a metal is the fundamental basis from which its properties can be understood. In underdoped cuprate superconductors, the Fermi surface undergoes a reconstruction that produces a small electron pocket, but whether there is another, as yet undetected portion to the Fermi surface is unknown. Establishing the complete topology of t...

Two critical points have been revealed in the normal-state phase diagram of the electron-doped cuprate superconductor Nd$_{2-x}$Ce$_x$CuO$_4$ by exploring the Fermi surface properties of high quality single crystals by high-field magnetotransport. First, the quantitative analysis of the Shubnikov-de Haas effect shows that the weak superlattice pote...

In the quest to increase the critical temperature Tc of cuprate superconductors, it is essential to identify the factors that limit the strength of superconductivity. The upper critical field Hc2 is a fundamental measure of that strength, yet there is no agreement on its magnitude and doping dependence in cuprate superconductors. Here we show that...

The metallic state of the underdoped high-Tc cuprates has remained an enigma: How may seemingly disconnected Fermi surface segments, observed in zero magnetic field as a result of the opening of a partial gap (the pseudogap), possess conventional quasiparticle properties? How do the small Fermi-surface pockets evidenced by the observation of quantu...

Different instabilities have been speculated for a three-dimensional electron gas confined to its lowest Landau level. The phase transition induced in graphite by a strong magnetic field, and believed to be a Charge Density Wave (CDW), is the only experimentally established case of such instabilities. Studying the magnetoresistance in graphite for...

Driving a two-dimensional superconductor normal by applying a high magnetic field may lead to Cooper pair localization. In this case, there should be a quantum critical point associated with specific scaling laws. Such a transition has been evidenced in a number of low critical temperature superconducting thin films and has been suggested to occur...

It is generally thought that the upper critical field Hc2 of underdoped cuprate superconductors is far greater than the vortex-solid melting field Hvs at which the state of zero resistance ends, even at T = 0 [1]. Here we compare electrical measurements of Hvs and thermal measurements of Hc2 [2] in the cuprate YBCO and show that Hc2= Hvs at T ->0,...

The magnetic field driven superconductor/insulator transition is studied in a large variety of La2-xSrxCuO4 thin films of various Sr dopings. Temperature dependence of the resistivity down to 4.2 or 1.5 K under high pulsed magnetic field (up to 57 T) is analyzed. In particular, the existence of plateaus in the resistance versus temperature curves f...

This article constitutes an update made of numerous elements from an article by Vignolle et al. [C. R. Phys. 12 (2011) 446] published in the issue of C. R. Physique dedicated to superconductivity. By including this article to the present issue on physics in high magnetic field, we have aimed, in agreement with the editorial board of the review, off...

Charge density-wave order has been observed in cuprate superconductors whose crystal structure breaks the square symmetry of the CuO2 planes, such as orthorhombic YBa2Cu3Oy (YBCO), but not so far in cuprates that preserve that symmetry, such as tetragonal HgBa2CuO4+d (Hg1201). We have measured the Hall (R_H), Seebeck (S), and Nernst coefficients of...

Vortices in a type-II superconductor form a lattice structure that melts when the thermal displacement of the vortices is an appreciable fraction of the distance between vortices. In an anisotropic high-Tc superconductor, such as YBa2Cu3Oy, the magnetic field value where this melting occurs can be much lower than the mean-field critical field Hc2....

The magnetic field driven superconductor/insulator transition is studied in a large variety of $La_{2-x}Sr_xCuO_4$ thin films of various Sr dopings. Temperature dependence of the resistivity down to 4.2 or 1.5 K under high pulsed magnetic field (up to 57 T) is analyzed. In particular, the existence of plateaus in the resistance versus temperature c...

The electrical resistivity ρc of the underdoped cuprate superconductor YBa2Cu3Oy was measured perpendicular to the CuO2 planes on ultrahigh quality single crystals in magnetic fields large enough to suppress superconductivity. The incoherent insulating-like behavior of ρc at high temperature, characteristic of all underdoped cuprates, is found to c...

Over 20 years since the discovery of high temperature superconductivity in cuprates (Bednorz and Müller, 1986 [1]), the first convincing observation of quantum oscillations in underdoped YBa2Cu3O6.5 (Doiron-Leyraud et al., 2007 [2]) has deeply changed the theoretical landscape relevant to these materials. The Fermi surface is a basic concept of sol...

From analysis of the in-plane resistivity ρ(ab)(T) of La(2-x)Sr(x)CuO(4), we show that normal state transport in overdoped cuprates can be delineated into two regimes in which the electrical resistivity varies approximately linearly with temperature. In the low-temperature limit, the T-linear resistivity extends over a very wide doping range, in ma...

In underdoped cuprate superconductors, phase stiffness is low and long-range superconducting order is destroyed readily by thermally generated vortices (and anti-vortices), giving rise to a broad temperature regime above the zero-resistive state in which the superconducting phase is incoherent. It has often been suggested that these vortex-like exc...

The Hall coefficient R_H of the cuprate superconductor YBa2Cu3Oy was measured in magnetic fields up to 60 T for a hole concentration p from 0.078 to 0.152, in the underdoped regime. In fields large enough to suppress superconductivity, R_H(T) is seen to go from positive at high temperature to negative at low temperature, for p > 0.08. This change o...

We report transport measurements using pulsed magnetic fields to suppress the superconducting fluctuations (SCF) conductivity in a series of YBa_2Cu_3O_(6+x) samples. These experiments allow us altogether to measure the temperature T'c at which SCF disappear, and the pseudogap temperature T*. While the latter are consistent with previous determinat...

Measurements of quantum oscillations in the cuprate superconductors afford a new opportunity to assess the extent to which the electronic properties of these materials yield to a description rooted in Fermi liquid theory. However, such an analysis is hampered by the small number of oscillatory periods observed. Here we employ a genetic algorithm to...

We report on the doping dependence of the normal-state Hall coefficient RH(T) in the high-Tc superconductor YBa2Cu3Oy for 0.08 < p < 0.15, measured in magnetic fields up to 60 T. RH(T) is seen to drop below a temperature TH, to become negative at low temperature, as previously reported for two dopings (1). We attribute this drop to a reconstruction...

A study of the antiferromagnet CeRh2Si2 by torque, magnetostriction, and transport in pulsed magnetic fields up to 50 T and by thermal expansion in static fields up to 13 T is presented. The magnetic field temperature phase diagram of CeRh2Si2, where the magnetic field is applied along the easy axis c, is deduced from these measurements. The second...

A study of the antiferromagnet CeRh$_2$Si$_2$ by torque, magnetostriction, and transport in pulsed magnetic fields up to 50 Tesla and by thermal expansion in static fields up to 13 Tesla is presented. The magnetic field-temperature phase diagram of CeRh$_2$Si$_2$, where the magnetic field is applied along the easy axis $\mathbf{c}$, is deduced from...

Using the de Haas-van Alphen effect we have measured the evolution of the Fermi surface of BaFe2(As1-xPx){2} as a function of isoelectric substitution (As/P) for 0.41<x<1 (T{c} up to 25 K). We find that the volumes of electron and hole Fermi surfaces shrink linearly with decreasing x. This shrinking is accompanied by a strong increase in the quasip...

Using an elastic neutron scattering technique under a pulsed magnetic field up to 30 T, we determined the magnetic structure in the half-magnetization plateau phase in the spinel ${\mathrm{CdCr}}_{2}{\mathrm{O}}_{4}$. The magnetic structure has a cubic $P{4}_{3}32$ symmetry, which is the same as that observed in ${\mathrm{HgCr}}_{2}{\mathrm{O}}_{4}...

Shubnikov-de Haas and de Haas-van Alphen effects have been measured in the underdoped high temperature superconductor YBa$_2$Cu$_3$O$_{6.51}$. Data are in agreement with the standard Lifshitz-Kosevitch theory, which confirms the presence of a coherent Fermi surface in the ground state of underdoped cuprates. A low frequency $F = 530 \pm 10$ T is re...

From analysis of the in-plane resistivity $\rho_{ab}(T)$ of La$_{2-x}$Sr$_x$CuO$_4$, we show that normal state transport in overdoped cuprates can be delineated into two regimes in which the electrical resistivity varies approximately linearly with temperature. In the low temperature limit, the $T$-linear resistivity extends over a very wide doping...

We present a transport study of semi-metallic bismuth in presence of a magnetic field applied along the trigonal axis extended to 55 T for electric conductivity and to 45 T for thermoelectric response. The results uncover a new field scale at about 40 T in addition to the previously detected ones. Large anomalies in all transport properties point t...

We present the first application of pulsed high magnetic fields up to 30 T for neutron diffraction experiments. As the first study, field variations of a couple of magnetic Bragg reflections have successfully been measured in the frustrated antiferromagnet TbB4. The results show that the conventional models fail, and a model, which is a mixture of...

We use inelastic neutron scattering to measure the magnetic excitations in underdoped La2-xSrxCuO4 (x=0.085, Tc=22 K) for large energy (5<E<200 meV) and temperature (5<T<300 K) ranges. At low T, the response is highly structured in E and q, with peaks in the local susceptibility at 15 and 50 meV and a four-peaked structure in q for E185 meV. Raisin...

Shubnikov-de Haas and de Haas-van Alphen effects have been measured in the underdoped high temperature superconductor YBa2Cu3O6.51. Data are in agreement with the standard Lifshitz-Kosevitch theory, which confirms the presence of a coherent Fermi surface in the ground state of underdoped cuprates. A low frequency F=530±10 T is reported in both meas...

We use inelastic neutron scattering to measure the magnetic excitations in the underdoped superconductor La2-xSrxCuO4 (x=0.085, Tc=22 K) over wider energy (5

The presence or absence of a quantum critical point and its location in the phase diagram of high-temperature superconductors have been subjects of intense scrutiny. Clear evidence for quantum criticality, particularly in the transport properties, has proved elusive because the important low-temperature region is masked by the onset of superconduct...

The nature of the metallic phase in the high-transition-temperature (high-T(c)) copper oxide superconductors, and its evolution with carrier concentration, has been a long-standing mystery. A central question is how coherent electronic states, or quasiparticles, emerge from the antiferromagnetic insulator with doping. Recent quantum oscillation exp...

We use inelastic neutron scattering to measure the magnetic excitations in the underdoped superconductor La2-xSrxCuO4 (x=0.085, Tc=22 K) over energy and temperatures ranges 5 < E < 200 meV and 5 < T < 300 K respectively. At high temperature (T = 300 K), we observe strongly damped excitations with a characteristic energy scale of approximately 50 me...

The de Haas-van Alphen effect was observed in the underdoped cuprate YBa2Cu3O6.5 via a torque technique in pulsed magnetic fields up to 59 T. Above a field of approximately 30 T the magnetization exhibits clear quantum oscillations with a single frequency of 540 T and a cyclotron mass of 1.76 times the free electron mass, in excellent agreement wit...

The recent report of quantum oscillations in the single-chain underdoped cuprate YBa2Cu3O6.5 - ortho II (hole doping p˜0.10) points to the possibility that the underlying electronic structure in the underdoped region of the cuprate phase diagram contains Fermi surface pocket(s), at odds with results from ARPES experiments. In this talk I will descr...

We report the observation of Shubnikov-de Haas oscillations in the underdoped cuprate superconductor YBa2Cu4O8 (Y124). For fields aligned along the c axis, the frequency of the oscillations is 660+/-30 T, which corresponds to approximately 2.4% of the total area of the first Brillouin zone. The effective mass of the quasiparticles on this orbit is...

We report the observation of Shubnikov-de Haas oscillations in the underdoped cuprate superconductor YBa$_2$Cu$_4$O$_8$ (Y124). For field aligned along the c-axis, the frequency of the oscillations is $660\pm 30$ T, which corresponds to $\sim 2.4$ % of the total area of the first Brillouin zone. The effective mass of the quasiparticles on this orbi...

We report a detailed inelastic neutron scattering study of the collective magnetic excitations of overdoped superconducting La(1.78)Sr(0.22)CuO(4) for the energy range 0-160 meV. Our measurements show that overdoping suppresses the strong response present for optimally doped La(2-x)Sr(x)CuO(4) which is peaked near 50 meV. The remaining response is...

The excitations responsible for producing high-temperature superconductivity in the copper oxides have yet to be identified. Two promising candidates are collective spin excitations and phonons(1). A recent argument against spin excitations is based on their inability to explain structures observed in electronic spectroscopies such as photoemission...

Thenatureofthemetallicphaseinthehigh-transition-temperature (high-Tc) copper oxide superconductors, and its evolution with carrier concentration,has beena long-standingmystery 1 .Acentral question is how coherent electronic states, or quasiparticles, emerge from the antiferromagnetic insulator with doping. Recent quantum oscillation experiments on...