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An overview of WJ micronozzle (A and B) Internal view of the WJ micronozzle during operation (A) and outside view of the gas focused self-sequencing WJ observed at 0.5 bar applied gas pressure and 66 mL/s liquid flow rate (B) A perpendicular illustrating the 2D aspect of the droplet fan can be found in Figure S3. (C) Schematic representation of the WJ from a high-aspect-ratio WJ micronozzle. (D) Nozzle design parameters (left, see Table S1 for details), scanning electron microscopic image of polydimethylsiloxane (PDMS) nozzle (middle), and the high-aspect-ratio nozzle outlet (right).

An overview of WJ micronozzle (A and B) Internal view of the WJ micronozzle during operation (A) and outside view of the gas focused self-sequencing WJ observed at 0.5 bar applied gas pressure and 66 mL/s liquid flow rate (B) A perpendicular illustrating the 2D aspect of the droplet fan can be found in Figure S3. (C) Schematic representation of the WJ from a high-aspect-ratio WJ micronozzle. (D) Nozzle design parameters (left, see Table S1 for details), scanning electron microscopic image of polydimethylsiloxane (PDMS) nozzle (middle), and the high-aspect-ratio nozzle outlet (right).

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Well-defined aerosols pave the way for versatile basic and applied research. Here, we demonstrate a unique whipping instability that generates from a high-aspect-ratio microfluidic device resulting in a unique steady-state gas-focused whipping jet (WJ) without any need for electrification. This WJ device emanates a multi-monodisperse whipping spray...

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... we describe a new gas-focused whipping jet (WJ) microfluidic device to address these limitations that could emanate a novel multi-monodisperse whipping spray jet with a 2D profile with a similar nozzle operation as that of a gas-focused microfluidic nozzle. 2 The principal design and operation of this microfluidic device is shown in Figure 1 and is further described below and in Note S2. Here, we report our analytic derivation that predicts the whipping behavior of our new anisotropic microfluidic liquid jet device. ...
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... this study, we investigate the whipping behavior of an anisotropic microfluidic liquid jet device. This device is based on our previous polydimethylsiloxane (PDMS) gas dynamic virtual nozzle design, 2 but it features a higher PDMS central layer with 300 mm height (see Figure 1) and, hence, a rectangular/anisotropic structure. Unlike the commonly reported WJ devices, which typically emit a 3D cone pattern, 26,39 our WJ device produces a unique pattern of well-sorted, uniformly distributed, and 2D spray patterns (Figure 1). ...
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... device is based on our previous polydimethylsiloxane (PDMS) gas dynamic virtual nozzle design, 2 but it features a higher PDMS central layer with 300 mm height (see Figure 1) and, hence, a rectangular/anisotropic structure. Unlike the commonly reported WJ devices, which typically emit a 3D cone pattern, 26,39 our WJ device produces a unique pattern of well-sorted, uniformly distributed, and 2D spray patterns (Figure 1). An additional orthogonal view highlighting the 2D nature of the spray pattern can be found in Figure S3. ...
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... the evolution of lateral (m = 1) perturbations is a result of the competition between the destabilizing aerodynamic pressure r l (v 2 Àv 1 ) 2 associated with the slip velocity (v 2 Àv 1 ) and the restoring capillary stress due to the surface tension s. In the WJ device, a meniscus is formed at the exit of the main channel ( Figure S1) by the flow-focusing gas stream ( Figure 2A). The meniscus radius can be defined by the characteristic length (e), which depends on the shear tension stress. ...
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... 7 is used for calculating jet diameters in Figures 3B and 3C using a combination of literature values for the used fluids and experimentally fitted parameters (using Fiji, image processing package) as shown in Table S1. For a given scaling of WJ geometry, the semi-empirical equation of the spreading angle of WJ (q) can be written as (see supplemental information for derivation; Note S4) As shown above in Equation 8, the spreading angle (q) is a function of the ratio of critical jet flow rate (Q critical ) to the jet flow rate (Q) and the dimensions, i.e., width of the main channel (r i ), width of the outlet (r o ), and the central layer height device (h) (see Figure S1). ...
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... master mold fabrication process was started by spin coating a 3" silicon wafer with a negative photoresist (SU-8 2050, Microchem Co, USA). The designs ( Figure S1 A, B and C) were exposed under vacuum contact mode using a MJB4 mask aligner (Suss Micro Tech, Germany) in a sequence as outlined before. 1,2 In short, a sequences of layers was spin-coated and exposed using the steps outlined below to create two mold halves; one with the layers A+B+C, and one with the layers B+C. ...
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... activated device halves were aligned under a microscope and bound in an oven overnight at 45 0 C as shown in Figure S1. SEM images of nozzle outlet with high aspect ratios are shown in Figure S1. ...
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... activated device halves were aligned under a microscope and bound in an oven overnight at 45 0 C as shown in Figure S1. SEM images of nozzle outlet with high aspect ratios are shown in Figure S1. with respect to varying flow rate at applied gas pressure at constant 0.5 bar. ...