M. D. Lukin

Harvard University, Cambridge, MA, USA

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Publications (169)1034.65 Total impact

  • Source
    Article: Switching of Light with Light Using Cold Atoms Inside a Hollow Optical Fiber
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    ABSTRACT: eap/ We demonstrate a fiber-optical switch that operates with a few hundred pho-tons per switching pulse. The light-light interaction is mediated by laser-cooled atoms. The required strong interaction between atoms and light is achieved by simultaneously confining photons and atoms inside the microscopic hollow core of a single-mode photonic-crystal fiber.
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  • Article: Coupling a Single Trapped Atom to a Nanoscale Optical Cavity.
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    ABSTRACT: Hybrid quantum devices, where dissimilar quantum systems are combined to attain qualities not available with either system alone, may enable far-reaching control in quantum measurement, sensing, and information processing. A paradigmatic example is trapped ultra-cold atoms, which offer excellent quantum coherent properties, coupled to nanoscale solid-state systems, which allow for strong interactions. We demonstrate a deterministic interface between a single trapped rubidium atom and a nanoscale photonic crystal cavity. Precise control over the atom's position allows us to probe the cavity near-field with a resolution below the diffraction limit, and to observe large atom-photon coupling. This approach may enable the realization of integrated, strongly coupled quantum nano-optical circuits.
    Science 04/2013; · 31.20 Impact Factor
  • Article: Optical magnetic imaging of living cells.
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    ABSTRACT: Magnetic imaging is a powerful tool for probing biological and physical systems. However, existing techniques either have poor spatial resolution compared to optical microscopy and are hence not generally applicable to imaging of sub-cellular structure (for example, magnetic resonance imaging), or entail operating conditions that preclude application to living biological samples while providing submicrometre resolution (for example, scanning superconducting quantum interference device microscopy, electron holography and magnetic resonance force microscopy). Here we demonstrate magnetic imaging of living cells (magnetotactic bacteria) under ambient laboratory conditions and with sub-cellular spatial resolution (400 nanometres), using an optically detected magnetic field imaging array consisting of a nanometre-scale layer of nitrogen-vacancy colour centres implanted at the surface of a diamond chip. With the bacteria placed on the diamond surface, we optically probe the nitrogen-vacancy quantum spin states and rapidly reconstruct images of the vector components of the magnetic field created by chains of magnetic nanoparticles (magnetosomes) produced in the bacteria. We also spatially correlate these magnetic field maps with optical images acquired in the same apparatus. Wide-field microscopy allows parallel optical and magnetic imaging of multiple cells in a population with submicrometre resolution and a field of view in excess of 100 micrometres. Scanning electron microscope images of the bacteria confirm that the correlated optical and magnetic images can be used to locate and characterize the magnetosomes in each bacterium. Our results provide a new capability for imaging bio-magnetic structures in living cells under ambient conditions with high spatial resolution, and will enable the mapping of a wide range of magnetic signals within cells and cellular networks.
    Nature 04/2013; 496(7446):486-9. · 36.28 Impact Factor
  • Article: Coherence and Raman sideband cooling of a single atom in an optical tweezer.
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    ABSTRACT: We investigate quantum control of a single atom in a tightly focused optical tweezer trap. We show that inevitable spatially varying polarization gives rise to significant internal-state decoherence but that this effect can be mitigated by an appropriately chosen magnetic bias field. This enables Raman sideband cooling of a single atom close to its three-dimensional ground state (vibrational quantum numbers n[over ¯]_{x}=n[over ¯]_{y}=0.01, n[over ¯]_{z}=8) even for a trap beam waist as small as w=900 nm. The small atomic wave packet with δx=δy=24 nm and δz=270 nm represents a promising starting point for future hybrid quantum systems where atoms are placed in close proximity to surfaces.
    Physical Review Letters 03/2013; 110(13):133001. · 7.37 Impact Factor
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    Article: Topologically protected quantum state transfer in a chiral spin liquid.
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    ABSTRACT: Topology plays a central role in ensuring the robustness of a wide variety of physical phenomena. Notable examples range from the current-carrying edge states associated with the quantum Hall and the quantum spin Hall effects to topologically protected quantum memory and quantum logic operations. Here we propose and analyse a topologically protected channel for the transfer of quantum states between remote quantum nodes. In our approach, state transfer is mediated by the edge mode of a chiral spin liquid. We demonstrate that the proposed method is intrinsically robust to realistic imperfections associated with disorder and decoherence. Possible experimental implementations and applications to the detection and characterization of spin liquid phases are discussed.
    Nature Communications 03/2013; 4:1585. · 7.40 Impact Factor
  • Article: Phonon-induced spin-spin interactions in diamond nanostructures: application to spin squeezing
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    ABSTRACT: We propose and analyze a novel mechanism for long-range spin-spin interactions in diamond nanostructures. The interactions between electronic spins, associated with nitrogen-vacancy centers in diamond, are mediated by their coupling via strain to the vibrational mode of a diamond mechanical nanoresonator. This coupling results in phonon-mediated effective spin-spin interactions that can be used to generate squeezed states of a spin ensemble. We show that spin dephasing and relaxation can be largely suppressed, allowing for substantial spin squeezing under realistic experimental conditions. Our approach has implications for spin-ensemble magnetometry, as well as phonon-mediated quantum information processing with spin qubits.
    01/2013;
  • Article: Preparation of Non-equilibrium Nuclear Spin States in Double Quantum Dots
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    ABSTRACT: We theoretically study the dynamic polarization of lattice nuclear spins in GaAs double quantum dots containing two electrons. In our prior work [Phys. Rev. Lett. 104, 226807 (2010)] we identified three regimes of long-term dynamics, including the build up of a large difference in the Overhauser fields across the dots, the saturation of the nuclear polarization process associated with formation of so-called "dark states," and the elimination of the difference field. In particular, when the dots are different sizes we found that the Overhauser field becomes larger in the smaller dot. Here we present a detailed theoretical analysis of these problems including a systematic description of the polarization dynamics and the development of a new numerical method to efficiently simulate semiclassical-central-spin problems. When nuclear spin noise is included, the results agree with our prior work indicating that large difference fields and dark states are stable configurations, while the elimination of the difference field is unstable; however, in the absence of noise we find all three steady states are achieved depending on parameters. These results are in good agreement with dynamic nuclear polarization experiments in double quantum dots.
    12/2012;
  • Article: Topological Flat Bands from Dipolar Spin Systems.
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    ABSTRACT: We propose and analyze a physical system that naturally admits two-dimensional topological nearly flat bands. Our approach utilizes an array of three-level dipoles (effective S=1 spins) driven by inhomogeneous electromagnetic fields. The dipolar interactions produce arbitrary uniform background gauge fields for an effective collection of conserved hard-core bosons, namely, the dressed spin flips. These gauge fields result in topological band structures, whose band gap can be larger than the corresponding bandwidth. Exact diagonalization of the full interacting Hamiltonian at half-filling reveals the existence of superfluid, crystalline, and supersolid phases. An experimental realization using either ultracold polar molecules or spins in the solid state is considered.
    Physical Review Letters 12/2012; 109(26):266804. · 7.37 Impact Factor
  • Article: Nanoplasmonic Lattices for Ultracold Atoms.
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    ABSTRACT: We propose to use subwavelength confinement of light associated with the near field of plasmonic systems to create nanoscale optical lattices for ultracold atoms. Our approach combines the unique coherence properties of isolated atoms with the subwavelength manipulation and strong light-matter interaction associated with nanoplasmonic systems. It allows one to considerably increase the energy scales in the realization of Hubbard models and to engineer effective long-range interactions in coherent and dissipative many-body dynamics. Realistic imperfections and potential applications are discussed.
    Physical Review Letters 12/2012; 109(23):235309. · 7.37 Impact Factor
  • Article: Single-photon nonlinearities in two-mode optomechanics
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    ABSTRACT: We present a detailed theoretical analysis of a weakly driven multimode optomechanical system, in which two optical modes are strongly and near-resonantly coupled to a single mechanical mode via a three-wave mixing interaction. We calculate one- and two-time intensity correlations of the two optical fields and compare them to analogous correlations in atom-cavity systems. Nonclassical photon correlations arise when the optomechanical coupling $g$ exceeds the cavity decay rate $\kappa$, and we discuss signatures of one- and two-photon resonances as well as quantum interference. We also find a long-lived correlation that decays slowly with the mechanical decay rate $\gamma$, reflecting the heralded preparation of a single phonon state after detection of a photon. Our results provide insight into the quantum regime of multimode optomechanics, with potential applications for quantum information processing with photons and phonons.
    10/2012;
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    Article: Nanoscale magnetic imaging of a single electron spin under ambient conditions
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    ABSTRACT: The detection of ensembles of spins under ambient conditions has revolutionized the biological, chemical, and physical sciences through magnetic resonance imaging and nuclear magnetic resonance. Pushing sensing capabilities to the individual-spin level would enable unprecedented applications such as single molecule structural imaging; however, the weak magnetic fields from single spins are undetectable by conventional far-field resonance techniques. In recent years, there has been a considerable effort to develop nanoscale scanning magnetometers, which are able to measure fewer spins by bringing the sensor in close proximity to its target. The most sensitive of these magnetometers generally require low temperatures for operation, but measuring under ambient conditions (standard temperature and pressure) is critical for many imaging applications, particularly in biological systems. Here we demonstrate detection and nanoscale imaging of the magnetic field from a single electron spin under ambient conditions using a scanning nitrogen-vacancy (NV) magnetometer. Real-space, quantitative magnetic-field images are obtained by deterministically scanning our NV magnetometer 50 nanometers above a target electron spin, while measuring the local magnetic field using dynamically decoupled magnetometry protocols. This single-spin detection capability could enable single-spin magnetic resonance imaging of electron spins on the nano- and atomic scales and opens the door for unique applications such as mechanical quantum state transfer.
    09/2012;
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    Article: Magnetic field imaging with NV ensembles
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    ABSTRACT: We demonstrate a method of imaging spatially varying magnetic fields using a thin layer of nitrogen-vacancy (NV) centers at the surface of a diamond chip. Fluorescence emitted by the two-dimensional NV ensemble is detected by a CCD array, from which a vector magnetic field pattern is reconstructed. As a demonstration, AC current is passed through wires placed on the diamond chip surface, and the resulting AC magnetic field patterns are imaged using an echo-based technique with sub-micron resolution over a 140 \mu m x 140 \mu m field of view, giving single-pixel sensitivity ~100 nT/\sqrt{Hz}. We discuss ongoing efforts to further improve sensitivity and potential bioimaging applications such as real-time imaging of activity in functional, cultured networks of neurons.
    07/2012;
  • Article: Enhanced metrology using preferential orientation of nitrogen-vacancy centers in diamond
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    ABSTRACT: We demonstrate preferential orientation of nitrogen-vacancy (NV) color centers along two of four possible crystallographic axes in diamonds grown by chemical vapor deposition on the {100} face. We identify the relevant growth regime and present a possible explanation of this effect. We show that preferential orientation provides increased optical read-out contrast for NV multi-spin measurements, including enhanced AC magnetic field sensitivity, thus providing an important step towards high fidelity multi-spin-qubit quantum information processing, sensing and metrology.
    07/2012;
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    Article: Optomechanical quantum information processing with photons and phonons.
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    ABSTRACT: We describe how strong resonant interactions in multimode optomechanical systems can be used to induce controlled nonlinear couplings between single photons and phonons. Combined with linear mapping schemes between photons and phonons, these techniques provide a universal building block for various classical and quantum information processing applications. Our approach is especially suited for nano-optomechanical devices, where strong optomechanical interactions on a single photon level are within experimental reach.
    Physical Review Letters 07/2012; 109(1):013603. · 7.37 Impact Factor
  • Article: Dissipative phase transition in a central spin system
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    ABSTRACT: We investigate dissipative phase transitions in an open central spin system. In our model the central spin interacts coherently with the surrounding many-particle spin environment and is subject to coherent driving and dissipation. We develop analytical tools based on a self-consistent Holstein-Primakoff approximation that enable us to determine the complete phase diagram associated with the steady states of this system. It includes first- and second-order phase transitions, as well as regions of bistability, spin squeezing, and altered spin-pumping dynamics. Prospects of observing these phenomena in systems such as electron spins in quantum dots or nitrogen-vacancy centers coupled to lattice nuclear spins are briefly discussed.
    Physical Review A 07/2012; 86:012116. · 2.88 Impact Factor
  • Article: Reservoir engineering and dynamical phase transitions in optomechanical arrays
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    ABSTRACT: We study the driven-dissipative dynamics of photons interacting with an array of micromechanical membranes in an optical cavity. Periodic membrane driving and phonon creation result in an effective photon-number conserving non-unitary dynamics, which features a steady state with long-range photonic coherence. If the leakage of photons out of the cavity is counteracted by incoherent driving of the photonic modes, we show that the system undergoes a dynamical phase transition to the state with long-range coherence. A minimal system, composed of two micromechanical membranes in a cavity, is studied in detail, and it is shown to be a realistic setup where the key processes of the driven-dissipative dynamics can be seen.
    06/2012;
  • Article: Room-temperature quantum bit memory exceeding one second.
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    ABSTRACT: Stable quantum bits, capable both of storing quantum information for macroscopic time scales and of integration inside small portable devices, are an essential building block for an array of potential applications. We demonstrate high-fidelity control of a solid-state qubit, which preserves its polarization for several minutes and features coherence lifetimes exceeding 1 second at room temperature. The qubit consists of a single (13)C nuclear spin in the vicinity of a nitrogen-vacancy color center within an isotopically purified diamond crystal. The long qubit memory time was achieved via a technique involving dissipative decoupling of the single nuclear spin from its local environment. The versatility, robustness, and potential scalability of this system may allow for new applications in quantum information science.
    Science 06/2012; 336(6086):1283-6. · 31.20 Impact Factor
  • Article: Continuous mode cooling and phonon routers for phononic quantum networks
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    ABSTRACT: We study the implementation of quantum state transfer protocols in phonon networks, where in analogy to optical networks, quantum information is transmitted through propagating phonons in extended mechanical resonator arrays or phonon waveguides. We describe how the problem of a non-vanishing thermal occupation of the phononic quantum channel can be overcome by implementing optomechanical multi- and continuous mode cooling schemes to create a 'cold' frequency window for transmitting quantum states. In addition, we discuss the implementation of phonon circulators and switchable phonon routers, which rely on strong coherent optomechanical interactions only, and do not require strong magnetic fields or specific materials. Both techniques can be applied and adapted to various physical implementations, where phonons coupled to spin or charge based qubits are used for on-chip networking applications.
    05/2012;
  • Article: Measuring mechanical motion with a single spin
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    ABSTRACT: We study theoretically the measurement of a mechanical oscillator using a single two level system as a detector. In a recent experiment, we used a single electronic spin associated with a nitrogen vacancy center in diamond to probe the thermal motion of a magnetized cantilever at room temperature {Kolkowitz et al., Science 335, 1603 (2012)}. Here, we present a detailed analysis of the sensitivity limits of this technique, as well as the possibility to measure the zero point motion of the oscillator. Further, we discuss the issue of measurement backaction in sequential measurements and find that although backaction heating can occur, it does not prohibit the detection of zero point motion. Throughout the paper we focus on the experimental implementation of a nitrogen vacancy center coupled to a magnetic cantilever; however, our results are applicable to a wide class of spin-oscillator systems. Implications for preparation of nonclassical states of a mechanical oscillator are also discussed.
    05/2012;
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    Article: A robust scanning diamond sensor for nanoscale imaging with single nitrogen-vacancy centres.
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    ABSTRACT: The nitrogen-vacancy defect centre in diamond has potential applications in nanoscale electric and magnetic-field sensing, single-photon microscopy, quantum information processing and bioimaging. These applications rely on the ability to position a single nitrogen-vacancy centre within a few nanometres of a sample, and then scan it across the sample surface, while preserving the centre's spin coherence and readout fidelity. However, existing scanning techniques, which use a single diamond nanocrystal grafted onto the tip of a scanning probe microscope, suffer from short spin coherence times due to poor crystal quality, and from inefficient far-field collection of the fluorescence from the nitrogen-vacancy centre. Here, we demonstrate a robust method for scanning a single nitrogen-vacancy centre within tens of nanometres from a sample surface that addresses both of these concerns. This is achieved by positioning a single nitrogen-vacancy centre at the end of a high-purity diamond nanopillar, which we use as the tip of an atomic force microscope. Our approach ensures long nitrogen-vacancy spin coherence times (∼75 µs), enhanced nitrogen-vacancy collection efficiencies due to waveguiding, and mechanical robustness of the device (several weeks of scanning time). We are able to image magnetic domains with widths of 25 nm, and demonstrate a magnetic field sensitivity of 56 nT Hz(-1/2) at a frequency of 33 kHz, which is unprecedented for scanning nitrogen-vacancy centres.
    Nature Nanotechnology 04/2012; 7(5):320-4. · 27.27 Impact Factor

Institutions

  • 2001–200917
    • Harvard University
      • • Department of Physics
      • • Institute for Quantum Science and Engineering
      Cambridge, MA, USA
  • 2010
    • Max Planck Institute for the Physics of Complex Systems
      Dresden, Saxony, Germany
    • ETH Zurich
      • Institute of Quantum Electronics
      Zürich, ZH, Switzerland
  • 2009
    • Technische Universität Kaiserslautern
      • Fachbereich für Physik
      Kaiserslautern, Rhineland-Palatinate, Germany
  • 2003–2009
    • California Institute of Technology
      • Institute for Quantum Information and Matter
      Pasadena, CA, USA
  • 2000–2008
    • Harvard-Smithsonian Center for Astrophysics
      Cambridge, MA, USA
  • 2001–2006
    • Universität Innsbruck
      • Institut für Theoretische Physik
      Innsbruck, Tyrol, Austria
  • 1999
    • Texas A&M University
      College Station, TX, USA