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Article: Time-resolved photoelectron imaging using a femtosecond UV laser and a VUV free-electron laser
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ABSTRACT: A time-resolved photoelectron imaging using a femtosecond ultraviolet (UV) laser and a vacuum UV freeelectron laser is presented. Ultrafast internal conversion and intersystem crossing in pyrazine in a supersonic molecular beam were clearly observed in the time profiles of photoioinzation intensity and time-dependent photoelectron images.