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ABSTRACT: The evolution of the Fermi surface of CeRh(1-x)CoxIn5 was studied as a function of Co concentration x via measurements of the de Haas-van Alphen effect. By measuring the angular dependence of quantum oscillation frequencies, we identify a Fermi-surface sheet with f-electron character which undergoes an abrupt change in topology as x is varied. Surprisingly, this reconstruction does not occur at the quantum critical concentration x(c), where antiferromagnetism is suppressed to T=0. Instead we establish that this sudden change occurs well below x(c), at the concentration x approximately 0.4, where long-range magnetic order alters its character and superconductivity appears. Across all concentrations, the cyclotron effective mass of this sheet does not diverge, suggesting that critical behavior is not exhibited equally on all parts of the Fermi surface.
Physical Review Letters 09/2008; 101(5):056402. · 7.37 Impact Factor
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ABSTRACT: The evolution of the Fermi surface of CeRh$_{1-x}$Co$_x$In$_5$ was studied as a function of Co concentration $x$ via measurements of the de Haas-van Alphen effect. By measuring the angular dependence of quantum oscillation frequencies, we identify a Fermi surface sheet with $f$-electron character which undergoes an abrupt change in topology as $x$ is varied. Surprisingly, this reconstruction does not occur at the quantum critical concentration $x_c$, where antiferromagnetism is suppressed to T=0. Instead we establish that this sudden change occurs well below $x_c$, at the concentration x ~ 0.4 where long range magnetic order alters its character and superconductivity appears. Across all concentrations, the cyclotron effective mass of this sheet does not diverge, suggesting that critical behavior is not exhibited equally on all parts of the Fermi surface.
05/2008;
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ABSTRACT: Specific heat, magnetic susceptibility and electrical transport measurements were performed at ambient pressure on high-quality single crystal specimens of CeRhIn5 down to ultra-low temperatures. We report signatures of an anomaly observed in all measured quantities consistent with a bulk phase transition to a superconducting state at T_c=110 mK. Occurring far below the onset of antiferromagnetism at T_N=3.8 K, this transition appears to involve a significant portion of the available low-temperature density of electronic states, exhibiting an entropy change in line with that found in other members of the 115 family of superconductors tuned away from quantum criticality.
01/2008;
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ABSTRACT: A quantum critical point transforms the behavior of electrons so strongly that new phases of matter can emerge. The interactions at play are known to fall outside the scope of the standard model of metals, but a fundamental question remains: Is the basic concept of a quasiparticle-a fermion with renormalized mass-still valid in such systems? The Wiedemann-Franz law, which states that the ratio of heat and charge conductivities in a metal is a universal constant in the limit of zero temperature, is a robust consequence of Fermi-Dirac statistics. We report a violation of this law in the heavy-fermion metal CeCoIn5 when tuned to its quantum critical point, depending on the direction of electron motion relative to the crystal lattice, which points to an anisotropic destruction of the Fermi surface.
Science 07/2007; 316(5829):1320-2. · 31.20 Impact Factor
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ABSTRACT: One of the most notorious non-Fermi liquid properties of both archetypal heavy-fermion systems [1-4] and the high-Tc copper oxide superconductors [5] is an electrical resistivity that evolves linearly with temperature, T. In the heavy-fermion superconductor CeCoIn5 [5], this linear behaviour was one of the first indications of the presence of a zero-temperature instability, or quantum critical point. Here, we report the observation of a unique control parameter of T-linear scattering in CeCoIn5, found through systematic chemical substitutions of both magnetic and non-magnetic rare-earth, R, ions into the Ce sub-lattice. We find that the evolution of inelastic scattering in Ce1-xRxCoIn5 is strongly dependent on the f-electron configuration of the R ion, whereas two other key properties -- Cooper-pair breaking and Kondo-lattice coherence -- are not. Thus, T-linear resistivity in CeCoIn5 is intimately related to the nature of incoherent scattering centers in the Kondo lattice, which provides insight into the anomalous scattering rate synonymous with quantum criticality [7].
06/2007;
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ABSTRACT: Heat and charge transport were used to probe the magnetic field-tuned quantum critical point in the heavy-fermion metal CeCoIn5. A comparison of electrical and thermal resistivities reveals three characteristic energy scales. A Fermi-liquid regime is observed below T(FL), with both transport coefficients diverging in parallel and T(FL) -->0 as H --> Hc, the critical field. The characteristic temperature of antiferromagnetic spin fluctuations, T(SF), is tuned to a minimum but finite value at Hc, which coincides with the end of the T-linear regime in the electrical resistivity. A third temperature scale, T(QP), signals the formation of quasiparticles, as fermions of charge e obeying the Wiedemann-Franz law. Unlike T(FL), it remains finite at Hc, so that the integrity of quasiparticles is preserved, even though the standard signature of Fermi-liquid theory fails.
Physical Review Letters 09/2006; 97(10):106606. · 7.37 Impact Factor
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ABSTRACT: We show that the anomalous decrease in the thermal conductivity of cuprates below 300 mK, as has been observed recently in several cuprate materials including Pr$_{2-x}$Ce$_x$CuO$_{7-\delta}$ in the field-induced normal state, is due to the thermal decoupling of phonons and electrons in the sample. Upon lowering the temperature, the phonon-electron heat transfer rate decreases and, as a result, a heat current bottleneck develops between the phonons, which can in some cases be primarily responsible for heating the sample, and the electrons. The contribution that the electrons make to the total low-$T$ heat current is thus limited by the phonon-electron heat transfer rate, and falls rapidly with decreasing temperature, resulting in the apparent low-$T$ downturn of the thermal conductivity. We obtain the temperature and magnetic field dependence of the low-$T$ thermal conductivity in the presence of phonon-electron thermal decoupling and find good agreement with the data in both the normal and superconducting states.
04/2006;
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M A Tanatar, Johnpierre Paglione,
S Nakatsuji,
D G Hawthorn,
E Boaknin,
R W Hill,
F Ronning,
M Sutherland,
Louis Taillefer,
C Petrovic,
P C Canfield,
Z Fisk
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ABSTRACT: Thermal conductivity and specific heat were measured in the superconducting state of the heavy-fermion material Ce(1-x)La(x)CoIn5. With increasing impurity concentration x, the suppression of T(c) is accompanied by the increase in residual electronic specific heat expected of a d-wave superconductor, but it occurs in parallel with a decrease in residual electronic thermal conductivity. This contrasting behavior reveals the presence of uncondensed electrons coexisting with nodal quasiparticles. An extreme multiband scenario is proposed, with a d-wave superconducting gap on the heavy-electron sheets of the Fermi surface and a negligible gap on the light, three-dimensional pockets.
Physical Review Letters 09/2005; 95(6):067002. · 7.37 Impact Factor
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ABSTRACT: Heat and charge conduction were measured in the heavy-fermion metal CeRhIn(5), an antiferromagnet with T(N)=3.8 K. The thermal resistivity is found to be proportional to the magnetic entropy, revealing that spin fluctuations are as effective in scattering electrons as they are in disordering local moments. The electrical resistivity, governed by a q(2) weighting of fluctuations, increases monotonically with temperature. In contrast, the difference between thermal and electrical resistivities, characterized by a omega(2) weighting, peaks sharply at T(N) and eventually goes to zero at a temperature T(*) approximately = 8 K. T(*) thus emerges as a measure of the characteristic energy of magnetic fluctuations.
Physical Review Letters 07/2005; 94(21):216602. · 7.37 Impact Factor
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M. A. Tanatar, Johnpierre Paglione,
S. Nakatsuji,
D. G. Hawthorn,
E. Boaknin,
R. W. Hill,
F. Ronning,
M. Sutherland,
Louis Taillefer,
C. Petrovic,
P. C. Canfield,
Z. Fisk
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ABSTRACT: Thermal conductivity and specific heat were measured in the superconducting state of the heavy fermion material Ce_{1-x}La_{x}CoIn_{5}. With increasing impurity concentration x, the suppression of T_{c} is accompanied by the increase in the residual electronic specific heat expected of a d-wave superconductor, but it occurs in parallel with a decrease in residual electronic thermal conductivity. This contrasting behavior reveals the presence of uncondensed electrons coexisting with nodal quasiparticles. An extreme multiband scenario is proposed, with a d-wave superconducting gap on the heavy-electron sheets of the Fermi surface and a negligible gap on the light, three-dimensional pockets.
04/2005;
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D. G. Hawthorn,
S Y Li,
M. Sutherland,
Etienne Boaknin,
R. W. Hill,
C. Proust,
F. Ronning,
M. A. Tanatar, Johnpierre Paglione,
Louis Taillefer,
D. Peets,
Ruixing Liang,
D. A. Bonn,
W. N. Hardy,
N. N. Kolesnikov
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ABSTRACT: We present low-temperature thermal conductivity measurements on the cuprate Tl_2Ba_2CuO_{6+delta} throughout the overdoped regime. In the T -> 0 limit, the thermal conductivity due to d-wave nodal quasiparticles provides a bulk measurement of the superconducting gap, Delta. We find Delta to decrease with increasing doping, with a magnitude consistent with spectroscopic measurements (photoemission and tunneling). This argues for a pure and simple d-wave superconducting state in the overdoped region of the phase diagram, which appears to extend into the underdoped regime down to a hole concentration of 0.1 hole/Cu. As hole concentration is decreased, the gap-to-Tc ratio increases, showing that the suppression of the superconducting transition temperature Tc (relative to the gap) begins in the overdoped regime.
03/2005;
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ABSTRACT: The in-plane resistivity rho and thermal conductivity kappa of single crystal Na0.7CoO2 were measured down to 40 mK. Verification of the Wiedemann-Franz law, kappa/T=L(0)/rho as T-->0, and observation of a T2 dependence of rho at low temperature establish the existence of a well-defined Fermi-liquid state. The measured value of coefficient A reveals enormous electron-electron scattering, characterized by the largest Kadowaki-Woods ratio A/gamma(2) encountered in any material. The rapid suppression of A with magnetic field suggests a possible proximity to a magnetic quantum critical point. We also speculate on the possible role of magnetic frustration and proximity to a Mott insulator.
Physical Review Letters 07/2004; 93(5):056401. · 7.37 Impact Factor
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ABSTRACT: The in-plane resistivity, rho, and thermal conductivity, kappa, of a single crystal of Na_0.7CoO_2 were measured down to 40 mK. Verification of the Wiedemann-Franz law, kappa/T = L_0/rho as T -> 0, and observation of a T^2 dependence of rho at low temperature, rho = rho_0 + AT^2, establish the existence of a well-defined Fermi-liquid state. The measured value of coefficient A reveals enormous electron-electron scattering, characterized by the largest Kadowaki-Woods ratio, A/gamma^2, encountered in any material. The rapid suppression of A with magnetic field suggests a possible proximity to a magnetic quantum critical point. We also speculate on the possible role of magnetic frustration and proximity to a Mott insulator. Comment: 4 pages, 4 figures; replaced with published version; added references and supporting data
01/2004;
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ABSTRACT: The resistivity of the heavy-fermion superconductor CeCoIn5 was measured as a function of temperature, down to 25 mK and in magnetic fields of up to 16 T applied perpendicular to the basal plane. With increasing field, we observe a suppression of the non-Fermi liquid behavior, rho approximately T, and the development of a Fermi liquid state, with its characteristic rho=rho(0)+AT2 dependence. The field dependence of the T2 coefficient shows critical behavior with an exponent of 1.37. This is evidence for a field-induced quantum critical point (QCP), occurring at a critical field which coincides, within experimental accuracy, with the superconducting critical field H(c2). We discuss the relation of this field-tuned QCP to a change in the magnetic state, seen as a change in magnetoresistance from positive to negative, at a crossover line that has a common border with the superconducting region below approximately 1 K.
Physical Review Letters 01/2004; 91(24):246405. · 7.37 Impact Factor
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ABSTRACT: The resistivity of CeCoIn5 was measured down to 20 mK in magnetic fields of up to 16 T. With increasing field, we observe a suppression of the non-Fermi liquid behavior, ρ∼T, and the development of a Fermi liquid state, with its characteristic ρ=ρ0+AT2 dependence. The field dependence of the T2 coefficient shows critical behavior with an exponent of ∼4/3. This is evidence for a new field-induced quantum critical point, occurring in this case at a critical field which coincides with the superconducting upper critical field Hc2.
Physica C-superconductivity and Its Applications - PHYSICA C. 01/2004; 408:705-706.
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D G Hawthorn,
R W Hill,
C Proust,
F Ronning,
Mike Sutherland,
Etienne Boaknin,
C Lupien,
M A Tanatar, Johnpierre Paglione,
S Wakimoto,
H Zhang,
Louis Taillefer,
T Kimura,
M Nohara,
H Takagi,
N E Hussey
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ABSTRACT: The transport of heat and charge in cuprates was measured in single crystals of La(2-x)Sr(x)CuO(4+delta) (LSCO) across the doping phase diagram at low temperatures. In underdoped LSCO, the thermal conductivity is found to decrease with increasing magnetic field in the T-->0 limit, in striking contrast to the increase observed in all superconductors, including cuprates at higher doping. In heavily underdoped LSCO, where superconductivity can be entirely suppressed with an applied magnetic field, we show that a novel thermal metal-to-insulator transition takes place upon going from the superconducting state to the field-induced normal state.
Physical Review Letters 06/2003; 90(19):197004. · 7.37 Impact Factor
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ABSTRACT: The resistivity of CeCoIn_5 was measured down to 20 mK in magnetic fields of up to 16 T. With increasing field, we observe a suppression of the non-Fermi liquid behavior, rho~T, and the development of a Fermi liquid state, with its characteristic rho=rho_0+AT^2 dependence. The field dependence of the T^2 coefficient shows critical behavior with an exponent of ~4/3. This is evidence for a new field-induced quantum critical point, occuring in this case at a critical field which coincides with the superconducting upper critical field H_c2. Comment: 2 pages, 2 figures, submitted to M2S-Rio 2003 Proceedings
04/2003;
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Etienne Boaknin,
M. A. Tanatar, Johnpierre Paglione,
D. G. Hawthorn,
R. W. Hill,
F. Ronning,
M. Sutherland,
Louis Taillefer,
J. Sonier,
S. M. Hayden,
J. W. Brill
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ABSTRACT: The thermal conductivity of the layered s-wave superconductor NbSe_2 was measured down to T_c/100 throughout the vortex state. With increasing field, we identify two regimes: one with localized states at fields very near H_c1 and one with highly delocalized quasiparticle excitations at higher fields. The two associated length scales are most naturally explained as multi-band superconductivity, with distinct small and large superconducting gaps on different sheets of the Fermi surface. Comment: 2 pages, 2 figures, submitted to M2S-Rio 2003 Proceedings
04/2003;
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Etienne Boaknin,
M A Tanatar, Johnpierre Paglione,
D Hawthorn,
F Ronning,
R W Hill,
M Sutherland,
Louis Taillefer,
Jeff Sonier,
S M Hayden,
J W Brill
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ABSTRACT: The thermal conductivity kappa of the layered s-wave superconductor NbSe2 was measured down to T(c)/100 throughout the vortex state. With increasing field, we identify two regimes: one with localized states at fields very near H(c1) and one with highly delocalized quasiparticle excitations at higher fields. The two associated length scales are naturally explained as multiband superconductivity, with distinct small and large superconducting gaps on different sheets of the Fermi surface. This behavior is compared to that of the multiband superconductor MgB2 and the conventional superconductor V3Si.
Physical Review Letters 04/2003; 90(11):117003. · 7.37 Impact Factor
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D. G. Hawthorn,
R. W. Hill,
C. Proust,
F. Ronning,
Mike Sutherland,
Etienne Boaknin,
C. Lupien,
M. A. Tanatar, Johnpierre Paglione,
S. Wakimoto,
H Zhang,
Louis Taillefer,
T Kimura,
M. Nohara,
H Takagi,
N. E. Hussey
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ABSTRACT: The transport of heat and charge in cuprates was measured in single crystals of La_{2-x}Sr_xCuO_{4+\delta} (LSCO) across the doping phase diagram at low temperatures. In underdoped LSCO, the thermal conductivity is found to decrease with increasing magnetic field in the T goes to 0 limit, in striking contrast to the increase observed in all superconductors, including cuprates at higher doping. In heavily underdoped LSCO, where superconductivity can be entirely suppressed with an applied field, we show that a novel thermal metal-to-insulator transition takes place upon going from the superconducting state to the field-induced normal state. Comment: 4 pages, 3 figures, minor changes, replaced with published version
01/2003;
