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ABSTRACT: The title compound, [Nd(OH)(SO4)]n, was obtained hydrothermally from an aqueous solution of neodymium nitrate, 1,2-propanediamine and sulfuric acid. The structure features nonacoordinated neodymium with sulfate and hydroxide anions acting as bridging ligands. The OH group forms a weak O—H...O hydrogen bond with an O...O distance of 3.224 (5) Å.