Publications (41)31.97 Total impact
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Article: Sonkaew, T., C. von Savigny, K.-U. Eichmann, M. Weber, A. Rozanov, H. Bovensmann, and J. P. Burrows, Chemical ozone loss in Arctic and Antarctic polar winter/spring season derived from SCIAMACHY limb measurements 2002-2009, Atmos. Chem. Phys., 13, doi:10.5194/acp-13-1809-2013, 1809-1835, 2013
ATMOSPHERIC CHEMISTRY AND PHYSICS 01/2013; 13:1809-1835. · 5.52 Impact Factor -
Chapter: Investigation of solar irradiance variations and their impact on middle atmospheric ozone
01/2013; -
Dataset: Error Budget and SCIAMACHY LImb Ozone Datasets
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ABSTRACT: Impacts of parameter uncertainties on the retrieved ozone profiles have been investigated. In the first step the ozone profile retrieved from synthetic observations by using the SCIATRAN code for a given reference parameter can be compared with a set of profiles with different values of the same parameter. For example in order to calculate the possible impact of albedo A on the retrieved ozone profiles, a reference scenario of A_ref can be defined. In the second step the retrieval is then run with different albedo values. The relative uncertainties σ for a given altitude z are calculated with following relation: SCIAMACHY Limb Ozone: Error budget and data versions Ozone(A_ref+0.4, z) σ (dA: 0.4, z) = Ozone(A_ref, z) Ozone(A_ref, z) With Ozone(A_ref, z) as the ozone numbre density with the A_ref of 0.3 in the following example (See Fig. 1). Error Budget According to the error estimation for each individual parameter a total error budget can be established for the SCIAMACHY limb ozone retrieval. In our study we used the calculation for one orbit (1.Aug.2008, Orbit 33566). The corresponding average error profiles are shown for the following parameters: albedo, aerosol, pressure, temperature, tangent height and standard deviation (Fig. 2, from left top panel to left bottom panel). Figure 1. An example of calculated ozone error profile. -
Article: Mieruch, S., M. Weber, C. von Savigny, A. Rozanov, H. Bovensmann, J. P. Burrows, P. F. Bernath, C. D. Boone, L. Froidevaux, L. L. Gordley, M. G. Mlynczak, J. M. Russell III, L. W. Thomason, K. A. Walker, and J. M. Zawodny, Global and long-term comparison of SCIAMACHY limb ozone profiles with correlative satellite data (2002-2008), Atmos. Meas. Tech., 5, 771-788, doi:10.5194/amt-5-771-2012, 2012.
01/2012; -
Article: Sensitivity studies and first validation of stratospheric ozone profile retrievals from Odin/OSIRIS observations of limb-scattered solar radiation
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ABSTRACT: An error analysis and first validation results are presented for a method of retrieving stratospheric ozone density profiles from spectra of limb-scattered solar radiation, as measured with the OSIRIS instrument on the Odin satellite. The sensitivity study includes geophysical parameters such as ground albedo, stratospheric aerosols, cloud cover, and conditions in the background atmosphere, as well as instrumental parameters such as instrument noise, polarization sensitivity of the spectrograph, and levels of internal and external straylight. The dominating sources of error within the 1540 km altitude range are found to be stratospheric aerosols, ground albedo, and clouds, with each individual error being generally well below 5%. The total error in this altitude range is estimated to be on the order of 10% for an individual retrieved profile. A comparison of colocated measurements from OSIRIS and the POAM III occultation instrument during August of 2001 at northern-hemisphere mid-latitudes shows agreement to within about 5% between 15 and 35 km. The ozone densities from OSIRIS are found to be systematically lower than those from POAM III.PACS Nos.: 42.68.Ca, 82.33.TbCanadian Journal of Physics 02/2011; 83(9):957-972. · 0.86 Impact Factor -
Article: Chemical ozone loss in Arctic and Antarctic polar winter/spring season derived from SCIAMACHY limb measurements 2002–2009
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ABSTRACT: Stratospheric ozone profiles are retrieved for the period 2002–2009 from SCIAMACHY measurements of limb-scattered solar radiation in the Hartley and Chappuis absorption bands of ozone. This data set is used to determine the chemical ozone loss in both the Arctic and Antarctic polar vortices using the vortex average method. The chemical ozone loss at isentropic levels between 450 K and 600 K is derived from the difference between observed ozone abundances and the ozone modelled considering diabatic cooling, but no chemical ozone loss. The results show chemical ozone losses of up to 20–40% between the beginning of January and the end of March inside the Arctic polar vortex. Strong inter-annual variability of the Arctic ozone loss is observed, with the cold winters 2004/2005 and 2006/2007 showing the largest chemical ozone losses. The ozone mass loss inside the polar vortex is also estimated. In the coldest Arctic winter 2004/2005 the total ozone mass loss is about 30 million tons inside the polar vortex between the 450 K and 600 K isentropic levels from the beginning of January until the end of March. The Antarctic vortex averaged ozone loss as well as the size of the polar vortex do not vary much from year to year. At the 475 K isentropic level ozone losses of 70–80% between mid-August and mid-November are observed every year inside the vortex, also in the anomalous year 2002. The total ozone mass loss inside the Antarctic polar vortex between the 450 K and 600 K isentropic levels is about 55–75 million tons for the period between mid-August and mid-November. Comparisons of the vertical variation of ozone loss derived from SCIAMACHY observations with several independent techniques for the Arctic winter 2004/2005 show very good agreement.Atmospheric Chemistry and Physics Discussions. 01/2011; -
Article: SCIAMACHY stratospheric aerosol extinction profile retrieval
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ABSTRACT: The Ozone Mapper and Profiler Suite Limp Profiler (OMPS/LP) algorithm is used to retrieve ozone and aerosol profiles using a series of 120 SCIAMACHY limb measurements collocated with SAGE II solar occultation events. The primary goal of the study is to ascertain the capability of the OMPS/LP retrieval algorithm to accurately retrieve the vertical distribution of stratospheric aerosol extinction coefficient so as to better account for aerosol effects in the ozone profiling retrieval process. Using simulated radiances, we show that the aerosol extinction coefficient can be retrieved from limb scatter measurements within 5% and a standard deviation better than 15%, which is more than sufficient to improve the OMPS/LP ozone products to be used as Environmental Data Records. We also illustrate the ability of SCIAMACHY limb measurements to retrieve stratospheric aerosol profiles with accuracy comparable to other instruments. The retrieved aerosol profiles agree with collocated SAGE II measurements on average to within 25%, with a standard deviation of 35%.Atmospheric Measurement Techniques Discussions. 01/2010; -
Article: First evidence of a 27 day solar signature in noctilucent cloud occurrence frequency
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ABSTRACT: 1] This paper presents evidence of a connection between the 27 day modulation of the solar activity and noctilucent cloud (NLC) occurrence frequency as measured by the Scanning Imaging Absorption Spectrometer for Atmospheric Chartography (SCIAMACHY) and solar backscatter ultraviolet (SBUV) instruments. Observations show anticorrelations significant at the 90% confidence level between noctilucent cloud occurrence rate anomalies and Lyman-a irradiance variation during several seasons in both hemispheres. A superposed epoch analysis confirms these results and also reveals a clear recurrence pattern in noctilucent clouds occurrence anomalies with a $27 day period. The superposed epoch analysis also shows that the maximum NLC response in the Northern Hemisphere is clearly localized at 0 day phase lag, while in the Southern Hemisphere the maximum response is broader and occurs at 0 ± 2 day phase lag. Microwave Limb Sounder mesospheric products suggest that the more likely driver for the variation in NLC occurrence is temperature instead of water vapor, but the mechanisms responsible for the observed variations are not yet fully understood.J. Geophys. Res. 01/2010; 115:0-12. -
Article: Validation of ozone measurements from the Atmospheric Chemistry Experiment (ACE)
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ABSTRACT: This paper presents extensive {bias determination} analyses of ozone observations from the Atmospheric Chemistry Experiment (ACE) satellite instruments: the ACE Fourier Transform Spectrometer (ACE-FTS) and the Measurement of Aerosol Extinction in the Stratosphere and Troposphere Retrieved by Occultation (ACE-MAESTRO) instrument. Here we compare the latest ozone data products from ACE-FTS and ACE-MAESTRO with coincident observations from nearly 20 satellite-borne, airborne, balloon-borne and ground-based instruments, by analysing volume mixing ratio profiles and partial column densities. The ACE-FTS version 2.2 Ozone Update product reports more ozone than most correlative measurements from the upper troposphere to the lower mesosphere. At altitude levels from 16 to 44 km, the average values of the mean relative differences are nearly all within +1 to +8%. At higher altitudes (45–60 km), the ACE-FTS ozone amounts are significantly larger than those of the comparison instruments, with mean relative differences of up to +40% (about +20% on average). For the ACE-MAESTRO version 1.2 ozone data product, mean relative differences are within ±10% (average values within ±6%) between 18 and 40 km for both the sunrise and sunset measurements. At higher altitudes (~35–55 km), systematic biases of opposite sign are found between the ACE-MAESTRO sunrise and sunset observations. While ozone amounts derived from the ACE-MAESTRO sunrise occultation data are often smaller than the coincident observations (with mean relative differences down to −10%), the sunset occultation profiles for ACE-MAESTRO show results that are qualitatively similar to ACE-FTS, indicating a large positive bias (mean relative differences within +10 to +30%) in the 45–55 km altitude range. In contrast, there is no significant systematic difference in bias found for the ACE-FTS sunrise and sunset measurements.Atmospheric Chemistry and Physics 01/2009; · 4.88 Impact Factor -
Article: Evolution of stratospheric ozone and water vapour time series studied with satellite measurements
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ABSTRACT: The long term evolution of stratospheric ozone and water vapour has been investigated by extending satellite time series to April 2008. For ozone, we examine monthly average ozone values from various satellite data sets for nine latitude and altitude bins covering 60° S to 60° N and 20–45 km and covering the time period of 1979–2008. Data are from the Stratospheric Aerosol and Gas Experiment (SAGE I+II), the HALogen Occultation Experiment (HALOE), the Solar BackscatterUltraViolet-2 (SBUV/2) instrument, the Sub-Millimetre Radiometer (SMR), the Optical Spectrograph InfraRed Imager System (OSIRIS), and the SCanning Imaging Absorption spectroMeter for Atmospheric CHartograpY (SCIAMACHY). Monthly ozone anomalies are calculated by utilising a linear regression model, which also models the solar, quasi-biennial oscillation (QBO), and seasonal cycle contributions. Individual instrument ozone anomalies are combined producing an all instrument average. Assuming a turning point of 1997 and that the all instrument average is represented by good instrumental long term stability, the largest statistically significant ozone declines (at two sigma) from 1979–1997 are seen at the mid-latitudes between 35 and 45 km, namely −7.2%±0.9%/decade in the Northern Hemisphere and −7.1%±0.9%/in the Southern Hemisphere. Furthermore, for the period 1997 to 2008 we find that the same locations show the largest ozone recovery (+1.4% and +0.8%/decade respectively) compared to other global regions, although the estimated trend model errors indicate that the trend estimates are not significantly different from a zero trend at the 2 sigma level. An all instrument average is also constructed from water vapour anomalies during 1991–2008, using the SAGE II, HALOE, SMR, and the Microwave Limb Sounder (Aura/MLS) measurements. We report that the decrease in water vapour values after 2001 slows down around 2004–2005 in the lower tropical stratosphere (20–25 km) and has even shown signs of increasing until present. We show that a similar correlation is also seen with the temperature measured at 100 hPa during this same period.Atmospheric Chemistry and Physics. 01/2009; -
Article: Ozone and temperature trends in the upper stratosphere at five stations of the Network for the Detection of Atmospheric Composition Change
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ABSTRACT: Upper stratospheric ozone anomalies from the satellite-borne Solar Backscatter Ultra-Violet (SBUV), Stratospheric Aerosol and Gas Experiment II (SAGE II), Halogen Occultation Experiment (HALOE), Global Ozone Monitoring by Occultation of Stars (GOMOS), and Scanning Imaging Absorption Spectrometer for Atmospheric Chartography (SCIAMACHY) instruments agree within 5% or better with ground-based data from lidars and microwave radiometers at five stations of the Network for the Detection of Atmospheric Composition Change (NDACC), from 45 degrees S to 48 degrees N. From 1979 until the late 1990s, all available data show a clear decline of ozone near 40 km, by 10%-15%. This decline has not continued in the last 10 years. At some sites, ozone at 40 km appears to have increased since 2000, consistent with the beginning decline of stratospheric chlorine. The phaseout of chlorofluorocarbons after the International Montreal Protocol in 1987 has been successful, and is now showing positive effects on ozone in the upper stratosphere. Temperature anomalies near 40 km altitude from European Centre for Medium Range Weather Forecast reanalyses (ERA-40), from National Centers for Environmental Prediction (NCEP) operational analyses, and from HALOE and lidar measurements show good consistency at the five stations, within about 3 K. Since about 1985, upper stratospheric temperatures have been fluctuating around a constant level at all five NDACC stations. This non-decline of upper stratospheric temperatures is a significant change from the more or less linear cooling of the upper stratosphere up until the mid-1990s, reported in previous trend assessments. It is also at odds with the almost linear 1 K per decade cooling simulated over the entire 1979-2010 period by chemistry-climate models (CCMs). The same CCM simulations, however, track the historical ozone anomalies quite well, including the change of ozone tendency in the late 1990s.International Journal of Remote Sensing 01/2009; 30(15-16):3875-3886. · 1.12 Impact Factor -
Article: Cloud sensitivity studies for stratospheric and lower mesospheric ozone profile retrievals from measurements of limb-scattered solar radiation
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ABSTRACT: Clouds in the atmosphere play an important role in reflection, absorption and transmission of solar radiation and thus affect trace gas retrievals. The main goal of this paper is to examine the sensitivity of stratospheric and lower mesospheric ozone retrievals from limb-scattered radiance measurements to clouds using the SCIATRAN radiative transfer model and retrieval package. The retrieval approach employed is optimal estimation, and the considered clouds are vertically and horizontally homogeneous. Assuming an aerosol-free atmosphere and Mie phase functions for cloud particles, we compute the relative error of ozone profile retrievals in a cloudy atmosphere if clouds are neglected in the retrieval. To access altitudes from the lower stratosphere up to the lower mesosphere, we combine the retrievals in the Chappuis and Hartley ozone absorption bands. We find significant cloud sensitivity of the limb ozone retrievals in the Chappuis bands at lower stratospheric altitudes. The relative error in the retrieved ozone concentrations gradually decreases with increasing altitude and becomes negligible above approximately 40 km. The parameters with the largest impact on the ozone retrievals are cloud optical thickness, ground albedo and solar zenith angle. Clouds with different geometrical thicknesses or different cloud altitudes have a similar impact on the ozone retrievals for a given cloud optical thickness value, if the clouds are outside the field of view of the instrument. The effective radius of water droplets has a small influence on the error, i.e., less than 0.5% at altitudes above the cloud top height. Furthermore, the impact of clouds on the ozone profile retrievals was found to have a rather small dependence on the solar azimuth angle (less than 1% for all possible azimuth angles). For the most frequent cloud types, the total error is below 6% above 15 km altitude, if clouds are completely neglected in the retrieval. Neglecting clouds in the ozone profile retrievals generally leads to a low bias for a low ground albedo and to a high bias for a high ground albedo, assuming that the ground albedo is well known.Atmospheric Measurement Techniques. 01/2009; -
Article: Comparison of NLC particle sizes derived from SCIAMACHY/Envisat observations with ground-based LIDAR measurements at ALOMAR (69° N)
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ABSTRACT: SCIAMACHY, the Scanning Imaging Absorption spectroMeter for Atmospheric CHartographY provides measurements of limb-scattered solar radiation in the 220 nm to 2380 nm wavelength range since summer 2002. Measurements in the UV spectral range are well suited for the retrieval of particle sizes of noctilucent clouds (NLCs) and have been used to compile the largest existing satellite data base of NLC particle sizes. This paper presents a comparison of SCIAMACHY NLC size retrievals with the extensive NLC particle size data set based on ground-based LIDAR measurements at the Arctic LIDAR Observatory for Middle Atmosphere Research (ALOMAR, 69° N, 16° E) for the Northern Hemisphere NLC seasons 2003 to 2007. Most of the presented SCIAMACHY NLC particle size retrievals are based on cylindrical particles and a Gaussian particle size distribution with a fixed width. If the differences in spatial as well as vertical resolution between SCIAMACHY and the ALOMAR LIDAR are taken into account, very good agreement is found. The mean particle size derived from SCIAMACHY limb observations for the ALOMAR overpasses in 2003 to 2007 is 56.2 nm with a standard deviation of 12.5 nm, and the LIDAR observations yield a value of 54.2 nm with a standard deviation of 17.4 nm.Atmospheric Measurement Techniques Discussions. 01/2009; -
Article: The noctilucent cloud (NLC) display during the ECOMA/MASS sounding rocket flights on 3 August 2007: morphology on global to local scales
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ABSTRACT: During the ECOMA/MASS rocket campaign large scale NLC/PMC was observed by satellite, lidar and camera from polar to mid latitudes. We examine the observations from different instruments to investigate the morphology of the cloud. Satellite observations show a planetary wave 2 structure. Lidar observations from Kühlungsborn (54° N), Esrange (68° N) and ALOMAR (69° N) show a highly dynamic NLC layer. Under favorable solar illumination the cloud is also observable by ground-based cameras. The cloud was detected by cameras from Trondheim (63° N), Juliusruh (55° N) and Kühlungsborn. We investigate planetary scale morphology and local scale gravity wave structures, important for the interpretation of the small scale rocket soundings. We compare in detail the lidar observations with the NLC structure observed by the camera in Trondheim. The ALOMAR RMR-lidar observed only a faint NLC during the ECOMA launch window, while the camera in Trondheim showed a strong NLC display in the direction of ALOMAR. Using the high resolution camera observations (t~30 s, Δx<5 km) and the wind information from the meteor radar at ALOMAR we investigate the formation and destruction of NLC structures. We observe that the NLC brightness is reduced by a factor of 20–40 within 100 s which can be caused by a temperature about 15 K above the frostpoint temperature. A horizontal temperature gradient of more than 3 K/km is estimated.Annales Geophysicae. 01/2009; -
Article: Validation of ozone measurements from the Atmospheric Chemistry Experiment (ACE)
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ABSTRACT: This paper presents extensive validation analyses of ozone observations from the Atmospheric Chemistry Experiment (ACE) satellite instruments: the ACE Fourier Transform Spectrometer (ACE-FTS) and the Measurement of Aerosol Extinction in the Stratosphere and Troposphere Retrieved by Occultation (ACE-MAESTRO) instrument. The ACE satellite instruments operate in the mid-infrared and ultraviolet-visible-near-infrared spectral regions using the solar occultation technique. In order to continue the long-standing record of solar occultation measurements from space, a detailed quality assessment is required to evaluate the ACE data and validate their use for scientific purposes. Here we compare the latest ozone data products from ACE-FTS and ACE-MAESTRO with coincident observations from satellite-borne, airborne, balloon-borne and ground-based instruments, by analysing volume mixing ratio profiles and partial column densities. The ACE-FTS version 2.2 Ozone Update product reports more ozone than most correlative measurements from the upper troposphere to the lower mesosphere. At altitude levels from 16 to 44 km, the mean differences range generally between 0 and +10% with a slight but systematic positive bias (typically +5%). At higher altitudes (45–60 km), the ACE-FTS ozone amounts are significantly larger than those of the comparison instruments by up to ~40% (typically +20%). For the ACE-MAESTRO version 1.2 ozone data product, agreement within ±10% (generally better than ±5%) is found between 18 and 40 km for the sunrise and sunset measurements. At higher altitudes (45–55 km), systematic biases of opposite sign are found between the ACE-MAESTRO sunrise and sunset observations. While ozone amounts derived from the ACE-MAESTRO sunrise occultation data are often smaller than the coincident observations (by as much as −10%), the sunset occultation profiles for ACE-MAESTRO show results that are qualitatively similar to ACE-FTS and indicate a large positive bias (+10 to +30%) in this altitude range. In contrast, there is no significant difference in bias found for the ACE-FTS sunrise and sunset measurements. These systematic effects in the ozone profiles retrieved from the measurements of ACE-FTS and ACE-MAESTRO are being investigated. This work shows that the ACE instruments provide reliable, high quality measurements from the tropopause to the upper stratosphere and can be used with confidence in this vertical domain.Atmospheric Chemistry and Physics Discussions. 01/2008; -
Article: Comparison of the inversion algorithms applied to the ozone vertical profile retrieval from SCIAMACHY limb measurements
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ABSTRACT: This paper is devoted to an intercomparison of ozone vertical profiles retrieved from the measurements of scattered solar radiation performed by the SCIAMACHY instrument in the limb viewing geometry. Three different inversion algorithms including the prototype of the operational Level 1 to 2 processor to be operated by the European Space Agency are considered. The intercomparison was performed for 5 selected orbits of SCIAMACHY showing a good overall agreement of the results in the middle stratosphere, whereas considerable discrepancies were identified in the lower stratosphere and upper troposphere altitude region. Additionally, comparisons with ground-based lidar measurements are shown for selected profiles demonstrating an overall correctness of the retrievals.Atmospheric Chemistry and Physics Discussions. 01/2007; -
Article: Inter-comparison of stratospheric O3 and NO2 abundances retrieved from balloon borne direct sun observations and Envisat/SCIAMACHY limb measurements
Atmospheric Chemistry and Physics 12/2006; 6:1293-1314. · 4.88 Impact Factor -
Article: Inter-comparison of stratospheric O<sub>3</sub> and NO<sub>2</sub> abundances retrieved from balloon borne direct sun observations and Envisat/SCIAMACHY limb measurements
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ABSTRACT: Stratospheric O<sub>3</sub> and NO<sub>2</sub> abundances measured by different remote sensing instruments are inter-compared: (1) Line-of-sight absorptions and vertical profiles inferred from solar spectra in the ultra-violet (UV), visible and infrared (IR) wavelength ranges measured by the LPMA/DOAS (Limb Profile Monitor of the Atmosphere/Differential Optical Absorption Spectroscopy) balloon payload during balloon ascent/descent and solar occultation are examined with respect to internal consistency. (2) The balloon borne stratospheric profiles of O<sub>3</sub> and NO<sub>2</sub> are compared to collocated space-borne skylight limb observations of the Envisat/SCIAMACHY satellite instrument. The trace gas profiles are retrieved from SCIAMACHY spectra using different algorithms developed at the Universities of Bremen and Heidelberg and at the Harvard-Smithsonian Center for Astrophysics. A comparison scheme is used that accounts for the spatial and temporal mismatch as well as differing photochemical conditions between the balloon and satellite borne measurements. It is found that the balloon borne measurements internally agree to within ±10% and ±20% for O<sub>3</sub> and NO<sub>2</sub>, respectively, whereas the agreement with the satellite is ±20% for both gases in the 20 km to 30 km altitude range and in general worse below 20 km.01/2006; -
Article: Geophysical validation of SCIAMACHY Limb Ozone Profiles
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ABSTRACT: We discuss the quality of the two available SCIAMACHY limb ozone profile products. They were retrieved with the University of Bremen IFE's algorithm version 1.61 (hereafter IFE), and the official ESA offline algorithm (hereafter OL) versions 2.4 and 2.5. The ozone profiles were compared to a suite of correlative measurements from ground-based lidar and microwave, sondes, SAGE II and SAGE III (Stratospheric Aerosol and Gas Experiment). To correct for the expected Envisat pointing errors, which have not been corrected implicitly in either of the algorithms, we applied a constant altitude shift of -1.5 km to the SCIAMACHY ozone profiles. The IFE ozone profile data between 16 and 40 km are biased low by 3-6%. The average difference profiles have a typical standard deviation of 10% between 20 and 35 km. We show that more than 20% of the SCIAMACHY official ESA offline (OL) ozone profiles version 2.4 and 2.5 have unrealistic ozone values, most of these are north of 15° S. The remaining OL profiles compare well to correlative instruments above 24 km. Between 20 and 24 km, they underestimate ozone by 15±5%.Atmospheric Chemistry and Physics. 01/2006; -
Article: Latitudinal and vertical distribution of bromine monoxide in the lower stratosphere from Scanning Imaging Absorption Spectrometer for Atmospheric Chartography limb scattering measurements
Journal of Geophysical Research 01/2006; 111(D14301). · 3.02 Impact Factor
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Institutions
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2004–2006
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Universität Bremen
- Institut für Umweltphysik (IUP)
Bremen, Bremen, Germany
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