Natural radioactivity and radon exhalation rate in Brazilian igneous rocks

Departamento de Petrologia e Metalogenia, Instituto de Geociências e Ciências Exatas, Universidade Estadual Paulista, Av. 24-A No. 1515, Rio Claro, São Paulo, Brazil.
Applied radiation and isotopes: including data, instrumentation and methods for use in agriculture, industry and medicine (Impact Factor: 1.23). 03/2011; 69(7):1094-9. DOI: 10.1016/j.apradiso.2011.03.004
Source: PubMed


This paper reports the natural radioactivity of Brazilian igneous rocks that are used as dimension stones, following the trend of other studies on the evaluation of the risks to the human health caused by the rocks radioactivity as a consequence of their use as cover indoors. Gamma-ray spectrometry has been utilized to determine the (40)K, (226)Ra and (232)Th activity concentrations in 14 rock types collected at different quarries. The following activity concentration range was found: 12.18-251.90 Bq/kg for (226)Ra, 9.55-347.47 Bq/kg for (232)Th and 407.5-1615.0 Bq/kg for (40)K. Such data were used to estimate Ra(eq), H(ex) and I(γ), which were compared with the threshold limit values recommended in literature. They have been exceeded for Ra(eq) and H(ex) in five samples, where the highest indices corresponded to a rock that suffered a process of ductile-brittle deformation that caused it a microbrecciated shape. The exhalation rate of Rn and daughters has also been determined in slabs consisting of rock pieces ~10 cm-long, 5 cm-wide and 3 cm-thick. It ranged from 0.24 to 3.93 Bq/m(2)/h and exhibited significant correlation with eU (=(226)Ra), as expected. The results indicated that most of the studied rocks did not present risk to human health and may be used indoors, even with low ventilation. On the other hand, igneous rocks that yielded indices above the threshold limit values recommended in literature may be used outdoors without any restriction or indoors with ample ventilation.

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    • "The new types of building materials are brought from various places around the world, and some may be extracted from areas with high background radiation . The contribution of building materials to indoor radon has been investigated in some previous studies in different regions [5] [6] [7]. "
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    ABSTRACT: Radon levels and radioactivity were measured in 50 shops and storage areas for building materials in Sudan. Charcoal canister and gamma spectrometry systems were used to measure radon in 55 types of natural material, and concentrations of 71-292 Bq/m3 (mean, 154 ± 38 Bq/m3) were found. The concentration of radium (226Ra) ranged from 2.8 to 182.5 Bq/kg, of thorium (232Th) from 1.2 to 302 Bq/kg and of potassium (40K) from 82.3 to 1413.3 Bq/kg. Porcelain, ceramic and marble showed high values, while gravel types had low radioactivity. Radium in building materials was well correlated with radon (r2 = 0.77). The average annual dose of workers at these sites due to inhalation of radon was estimated to be 2.8 mSv. The activity index of building materials ranged between 0.33 and 1.97 (mean, 0.77).
    10/2014; 8(4):394-400. DOI:10.1016/j.jtusci.2014.06.004
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    • "and they are widely used in recent publications for presenting the radioactive hazard of building materials (e.g. Al-Sulaiti et al., 2011; Damla et al., 2011; Moura et al., 2011). "
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    Journal of Environmental Radioactivity 12/2012; 118C:64-74. DOI:10.1016/j.jenvrad.2012.11.008 · 2.48 Impact Factor
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    ABSTRACT: Most destructive earthquakes nucleate at between 5–7 km and about 35–40 km depth. Before earthquakes, rocks are subjected to increasing stress. Not every stress increase leads to rupture. To understand pre-earthquake phenomena we note that igneous and high-grade metamorphic rocks contain defects which, upon stressing, release defect electrons in the oxygen anion sublattice, known as positive holes. These charge carriers are highly mobile, able to flow out of stressed rocks into surrounding unstressed rocks. They form electric currents, which emit electromagnetic radiation, sometimes in pulses, sometimes sustained. The arrival of positive holes at the ground-air interface can lead to air ionization, often exclusively positive. Ionized air rising upward can lead to cloud condensation. The upward flow of positive ions can lead to instabilities in the mesosphere, to mesospheric lightning, to changes in the Total Electron Content (TEC) at the lower edge of the ionosphere, and electric field turbulences. Advances in deciphering the earthquake process can only be achieved in a broadly multidisciplinary spirit.
    Acta Geophysica 08/2013; 61(4). DOI:10.2478/s11600-013-0130-4 · 1.07 Impact Factor
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