Tracing troposphere-to-stratosphere transport above a mid-latitude deep convective system

ATMOSPHERIC CHEMISTRY AND PHYSICS (Impact Factor: 5.3). 05/2004; 4(3). DOI: 10.5194/acp-4-741-2004
Source: DOAJ

ABSTRACT Within the project SPURT (trace gas measurements in the tropopause region) a variety of trace gases have been measured in situ in order to investigate the role of dynamical and chemical processes in the extra-tropical tropopause region. In this paper we report on a flight on 10 November 2001 leading from Hohn, Germany (52ºN) to Faro, Portugal (37ºN) through a strongly developed deep stratospheric intrusion. This streamer was associated with a large convective system over the western Mediterranean with potentially significant troposphere-to-stratosphere transport. Along major parts of the flight we measured unexpectedly high NOy mixing ratios. Also H2O mixing ratios were significantly higher than stratospheric background levels confirming the extraordinary chemical signature of the probed air masses in the interior of the streamer. Backward trajectories encompassing the streamer enable to analyze the origin and physical characteristics of the air masses and to trace troposphere-to-stratosphere transport. Near the western flank of the intrusion features caused by long range transport, such as tropospheric filaments characterized by sudden drops in the O3 and NOy mixing ratios and enhanced CO and H2O can be reconstructed in great detail using the reverse domain filling technique. These filaments indicate a high potential for subsequent mixing with the stratospheric air. At the south-western edge of the streamer a strong gradient in the NOy and the O3 mixing ratios coincides very well with a sharp gradient in potential vorticity in the ECMWF fields. In contrast, in the interior of the streamer the observed highly elevated NOy and H2O mixing ratios up to a potential temperature level of 365 K and potential vorticity values of maximum 10 PVU cannot be explained in terms of resolved troposphere-to-stratosphere transport along the backward trajectories. Also mesoscale simulations with a High Resolution Model reveal no direct evidence for convective H2O injection up to this level. Elevated H2O mixing ratios in the ECMWF and HRM model are seen only up to about tropopause height at 340 hPa and 270hPa, respectively, well below flight altitude of about 200 hPa. However, forward tracing of the convective influence as identified by satellite brightness temperature measurements and counts of lightning strokes shows that during this part of the flight the aircraft was closely following the border of an air mass which was heavily impacted by convective activity over Spain and Algeria. This is evidence that deep convection at mid-latitudes may have a large impact on the tracer distribution of the lowermost stratosphere reaching well above the thunderstorms anvils as claimed by recent studies using cloud-resolving models.

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Available from: M. I. Hegglin, Aug 28, 2015
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    • "The authors use aircraft data and infrared satellite brightness temperature to associate the observed variability with coincident convection. [6] A considerable amount of attention has been given to the occurrence of convection that overshoots the lapse-rate tropopause [e.g., Poulida et al., 1996; Fischer et al., 2003; Wang, 2003; Hegglin et al., 2004; Ray et al., 2004; Setvák et al., 2008; Bedka et al., 2009; Pan and Munchak, 2011]. Although the chemical impacts of overshooting convection and convective injection into stratospheric intrusions may be comparable (both mix tropospheric boundary layer and stratospheric air), they occur under significantly different dynamical conditions. "
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    Journal of Geophysical Research Atmospheres 12/2011; 116:0198-. DOI:10.1029/2011JD016724 · 3.44 Impact Factor
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    • "Many publications have examined the stratosphere‐ troposphere exchange and the resulting ozone flux, in terms of its magnitude, seasonality and geographic pattern [e.g., Gettelman et al., 1997; Roelofs and Lelieveld, 1997; Olsen et al., 2004; Hsu et al., 2005]. Others have examined the meteorological processes that drive STE, such as, tropopause folds near jet streams [Sprenger et al., 2003, Figure 3b], wave breaking [Scott et al., 2001], cutoff lows [Ebel et al., 1991], mid‐latitude deep convection [Poulida et al., 1996; Fischer et al., 2003; Gray, 2003; Hegglin et al., 2004]. [13] The link between deep convection and the STE O 3 flux has only been found for extreme events on a case‐study basis. "
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    • "The advantage of such a coordinate system in representing trace gas distributions in the LMS is that a substantial amount of scatter in the observations can be removed (e.g. Hoor et al., 2004; Hegglin et al., 2004). This is due to the fact that the ϕ e − θ-coordinate system accounts for adiabatic air parcel displacements, e.g. the influence of transient (and largely reversible) north-south excursions of air parcels associated with dynamical features like Rossby waves, which significantly contribute to the variability in geographical space. "
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