A unified analysis of ultrafast vibrational and orientational dynamics of HOD in D2O
ABSTRACT Vibrational echo peak shift and polarization-selective pump-probe measurements with broadband 45 femtosecond infrared pulses
have been used to study the OH stretching Vibration of HOD in D2O. A unified analysis of all experiments allows a characterization of the ensemble-averaged vibrational dephasing, lifetime,
and orientational dynamics.