Effect of Electron-Phonon Interaction Range for a Half-Filled Band in One Dimension
ABSTRACT We demonstrate that fermion-boson models with nonlocal interactions can be
simulated at finite band filling with the continuous-time quantum Monte Carlo
method. We apply this method to explore the influence of the electron-phonon
interaction range for a half-filled band in one dimension, covering the full
range from the Holstein to the Fr\"ohlich regime. The phase diagram contains
metallic, Peierls, and phase-separated regions, which we characterize in terms
of static and dynamical correlation functions. In particular, our results
reveal a suppression of $2k_F$ charge correlations with increasing interaction
range, allowing for a power-law decay comparable to the pairing correlations.
- SourceAvailable from: Masaki Tezuka[Show abstract] [Hide abstract]
ABSTRACT: Employing the recently developed self-consistent variational basis generation scheme, we have investigated the bipolaron-bipolaron interaction within the purview of Holstein-Hubbard and the Froehlich-Hubbard model on a discrete one-dimensional lattice. The density-matrix renormalization group (DMRG) method has also been used for the Holstein-Hubbard model. We have shown that there exists no bipolaron-bipolaron attraction in the Holstein-Hubbard model. In contrast, we have obtained clear-cut bipolaron-bipolaron attraction in the Froehlich-Hubbard model. Composite bipolarons are formed above a critical electron-phonon coupling strength, which can survive the finite Hubbard U effect. We have constructed the phase diagram of Froehlich-Hubbard polarons and bipolarons, and discussed the phase separation in terms of the formation of composite bipolarons.Physical Review B 01/2014; 89:035146. · 3.66 Impact Factor
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ABSTRACT: We determine the phase diagram of a polaron model with mixed breathing-mode and Su-Schrieffer-Heeger couplings and show that it has two sharp transitions, in contrast to pure models which exhibit one (for Su-Schrieffer-Heeger coupling) or no (for breathing-mode coupling) transition. We then show that ultracold molecules trapped in optical lattices can be used as a quantum simulator to study precisely this mixed Hamiltonian, and that the relative contributions of the two couplings can be tuned with external electric fields. The parameters of current experiments place them in the region where one of the transitions occurs. We also propose a scheme to measure the polaron dispersion using stimulated Raman spectroscopy.Physical Review Letters 05/2013; 110(22):223002. · 7.73 Impact Factor
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ABSTRACT: We analyze the dynamical response of a ultracold binary gas mixture in presence of strong boson-fermion couplings. Mapping the problem onto that of the optical response of a metal/semiconductor electronic degrees of freedom to electromagnetic perturbation we calculate the corresponding dynamic linear response susceptibility in the non-perturbative regimes of strong boson-fermion coupling using diagrammatic resummation technique as well as quantum Monte Carlo simulations. We evaluate the Bragg spectral function as well as the optical conductivity and find a pseudogap, which forms in certain parameter regimes.Physica B Condensed Matter 12/2014; 454:224-234. · 1.28 Impact Factor
Effect of Electron-Phonon Interaction Range for a Half-Filled Band in One Dimension
Martin Hohenadler,1Fakher F. Assaad,1and Holger Fehske2
1Institut f¨ ur Theoretische Physik und Astrophysik, Universit¨ at W¨ urzburg, 97074 W¨ urzburg, Germany
2Institut f¨ ur Physik, Ernst-Moritz-Arndt-Universit¨ at Greifswald, 17487 Greifswald, Germany
(Dated: September 19, 2012)
We demonstrate that fermion-boson models with nonlocal interactions can be simulated at finite
band filling with the continuous-time quantum Monte Carlo method. We apply this method to
explore the influence of the electron-phonon interaction range for a half-filled band in one dimension,
covering the full range from the Holstein to the Fr¨ ohlich regime.
metallic, Peierls, and phase-separated regions. Nonlocal interactions suppress the Peierls instability,
and thereby lead to almost degenerate power-law exponents for charge and pairing correlations.
The phase diagram contains
PACS numbers: 71.10.Hf, 71.10.Pm, 71.30.+h, 71.45.Lr
Introduction.—Electron-phonon interaction has an es-
sential influence on the properties of many materials .
It plays a key role for pairing and superconductivity, mass
renormalization, and charge ordering phenomena. Tak-
ing into account quantum lattice fluctuations leads to a
complex, many-body problem. Consequently, theoreti-
cal studies usually rely on simplified microscopic models.
A frequently invoked approximation, in particular for nu-
merical studies, is to consider a completely local electron-
phonon coupling as in Holstein’s molecular-crystal model
. However, nonlocal interactions are expected to play
an important role in materials with incomplete screen-
ing such as quasi-one-dimensional (quasi-1D) organics
. Long-range interactions, as described by the Fr¨ ohlich
model , have been investigated in the context of high-
temperature superconducting cuprates [5–9], and were
found to support light polarons and bipolarons [10–12].
Exact numerical methods have played an important
role for the understanding of coupled electron-phonon
systems. Whereas efficient algorithms exist for Holstein-
type models at arbitrary band filling [13–18], extended
interactions could so far be addressed only in the empty-
band limit, see, for example, [10, 19–22], and  for a re-
view. Consequently, key phenomena such as the Peierls
instability  were out of reach. The latter occurs in
quasi-1D systems with commensurate fillings, for exam-
ple in TTF-TCNQ , and drives a transition to a
Peierls insulator with charge-density-wave order. For the
Holstein model, it is known that quantum lattice fluc-
tuations can destroy the charge order , leading to
a metal-insulator quantum phase transition at a finite
value of the electron-phonon coupling strength.
Unbiased investigations of the effect of nonlocal inter-
actions at finite band-filling represent a long-standing,
open problem. In this Letter, we use the continuous-
time quantum Monte Carlo (CTQMC) method  to
study a model that interpolates between and includes
the paradigmatic Holstein and Fr¨ ohlich limits.
Model.—We consider a HamiltonianˆH = ˆH0+ˆH1,
iσcjσ+ H.c.) describes 1D
fermions with nearest-neighbor hopping t, and
The first term describes lattice fluctuations in the har-
monic approximation, with the phonon frequency ω0and
the stiffness constant K = ω2
resents the electron-phonon interaction, in the form of a
nonlocal density-displacement coupling, with the density
operator ˆ ni =
elements are chosen as [9, 10, 27]
f(r)ˆQi+r(ˆ ni− 1). (1)
0M. The second term rep-
σˆ niσ and ˆ niσ = c†
iσciσ. The matrix
(r2+ 1)3/2e−r/ξ,0 ≤ r < L/2,(2)
where the lattice constant a = 1. For ξ → ∞, this cou-
pling represents a lattice version of the Fr¨ ohlich interac-
tion . More generally,ˆH1 may be viewed as an ex-
tended Holstein interaction with screening length ξ; the
original Holstein model  is recovered in the limit ξ → 0.
For ω0→ ∞, the model maps onto an attractive, general-
ized Hubbard model. Our method can be applied to any
coupling which preserves translational invariance. The
restriction of r is due to periodic boundary conditions.
Method.—For electron-phonon problems ,
starting point is the partition function at inverse tem-
perature β = 1/kBT,
where ψ,ψ are Grassmann fields, and q denotes phonon
coordinates. The phonons can be integrated out exactly
, leading to a purely fermionic action with a nonlocal
(in space and time) interaction
[ni(τ) − 1]Dτ,τ?
i,j[nj(τ?) − 1]. (4)
The phonon propagator takes the form Dτ,τ?
j)D(τ − τ?) with F(i − j) =?
= F(i −
rf(r + i − j)f(r) and
arXiv:1205.0612v2 [cond-mat.str-el] 18 Sep 2012
the Holstein propagator D(τ − τ?).
range in space (time) is determined by ξ (ω0).
CTQMC method used here is based on an exact expan-
sion around γ = 0 . A hybridization expansion algo-
rithm for electron-phonon impurity problems also exists
. Monte Carlo updates consist of adding or removing
single vertices, and flipping auxiliary Ising spins [18, 26].
The numerical effort scales with the cube of the aver-
age expansion order. Because of the underlying weak-
coupling expansion, the CTQMC method is particularly
efficient for problems with small expansion orders, such
as the Peierls transition in the adiabatic regime ω0/t ? 1
. Importantly, the method enables us to study the
many-electron problem . We have verified that it re-
produces exact results in the Holstein limit ξ → 0, and
in the anti-adiabatic limit ω0→ ∞ where the model (1)
maps onto an extended attractive Hubbard model.
Results.—We choose a phonon frequency ω0/t = 0.5.
In this regime, representative of many materials, neither
static nor instantaneous approximations are valid, and
numerical simulations are essential. The dimensionless
ratio λ = ?p/2t, where ?pis the polaron binding energy
in the atomic limit (t = 0)  and 2t is half of the free
bandwidth, allows us to compare different ξ at the same
effective coupling strength. We use t as the energy unit,
and set ? = M = 1. All results are for a half-filled band.
The phase diagram as a function of ξ and λ, obtained
from CTQMC simulations with up to L = 42 sites, is
shown in Fig. 1. Because the Holstein model is recov-
ered for ξ = 0, its previously studied metallic and Peierls
insulating phases [15, 32, 33] smoothly extend to ξ > 0.
However, we observe a significant ξ-dependence for small
ξ, and saturation for larger values. Additionally, for suf-
ficiently large ξ and λ, we find a region of phase sep-
aration or charge segregation. The metallic phase and
the metal-insulator transition extend all the way to the
Fr¨ ohlich limit ξ = ∞ [λPI
the range of λ shown in Fig. 1, phase separation is absent
for ξ ≤ 2, and becomes more favorable with increasing ξ.
The different phases can be characterized by the den-
sity correlator Sρ(r) = ?(ˆ nr−1)(ˆ n0−1)? and the density
structure factor Sρ(q). In the metallic phase [Fig. 2(a)],
Sρ(r) shows a power-law decay of 2kFcorrelations (with
exponent Kρ) as expected from bosonization, and is lin-
ear for q → 0. Together with exponentially suppressed
spin correlations (not shown), these findings are consis-
tent with a bipolaronic Luther-Emery phase [34, 35].
The Peierls state exhibits quasi-long-range 2kFdensity
correlations [Fig. 2(a)], corresponding to charge-density-
wave order at T = 0 with two electrons of opposite spin
forming bipolarons on every other site. The phase bound-
ary for the Peierls transition can be determined from the
staggered charge susceptibility 
c = 0.48(2)]; see also Fig. 3. For
dτ?ˆ ni(τ)ˆ nj(0)?.(5)
action range ξ and electron-phonon coupling strength λ. The
regions correspond to a metal, a Peierls insulator, and phase
separation. The metallic and Peierls phases (and presumably
also phase separation) extend to the Fr¨ ohlich limit ξ = ∞.
Lines are guides to the eye. Here ω0/t = 0.5.
(Color online) Phase diagram as a function of inter-
For fixed β/L, χρ(π)/L is universal at the critical point,
and the crossing of curves for different L gives λPI
example, we have λPI
= 0.33(1) for ξ = 2 in Fig. 2(c).
As for the Holstein model [32, 36], the Peierls transition
is expected to be of the Kosterlitz-Thouless type also for
ξ > 0. Extended interactions (ξ > 0) promote metallic
behavior by dissociating the onsite bipolarons predomi-
nant in the Holstein regime, and we see a Peierls insulator
to metal transition as a function of ξ [Fig. 2(a)]. By the
same mechanism, the critical coupling for the transition
to the Peierls insulator, λPI
c, increases with increasing ξ,
see Fig. 1. The onset of charge order is also reflected in
the divergent q = 2kFpeak in Sρ(q), see Fig. 2(b).
Phase separation as a result of the phonon-induced at-
traction manifests itself as a peak at small q in Sρ(q),
as shown in Fig. 2(b). In the phase-separated region of
Fig. 1, the quantity πSρ(q1)/q1(with q1= 2π/L)—whose
thermodynamic limit is related to Kρ in a Luttinger
liquid—diverges with system size. In the Peierls phase
Kρ= 0, as verified on very large systems . Formally,
Kρ= ∞, reflecting phase separation, implies a divergent
compressibility . The divergence of πSρ(q1)/q1in the
phase-separated region is shown for ξ = 6 in Fig. 2(d),
and we deduce a critical value of λPS
are two possible scenarios for the transition from the
Peierls to the phase separated region. A continuous tran-
sition would imply a melting of the charge-ordered Peierls
state before the formation of multipolaron droplets, al-
lowing for an intervening (narrow) metallic region with
finite Kρ. Alternatively, the insulator-insulator transi-
tion could be of first order. Evidence for the latter pos-
sibility comes from the occurrence of metastable config-
urations and hysteresis at low temperatures in our sim-
ulations. The occurrence of phase separation in models
with long-range electron-phonon coupling had been sug-
= 0.55(2). There
(a) λ = 0.325
(b) ξ = 6
(c) ξ = 2
(d) ξ = 6
ξ = 0.5(PI)
ξ = 5(M)
λ = 0.20(M)
λ = 0.45(PI)
λ = 0.55(PS)
L = 14
L = 18
L = 22
L = 26
λ = 0.525
λ = 0.540
λ = 0.545
λ = 0.550
λ = 0.560
(PI, ξ = 0.5) and the metallic phase (M, ξ = 5). (b) Structure factor Sρ(q) at ξ = 6 in the three phases of Fig. 1. We used
L = 22, and β = L (L/2) for λ = 0.2, 0.45 (0.55). (c) Scaling of the charge susceptibility χρ(π) [Eq. (5)] at ξ = 2, defining the
critical point λPI
= 0.33(1) of the Peierls transition. Here β = L. (d) Finite-size scaling of πSρ(q1)/q1 = LSρ(2π/L)/2 with
β = L/2. The divergence for λ ≥ 0.55 indicates phase separation (PS). All results are for ω0/t = 0.5.
(Color online) (a) Density-density correlation function Sρ(r), for λ = 0.325 and βt = L = 22, in the Peierls insulator
gested before  and observed in analytical work [6, 7];
for short-range interactions, it is suppressed by the ab-
sence of bound triplet states , but may occur in the
vicinity of a Mott transition . Phase separation is
expected to be suppressed in the presence of additional
long-range electron-electron interaction .
In combination with analytical continuation , we
can calculate the single-particle spectral function
where |i? is an eigenstate with energy Ei, and ∆ji =
Ej−Ei. Results in the metallic phase (λ = 0.2) are shown
in Fig. 3 for the extreme Holstein (ξ = 0.1) and Fr¨ ohlich
limits (ξ = ∞). The locus of spectral weight follows the
free band dispersion, −2tcosk. The exponentially small
Luther-Emery spin gap is not resolved for the parame-
ters chosen, and the spectrum is particle-hole symmet-
ric. Excitations are sharp inside the coherent interval
[−ω0,ω0], whereas they are substantially broadened as a
result of multiphonon processes at higher energies .
As expected for our 1D model, the spectrum agrees well
with the exact bosonization result , which predicts
a hybridization of the spin, charge and phonon modes,
although spin-charge separation is not visible due to the
weak coupling and small ω0. Comparing Figs. 3(a)
and (b) we see that in contrast to previous work on one
and two electrons [8, 10, 19–22], the impact of the inter-
action range is remarkably small. This important char-
acteristic of the many-electron case can be related to the
absence of significant polaron and bipolaron effects in the
metallic phase of Fig. 1.
Figures 4(a),(b) show A(k,ω) in the Peierls phase
(λ = 0.4). In the Holstein regime (ξ = 0.1), the spec-
trum consists of two sets of features. The cosine band
seen in Fig. 3 has acquired a gap at the Fermi level and
reveals additional, backfolded shadow bands as a result of
dimerization and the corresponding doubling of the unit
cell . These signatures are labeled (1) and (1’) in
Fig. 4(a), respectively. In addition, we find lower-energy
excitations labeled (2) corresponding to bound soliton-
antisoliton pairs or, equivalently, polarons [30, 44], which
are absent in a homogeneous mean-field solution that
captures only (1) and (1’) . The soliton dispersion
indicates a mass larger than the electron mass. Because
their energy at the Fermi level is lower than the Peierls
gap, doping would lead to the formation of solitons .
Increasing the interaction range from ξ = 0.1 to ξ = 4
(a) A(k,ω), ξ = 0.1
(b) A(k,ω), ξ = ∞
A(k,ω) [Eq. (6)] in the metallic phase at λ = 0.2 for (a)
ξ = 0.1, (b) ξ = ∞. Here ω0/t = 0.5, βt = L = 30. The
dashed lines indicate the Fermi level (ω = 0) and ω = ±ω0.
(Color online) Single-particle spectral function
(a) A(k,ω), ξ = 0.1
(b) A(k,ω), ξ = 4
(c) Sρ(q,ω), ξ = 4
tion A(k,ω) in the Peierls phase at λ = 0.4 for (a) ξ = 0.1,
(b) ξ = 4. (c) Dynamical charge structure factor [Eq. (7)] for
the same parameters as in (b). Here ω0/t = 0.5, βt = L = 22.
The dashed lines indicate (a),(b) the Fermi level and (c) ω0.
The labels (1), (1’), and (2) in (a) are explained in the text.
(Color online) (a),(b) Single-particle spectral func-
drives the system into the vicinity of the metal-insulator
transition, see Fig. 1. This is reflected by a much smaller
gap at the Fermi level, reduced spectral weight of the po-
laron excitations, and the suppression of shadow bands.
Consequently, the spectral function becomes quite simi-
lar (but not identical) to that shown in Fig. 3, and illus-
trates the continuous evolution of A(k,ω) across λPI
A hallmark feature of the Peierls state is phonon soft-
ening at q = 2kF, which is visible [30, 46] in the dynami-
(a) ξ = 0.1
(b) ξ = ∞
distance r = L/2 for (a) ξ = 0.1, (b) ξ = ∞. Here ω0/t = 0.5
and λ = 0.2. Lines are fits to a power law f(r) = Ar−η.
(Color online) Charge and pairing correlations at
cal charge structure factor [ˆ ρq=?
reiqr(ˆ nr−?ˆ nr?)/√L]
|?i| ˆ ρq|j?|2e−βEjδ(∆ji− ω).(7)
The results in Fig. 4(c) for λ = 0.4, ξ = 4 [the same
parameters as in Fig. 4(b)] reveal a clear signature of
the renormalized phonon dispersion. The spectrum is
dominated by the soft phonon mode at ω = 0, q = 2kF.
Furthermore, we observe a continuum of particle-hole ex-
citations, and a charge gap at long wavelengths (q → 0).
Finally, we consider the interaction-range effect on the
competition of charge and pairing correlations. Figure 5
shows results for Sρ(r) and the s-wave pair correlator
P(r) = ?∆†
phase. For ξ = 0.1, Fig. 5(a) reflects the dominance of
charge correlations previously observed for the Holstein
model . However, Fig. 5(b) reveals that long-range
electron-phonon interaction (here ξ = ∞) suppresses
charge correlations and thereby results in almost identical
power-law exponents in both channels. Additional short-
range electron-electron repulsion is expected to further
suppress onsite bipolaron formation—promoting nonlo-
cal pairing—and to lead to a more general phase diagram
with Mott, metallic, Peierls and phase-separated ground
states. It will be interesting to explore this issue further,
both at and away from half filling, also in the light of a
recently reported phase of correlated singlets .
Conclusions.—We used exact Monte Carlo simulations
to study many-electron systems with nonlocal and even
long-range electron-phonon interaction.
the Holstein model, extended interactions suppress the
Peierls instability—making pairing more favorable—and
can lead to phase separation.
materials modeling are that interactions of finite but
small range are well described by Holstein-type models,
whereas long-range interactions can have substantial ef-
fects on the balance of pairing and charge correlations.
We are grateful to F. Essler and A. Muramatsu for
helpful discussions, and acknowledge support from the
DFG Grant No. Ho 4489/2-1 as well as computer time at
the LRZ Munich and the J¨ ulich Supercomputing Centre.
r∆0? (with ∆†
r↓) in the metallic
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