Article

# Kondo Effects in Carbon Nanotubes: From SU(4) to SU(2) symmetry

Physical Review B (Impact Factor: 3.77). 08/2006; DOI:10.1103/PhysRevB.74.205119
Source: arXiv

ABSTRACT We study the Kondo effect in a single-electron transistor device realized in a single-wall carbon nanotube. The K-K' double orbital degeneracy of a nanotube, which originates from the peculiar two-dimensional band structure of graphene, plays the role of a pseudo-spin. Screening of this pseudo-spin, together with the real spin, can result in an SU(4) Kondo effect at low temperatures. For such an exotic Kondo effect to arise, it is crucial that this orbital quantum number is conserved during tunneling. Experimentally, this conservation is not obvious and some mixing in the orbital channel may occur. Here we investigate in detail the role of mixing and asymmetry in the tunneling coupling and analyze how different Kondo effects, from the SU(4) symmetry to a two-level SU(2) symmetry, emerge depending on the mixing and/or asymmetry. We use four different theoretical approaches to address both the linear and non-linear conductance for different values of the external magnetic field. Our results point out clearly the experimental conditions to observe exclusively SU(4) Kondo physics. Although we focus on nanotube quantum dots, our results also apply to vertical quantum dots. We also mention that a finite amount of orbital mixing corresponds, in the pseudospin language, to having non-collinear leads with respect to the orbital ''magnetization'' axis which defines the two pseudospin orientations in the nanotube quantum dot. In this sense, some of our results are also relevant to the problem of a Kondo quantum dot coupled to non-collinear ferromagnetic leads. Comment: 17 pages, 15 figures; Updated references, fig13 corrected, typos corrected; to appear in Phys. Rev. B

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##### Article: Tunable Kondo effect in a single donor atom.
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ABSTRACT: The Kondo effect has been observed in a single gate-tunable atom. The measurement device consists of a single As dopant incorporated in a silicon nanostructure. The atomic orbitals of the dopant are tunable by the gate electric field. When they are tuned such that the ground state of the atomic system becomes a (nearly) degenerate superposition of two of the silicon valleys, an exotic and hitherto unobserved valley Kondo effect appears. Together with the "regular" spin Kondo, the tunable valley Kondo effect allows for reversible electrical control over the symmetry of the Kondo ground state from an SU(2) to an SU(4) configuration.
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##### Article: Noisy Kondo impurities
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ABSTRACT: The anti-ferromagnetic coupling of a magnetic impurity carrying a spin with the conduction electrons spins of a host metal is the basic mechanism responsible for the increase of the resistance of an alloy such as Cu${}_{0.998}$Fe${}_{0.002}$ at low temperature, as originally suggested by Kondo . This coupling has emerged as a very generic property of localized electronic states coupled to a continuum . The possibility to design artificial controllable magnetic impurities in nanoscopic conductors has opened a path to study this many body phenomenon in unusual situations as compared to the initial one and, in particular, in out of equilibrium situations. So far, measurements have focused on the average current. Here, we report on \textit{current fluctuations} (noise) measurements in artificial Kondo impurities made in carbon nanotube devices. We find a striking enhancement of the current noise within the Kondo resonance, in contradiction with simple non-interacting theories. Our findings provide a test bench for one of the most important many-body theories of condensed matter in out of equilibrium situations and shed light on the noise properties of highly conductive molecular devices. Comment: minor differences with published version
Nature Physics 01/2009; 5:208. · 19.35 Impact Factor
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##### Thesis: High frequency quantum noise of mesoscopic systems and current-phase relation of hybrid junctions
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ABSTRACT: This thesis discusses two experiments of mesoscopic physics regarding the high frequency quantum noise and the superconducting proximity effect. We nevertheless focused on a single model system: the carbon nanotube. The first experiment aims to measure the high frequency quantum noise of the tube. In order to measure those fluctuations we have designed an original on-chip detection scheme in which the noise source and the detector, a Superconductor/Insulator/Superconductor junction, were coupled through a resonant circuit. This first allowed us to measure the equilibrium noise of the resonator. It exhibits a strong asymmetry between emission and absorption related to zero point fluctuations. We have then measured the out-of-equilibrium emission noise of quasiparticles tunneling of a Josephson junction. It exhibits a strong frequency dependence in agreement with theoretical predictions and allowed us to validate the detection scheme. Finally, the out-of-equilibrium emission noise associated to the Kondo effect (characteristic energy kBTK with TK the Kondo temperature) in a carbon nanotube quantum dot was measured. We find a strong singularity at voltage V=hν/e (ν is the measurement frequency) for frequency ν~kBTK/h. This singularity is related to resonances in the density of states of the dot pinned at the Fermi energy of the leads. At higher frequency hν~3kBTK the singularity vanishes and understood in terms of decoherence effects induced by the bias voltage. In the second experiment, we have developed a technique allowing to measure in the same experiment the current-phase relation and the current-voltage characteristic of a weak link separating two superconductors. We have characterized a carbon nanotube based junction through which a gate tunable current-phase relation was observed. Jointly to a high critical current amplitude, an anharmonic current-phase relation was measured.
10/2011, Degree: PhD, Supervisor: Richard Deblock and Helene Bouchiat